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Both the stretch and bend vibrational spectrum and the intensity of infrared transitions in a tetrahedral molecule are studied in a U(2) algebraic model, where the spurious states in the model Hamiltonian and the wavefunctions are exactly…

Chemical Physics · Physics 2009-10-31 Xi-Wen Hou , Shi-Hai Dong , Mi Xie , Zhong-Qi Ma

An algebraic model of Boson-realization is proposed to study the vibrational spectra of a tetrahedral molecule, where ten sets of boson creation and annihilation operators are used to construct the Hamiltonian with $T_{d}$ symmetry. There…

chem-ph · Physics 2009-10-28 Zhong-Qi Ma , Xi-Wen Hou , Mi Xie

The highly excited stretching vibrational energy levels and the intensities of infrared transitions in tetrahedral molecules are studied in a U(2) algebraic model. Its applications to silane and silicon tetrafluoride are presented with…

Chemical Physics · Physics 2007-05-23 Xi-Wen Hou , Zhong-Qi Ma

Double-$\gamma$ vibrations in deformed nuclei are analyzed in the context of the interacting boson model. A simple extension of the original version of the model towards higher-order interactions is required to explain the observed…

Nuclear Theory · Physics 2009-11-06 J. E. Garcia-Ramos , J. M Arias , P. Van Isacker

A general study of excitations up to two-phonon states is carried out using the intrinsic-state formalism of the Interacting Boson Model (IBM). Spectra and transitions for the different dynamical symmetries are analyzed and the…

Nuclear Theory · Physics 2009-10-31 J. E. Garcia-Ramos , C. E. Alonso , J. M. Arias , P. Van Isacker , A. Vitturi

A Fermi resonance-algebraic model is proposed for molecular vibrations, where a U(2) algebra is used for describing the vibrations of each bond, and Fermi resonances between stretching and bending modes are taken into account. The model for…

Chemical Physics · Physics 2015-06-26 Xi-Wen Hou , Shi-Hai Dong , Zhong-Qi Ma

We study the electronic spectral properties in two examples of strongly interacting systems: a Mott-Hubbard insulator with additional electron-boson interactions, and a polaronic semiconductor. An approximate unified framework is developed…

Strongly Correlated Electrons · Physics 2009-11-11 S. Fratini , S. Ciuchi

We present a practical method to compute the vibrational resonant Raman spectra in solids with delocalized excitations. We apply this approach to the study of tetrahedrous amorphous carbon. We determine the vibrational eigenmodes and…

Materials Science · Physics 2009-11-07 Mickael Profeta , Francesco Mauri

The interacting boson model is extended to describe the spectroscopy of superdeformed bands. Microscopic structure of the model in the second minimum is discussed and superdeformed bosons are introduced as the new building blocks. Solutions…

Nuclear Theory · Physics 2009-09-25 S. Kuyucak , M. Honma , T. Otsuka

A general theory of electronic excitations in aggregates of molecules coupled to intramolecular vibrations and the harmonic environment is developed for simulation of the third-order nonlinear spectroscopy signals. The model is applied in…

Chemical Physics · Physics 2014-01-17 Vytautas Butkus , Leonas Valkunas , Darius Abramavicius

Exact and approximate expressions for thermodynamic characteristics of heated matter, which consists of particles with finite mass-widths, are constructed. They are expressed in terms of Fermi/Bose distributions and spectral functions,…

Nuclear Theory · Physics 2008-11-26 D. N. Voskresensky

We calculate the single-particle spectral functions and quasi-particle dispersions for a Bose-Fermi mixture when the boson-fermion attraction is sufficiently strong to suppress completely the condensation of bosons at zero temperature.…

Quantum Gases · Physics 2015-06-16 Elisa Fratini , Pierbiagio Pieri

Spatio-spectral properties of twin beams at their transition from low to high intensities are analyzed in parametric and paraxial approximations using the decomposition into paired spatial and spectral modes. Intensity auto- and…

Quantum Physics · Physics 2016-01-05 Jan Perina

We describe a new approach based on semiclassical molecular dynamics that allows to simulate infrared absorption or emission spectra of molecular systems with inclusion of anharmonic intensities. This is achieved from semiclassical power…

Chemical Physics · Physics 2018-11-12 Marco Micciarelli , Riccardo Conte , Jaime Suarez , Michele Ceotto

In the present work, the analytical description of an intermolecular vibrational energy transfer, analyzed by two dimensional infrared spectroscopy, is established. The energy transfer process takes place between the dark combination states…

Chemical Physics · Physics 2013-09-04 Albert A. Villaeys , Kuo Kan Liang

The transition between the gas-, supercritical-, and liquid-phase behaviour is a fascinating topic which still lacks molecular-level understanding. Recent ultrafast two-dimensional infrared spectroscopy experiments suggested that the…

Chemical Physics · Physics 2023-03-22 Kai Töpfer , Debasish Koner , Shyamsunder Erramilli , Lawrence D. Ziegler , Markus Meuwly

Exploratory simulations of Bose-Fermi mixtures on the three-dimensional optical lattice at finite temperature are performed by adopting the lattice quantum chromodynamics technique. We analyze the bosonic superfluid transition and its…

Quantum Gases · Physics 2012-10-30 Arata Yamamoto , Tetsuo Hatsuda

We study the properties of dilute bosons immersed in a single component Fermi sea across a broad boson-fermion Feshbach resonance. The stability of the mixture requires that the bare interaction between bosons exceeds a critical value,…

Quantum Gases · Physics 2013-05-29 Zeng-Qiang Yu , Shizhong Zhang , Hui Zhai

In this article, we review the charge excitations of heavy fermion compounds probed by infrared spectroscopy. The article is not meant to be a comprehensive survey of experimental investigations. Rather it focuses on the dependence of…

Strongly Correlated Electrons · Physics 2016-05-25 R. Y. Chen , N. L. Wang

Infrared spectroscopy (IR) and quantum chemistry calculations that are based on the density functional theory (DFT) have been used to study the structure, molecular interactions of the nematic and twist-bend phases for thioether-linked…

Soft Condensed Matter · Physics 2022-06-16 Barbara Loska , Antoni Kocot , Yuki Arakawa , G. H. Mehl , Katarzyna Merkel
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