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We developed a mid-infrared optical frequency comb-based Fourier-transform spectrometer and performed a line-shape study of the fundamental vibrational band of CO perturbed by N${_2}$, which is crucial for atmospheric science and…

We describe a tunable broadband mid-infrared laser source based on difference-frequency mixing of a 100 MHz femtosecond Yb:fiber laser oscillator and a Raman-shifted soliton generated with the same laser. The resulting light is tunable over…

Optics · Physics 2015-05-30 Tyler W. Neely , Todd A. Johnson , Scott A. Diddams

Frequency-modulated diode laser transient absorption spectra of the ethynyl radical have been recorded at wavelengths close to 1.66 $\mu$m. The observed spectrum includes strong, regular, line patterns. The two main bands observed originate…

Chemical Physics · Physics 2020-12-29 Eisen C. Gross , Anh. T. Le , Gregory E. Hall , Trevor J. Sears

Sensing with undetected photons has become a vibrant, application-driven research domain with a special focus on the mid-infrared (mid-IR) wavelength region. Since the mid-IR contains spectral bands with highly specific and strong molecular…

Theoretical results are presented which show that noiseless phase quadrature amplification is possible, and limited experimentally only by the efficiency of the phase detection system. Experimental results obtained using a Nd:YAG laser show…

Quantum Physics · Physics 2009-10-31 Ben C. Buchler , Elanor H. Huntington , Timothy C. Ralph

In this article, we report the first observation of nanosecond laser induced transient dual absorption bands, one in the bandgap (TA1) and another in the sub-bandgap (TA2) regions of a-Ge5As30Se65 thin films. Strikingly, these bands are…

Materials Science · Physics 2015-09-25 Pritam Khan , Tarun Saxena , K. V. Adarsh

Self diffraction is a four-wave mixing process proportional to the square modulus of third-order nonlinearity susceptibility $\chi^{(3)}$, which is related to the material's electronic and thermal properties. In this study, we investigate…

In a frequency-modulation spectroscopy experiment, using the radiation from a single frequency diode laser, the spectra of molecular iodine hyperfine structure near 640 nm were recorded on the transition $B^3\Pi_{0_u^{+}}-X^1\Sigma^+_{g}$.…

Dispersive Fourier transformation is a powerful technique in which spectral information is mapped into the time domain using chromatic dispersion. It replaces a spectrometer with an electronic digitizer, and enables real-time spectroscopy.…

Optics · Physics 2009-11-13 J. Chou , D. R. Solli , B. Jalali

Nonlinear absorption of femtosecond laser pulses provides a unique opportunity to confine energy deposition in any medium to a region that is below the focal diameter of a pulse. Illumination of a polymer film through a transparent high…

We present a new design of a Fourier Domain Mode Locked laser (FDML laser), which provides a new record in sweep range at ~1um center wavelength: At the fundamental sweep rate of 2x417 kHz we reach 143nm bandwidth and 120nm with 4x…

Numerous molecules exhibit unique absorption bands in the fingerprint infrared (IR) region, allowing chemical identification and detection. This makes IR spectroscopy an essential tool in biomedical diagnostics, sensing, and material…

Optics · Physics 2022-02-04 Anna V. Paterova , Zi S. D. Toa , Hongzhi Yang , Leonid A. Krivitsky

We demonstrate 14.3-attosecond timing jitter [integrated from 10 kHz to 94 MHz offset frequency] optical pulse trains from 188-MHz repetition-rate mode-locked Yb-fiber lasers. In order to minimize the timing jitter, we shorten the non-gain…

We describe an all-fiber nonlinear interferometer based on four-wave mixing in highly nonlinear fiber. Our configuration realizes phase-sensitive interference with 97% peak visibility and >90% visibility over a broad 554 GHz optical band.…

Instrumentation and Detectors · Physics 2018-08-28 Joseph M. Lukens , Raphael C. Pooser , Nicholas A. Peters

We report the detection of strong absorption by interstellar hydrogen fluoride along the sight-line to the submillimeter continuum source G10.6-0.4 (W31C). We have used Herschel's HIFI instrument, in dual beam switch mode, to observe the…

Multiphoton microscopes employ femtosecond lasers as light sources because the high peak power of the ultrashort pulse allows for multiphoton excitation of fluorescence in the examined sample. However, such short pulses are susceptible to…

Optics · Physics 2024-08-13 Katarzyna Kunio , Jakub Bogusławski , Grzegorz Soboń

With electron beam durations down to femtoseconds and sub-femtoseconds achievable in current state-of-the-art accelerators, longitudinal bunch length diagnostics with resolution at the attosecond level are required. In this paper, we…

Mid-infrared spectroscopy probes molecular vibrations to identify chemical species and functional groups. Therefore, mid-infrared hyperspectral imaging is one of the most powerful and promising candidates for chemical imaging using optical…

Optics · Physics 2023-07-06 Yue Zhao , Shota Kusama , Yuji Furutani , Wei-Hong Huang , Chih-Wei Luo , Takao Fuji

A metamaterial perfect absorber consisting of a tri-layer (Al/ZnS/Al) metal-dielectric-metal system with top aluminium nano-disks is fabricated by laser-interference lithography and lift-off processing. The metamaterial absorber had peak…

Optics · Physics 2018-11-02 Sriram Guddala , Raghwendra Kumar , S. Anantha Ramakrishna

We extend the powerful frequency-domain analysis of femtosecond two-photon absorption to the intermediate-field regime, which involves both two- and four-photon transitions. Consequently, we find a broad family of shaped pulses that enhance…

Atomic Physics · Physics 2008-02-20 Lev Chuntonov , Leonid Rybak , Andrey Gandman , Zohar Amitay
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