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Related papers: Variational calculations on the hydrogen molecular…

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Three simple $7-, (7+3)-, 10-$parametric trial functions for the ${\rm H}_3^+$ molecular ion are presented. Each of them provides subsequently the most accurate approximation for the Born-Oppenheimer ground state energy among…

Quantum Physics · Physics 2015-05-28 J. C. Lopez Vieyra , A. V. Turbiner , H. Medel Cobaxin

A first detailed study of the ground state of the H$_3^+$ molecular ion in linear configuration, parallel to a magnetic field direction, and its low-lying $\Si,\Pi,\De$ states is carried out for magnetic fields $B=0-4.414 \times 10^{13} $G…

Atomic Physics · Physics 2009-11-11 A. V. Turbiner , N. L. Guevara , J. C. López Vieyra

We present a new computational method for the determination of energy levels in four-particle systems like H$_2$, HD, and HeH$^+$ using explicitly correlated exponential basis functions and analytic integration formulas. In solving the…

Chemical Physics · Physics 2018-02-14 Krzysztof Pachucki , Jacek Komasa

Although the existence of quasi-bound rotational levels of the $X^+ \ ^2\Sigma_g^+$ ground state of H$_2^+$ has been predicted a long time ago, these states have never been observed. Calculated positions and widths of quasi-bound rotational…

Chemical Physics · Physics 2017-01-16 Maximilian Beyer , Frédéric Merkt

Rate coefficients for dissociative recombination and state-to-state rotational transitions of the D$_{2}^{+}$ ion induced by collisions with very low-energy electrons have been reported following our previous studies on HD$^{+}$ and…

Atomic Physics · Physics 2022-03-30 M. D. Epée Epée , O. Motapon , N. Pop , F. Iacob , E. Roueff , I. F. Schneider , J. Zs Mezei

Highly precise variational calculations of non-relativistic energies of the (2p^2)^3P^e state of Helium atom are presented.We get an upper bound energy E=-0.71050015565678 a.u.,the lowest yet obtained.

Atomic Physics · Physics 2009-11-10 Tapan K. Mukherjee , Prasanta K. Mukherjee

Molecular helium represents a benchmark system for testing $\textit{ab initio}$ calculations on few-electron molecules. We report on the determination of the adiabatic ionization energy of the $a\,^3\Sigma_u^+$ state of He$_2$,…

The mass-correction functions in the second-order non-adiabatic Hamiltonian are computed for the $^4$He$^+_2$ molecular ion using the variational method, floating explicitly correlated Gaussian functions, and a general…

Chemical Physics · Physics 2018-12-05 Edit Mátyus

The major goal of the high-precision studies of ro-vibrational states in the hydrogen molecular ions is to provide an alternative way for improving the electron-to-proton mass ratio, or the atomic mass of electron. By now the complete set…

Atomic Physics · Physics 2008-04-16 V. I. Korobov

Using a single trial function we perform an accurate calculation of the ground state $1\sigma_g$ of the hydrogenic molecular ion $H^+_2$ in a constant uniform magnetic field ranging $0-10^{13}$ G. We show that this trial function also makes…

Astrophysics · Physics 2009-10-30 J. C. Lopez , P. O. Hess , A. Turbiner

The relativistic second-order corrections at orders $m\alpha^6$ and $m\alpha^6(m/M)$ in hydrogen molecular ions are calculated. Convergence of numerical results is studied, which allows estimating the relative numerical uncertainty to be…

Atomic Physics · Physics 2025-06-30 Vladimir I. Korobov , Jean-Philippe Karr , Zhen-Xiang Zhong

We present an accurate theoretical determination of rovibrational energy levels of the hydrogen molecule and its isotopologues in its electronic ground state. We consider all significant corrections to the Born-Oppenheimer approximation,…

We describe the current status of high-precision ab initio calculations of the spectra of molecular hydrogen ions (H_2^+ and HD^+) and of two experiments for vibrational spectroscopy. The perspectives for a comparison between theory and…

Atomic Physics · Physics 2017-02-20 B. Roth , J. Koelemeij , S. Schiller , L. Hilico , J. -Ph. Karr , V. I. Korobov , D. Bakalov

Analytic consideration of the Bohr-Oppenheimer (BO) approximation for diatomic molecules is proposed: accurate analytic interpolation for potential curve consistent with its rovibrational spectra is found. It is shown that in the…

Atomic Physics · Physics 2019-08-07 Horacio Olivares-Pilón , Alexander V. Turbiner

An accurate study of the lowest $1\sigma_g$ and the low-lying excited $1\sigma_u$, $1\pi_{u,g}$, $1\delta_{g,u}$ electronic states of the exotic molecular ion $H_3^{2+}$ in linear configuration parallel to a magnetic field is carried out.…

Astrophysics · Physics 2008-11-26 A. V. Turbiner , J. C. López Vieyra , N. L. Guevara

Selected states of the $EF\ ^1\Sigma_\mathrm{g}^+$ electronic manifold of the hydrogen molecule are computed as resonances of the four-body problem. Systematic improvement of the basis representation for the variational treatment is…

Chemical Physics · Physics 2019-10-02 Dávid Ferenc , Edit Mátyus

For rovibronic states corresponding to the $B$ and $B'\ ^1\Sigma_\text{u}^+$ electronic states of the hydrogen molecule, the pre-Born--Oppenheimer (four-particle) non-relativistic energy is converged to a 1-3 parts-per-billion relative…

Chemical Physics · Physics 2023-01-10 Eszter Saly , Dávid Ferenc , Edit Mátyus

We report the potential energy curve, the diagonal Born-Oppenheimer, non-adiabatic mass, relativistic, and leading-order QED corrections for the ground electronic state of the helium dimer cation; the higher-order QED and finite-nuclear…

Chemical Physics · Physics 2026-02-25 Edit Mátyus , Ádám Margócsy

A new state of the H$_2^+$ molecular ion with binding energy of 1.09$\times10^{-9}$ a.u. below the first dissociation limit is predicted, using highly accurate numerical nonrelativistic quantum calculations. It is the first L=0 excited…

The static dipole polarizability for the hydrogen molecular ions H$_2^+$, HD$^+$, and D$_2^+$ are calculated. These new data for polarizability takes into account the leading order relativistic corrections to the wave function of the…

Atomic Physics · Physics 2017-02-01 D. T. Aznabayev , A. K Bekbaev , S. A. Zhaugasheva , V. I. Korobov