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The tri-layered perovskite Sr4Rh3O10 is reported for the first time. High-pressure and high-temperature heating (6 GPa and 1500 C) brought about successful preparation of a polycrystalline sample of the expected member at n=3 of…

Strongly Correlated Electrons · Physics 2007-05-23 K. Yamaura , Q. Huang , D. P. Young , E. Takayama-Muromachi

The origin of the metal-to-insulator transition in RNiO3 perovskites with trivalent 4f ion has challenged the condensed matter research community for almost three decades. A drawback for progress in this direction has been the lack of…

CaCu$_3$Fe$_4$O$_{12}$ exhibits a temperature-induced transition from a ferrimagnetic-insulating phase, in which Fe appears charge disproportionated, as Fe$^{3+}$ and Fe$^{5+}$, to a paramagnetic-metallic phase at temperatures above 210 K,…

Strongly Correlated Electrons · Physics 2018-08-15 Ivon R. Buitrago , C. I. Ventura , R. Allub

We report a comprehensive investigation of the triple perovskite iridate Ba$_{3}$CoIr$_{2}$O$_{9}$. Stabilizing in the hexagonal $P6_{3}/mmc$ symmetry at room temperature, this system transforms to a monoclinic $C2/c$ symmetry at the…

Strongly Correlated Electrons · Physics 2021-02-03 Charu Garg , Deepak Roy , Martin Lonsky , Pascal Manuel , Antonio Cervellino , Jens Müller , Mukul Kabir , Sunil Nair

Contradictory results of high-pressure studies in cubic bixbyite-type indium oxide (c-In2O3) at room temperature (RT) have motivated us to perform high-pressure powder x-ray diffraction and Raman scattering measurements in this material. On…

Perovskite photovoltaic ABX$_3$ systems are being studied due to their high energy-conversion efficiencies with current emphasis placed on pure inorganic systems. In this work, synchrotron single-crystal diffraction measurements combined…

Barium titanate (BaTiO$_3$) is a prototypical ferroelectric perovskite that undergoes the rhombohedral-orthorhombic-tetragonal-cubic phase transitions as the temperature increases. In this work, we develop a classical interatomic potential…

Materials Science · Physics 2016-11-23 Yubo Qi , Shi Liu , Ilya Grinberg , Andrew M. Rappe

Theoretical DFT calculations using GGA+U and HSE06 frameworks enabled vibrational mode assignment and partial (atomic) phonon DOS determination in KAgF3 perovskite, a low-dimensional magnetic fluoroargentate(II). Twelve bands in the spectra…

Materials Science · Physics 2021-01-20 Kacper Koteras , Jakub Gawraczynski , Mariana Derzsi , Zoran Mazej , Wojciech Grochala

A key challenge for the practical application of metal halide perovskites (MHPs) is the instability of the desired perovskite phase relative to the optically non-active $\delta$ phase. To determine the phase stability, we previously…

Perovskite solid solutions PbHfO3-PbSnO3 offer valuable opportunities for studying the formation mechsnisms of incommensurate phases, owing to the presence of an intermediate (between cubic and incommensurate) phase, which is stabilized in…

Contrary to previous studies that identified the ground state crystal structure of the entire R_3Co series (R is a rare earth) as orthorhombic Pnma, we show that Y_3Co undergoes a structural phase transition at T_t=160K. Single crystal…

Materials Science · Physics 2013-07-18 A. Podlesnyak , G. Ehlers , H. Cao , M. Matsuda , M. Frontzek , O. Zaharko , V. A. Kazantsev , A. F. Gubkin , N. V. Baranov

The archetypal $3d$ Mott insulator hematite, Fe$_2$O$_3$, is one of the basic oxide components playing an important role in mineralogy of Earth's lower mantle. Its high pressure-temperature behavior, such as the electronic properties,…

Strongly Correlated Electrons · Physics 2019-10-07 I. Leonov , G. Kh. Rozenberg , I. A. Abrikosov

We have recently predicted and subsequently verified experimentally by specific heat measurements that EuTiO3 undergoes a structural phase transition at elevated temperature TS = 282 K. The origin of the phase transition has been attributed…

Materials Science · Physics 2012-05-25 J. Köhler , R. Dinnebier , A. Bussmann-Holder

We have performed first principles study for bismuth crystal structure at pressure from 0~14 GPa based on structure search and quasi-harmonic approximation. A new stable phase with Pbcm symmetry is predicted by structure search method. We…

Materials Science · Physics 2019-03-08 Ya-Fan Zhao , Shou-Rui Li , Xing-Yu Gao , Ming-Feng Tian , Hai-Feng Song

Atomic many-body phase transitions and quantum criticality have recently attracted much attention in non-standard optical lattices. Here we perform an experimental study of finite-temperature superfluid transition of bosonic atoms confined…

Quantum Gases · Physics 2019-07-09 Shengjie Jin , Xinxin Guo , Peng Peng , Xuzong Chen , Xiaopeng Li , Xiaoji Zhou

We use first-principles density functional theory calculations to investigate the dielectric response of BaZrO$_3$ perovskite. A previous study [Arkbarzadeh {\em et al.} Phys. Rev. B {\bf 72}, 205104 (2005)] reported a disagreement between…

Materials Science · Physics 2009-11-11 Joseph W. Bennett , Ilya Grinberg , Andrew M. Rappe

Organic-inorganic coupling in the hybrid lead-halide perovskite is a central issue in rationalizing the outstanding photovoltaic performance of these emerging materials. Here we compare and contrast the evolution of structure and dynamics…

We present an extensive investigation (magnetic, electric and thermal measurements and X-ray absorption spectroscopy) of the Pr0.5Ca0.5CoO3 and (Pr1-yYy)0.7Ca0.3CoO3 (y=0.0625-0.15) perovskites, in which a peculiar metal-insulator (M-I)…

Materials Science · Physics 2015-06-12 J. Hejtmanek , Z. Jirak , O. Kaman , K. Knizek , E. Santava , K. Nitta , T. Naito , H. Fujishiro

The structural phase transition in hexagonal BaMnO$_3$ occurring at $T_c$=130 K was studied in ceramic samples using electron and X-ray diffraction, second harmonic generation as well as by dielectric and lattice dynamic spectroscopies. The…

A realistic theory of the quantum paraelectric - ferroelectric transition is presented, involving parameters determined from band calculations and a renormalization group treatment of critical fluctuations. The effects of reduced…

Strongly Correlated Electrons · Physics 2007-05-23 R. Roussev , A. J. Millis