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We investigate conformations and dynamics of a polymer considering its monomers to be active Brownian particles. This active polymer shows very intriguing physical behavior which is absent in an active Rouse chain. The chain initially…

Soft Condensed Matter · Physics 2020-04-13 Shalabh K. Anand , Sunil P. Singh

We report molecular dynamics simulations of the segregation of two overlapping chains in cylindrical confinement. We find that the entropic repulsion between the chains can be sufficiently strong to cause segregation on a time scale that is…

Soft Condensed Matter · Physics 2011-11-09 Axel Arnold , Suckjoon Jun

We propose a two-body spherically symmetric (isotropic) potential such that particles interacting by the potential self assemble into linear semiflexible polymeric chains without branching. By suitable control of the potential parameters we…

Soft Condensed Matter · Physics 2018-05-09 Alex Abraham , Apratim Chatterji

The aim of this paper is twofold: - To give an elementary and self-contained proof of an explicit formula for the free energy for a general class of polymer chains interacting with an environment through periodic potentials. This…

Probability · Mathematics 2007-05-23 Francesco Caravenna , Giambattista Giacomin , Lorenzo Zambotti

Monte Carlo simulations are used to study the conformational properties of a folded semiflexible polymer confined to a long channel. We measure the variation in the conformational free energy with respect to the end-to-end distance of the…

Soft Condensed Matter · Physics 2018-09-05 James M. Polson

We consider a fully directed self-avoiding walk model on a cubic lattice to mimic the conformations of an infinitely long confined flexible polymer chain; and the confinement condition is achieved by two parallel athermal plates. The…

Soft Condensed Matter · Physics 2021-06-21 P K Mishra

We analyze static properties of a strongly confined semiflexible polymer, i.e. either trapped in a closed space or compressed by external forces, in an athermal solvent. Like a flexible polymer case, we can resort to an analogy with the…

Soft Condensed Matter · Physics 2009-11-13 Takahiro Sakaue

We calculate the two, three, four, and five-body (state independent) effective potentials between the centers of mass (CM) of self avoiding walk polymers by Monte-Carlo simulations. For full overlap, these coarse-grained n-body interactions…

Soft Condensed Matter · Physics 2009-11-07 P. G. Bolhuis , A. A. Louis , J. P. Hansen

Monte Carlo computer simulations are used to study the segregation behaviour of two polymers under cylindrical confinement. Using a multiple-histogram method, the conformational free energy, F, of the polymers was measured as a function of…

Soft Condensed Matter · Physics 2018-05-24 James M. Polson , Deanna R. -M. Kerry

We analyse the nature of the confinement of an infinitely long (and finite) linear semiflexible homo-polymer chain confined in between two geometrical constraints (A&B) under good solvent condition in two dimensions. The constraints are…

Soft Condensed Matter · Physics 2017-10-16 Pramod Kumar Mishra

Monte Carlo simulations are used to study the translocation of a polymer into a cavity. Modeling the polymer as a hard-sphere chain with a length up to N=601 monomers, we use a multiple-histogram method to measure the variation of the…

Soft Condensed Matter · Physics 2021-03-25 James M. Polson , David R. Heckbert

The free energy cost of confining a star polymer where $f$ flexible polymer chains containing $N$ monomeric units are tethered to a central unit in a slit with two parallel repulsive walls a distance $D$ apart is considered, for good…

Soft Condensed Matter · Physics 2013-10-29 J. Paturej , A. Milchev , S. A. Egorov , K. Binder

Despite its limitations, mainly due to its simplicity, Flory theory has been extended to many other important cases, e.g., linear chains with stiffness and polymers of various topology in a confined space. Surprisingly, the severe…

Soft Condensed Matter · Physics 2007-05-23 Suckjoon Jun , Bae-Yeun Ha

We study the swelling of a flexible linear chain composed of active particles by analytical theory and computer simulation. Three different situations are considered: a free chain, a chain confined to an external harmonic trap, and a chain…

Soft Condensed Matter · Physics 2015-03-31 Andreas Kaiser , Sonja Babel , Borge ten Hagen , Christian von Ferber , Hartmut Löwen

Monte Carlo simulations are used to study the conformational behavior of a semiflexible polymer confined to cylindrical and conical channels. The channels are sufficiently narrow that the conditions for the Odijk regime are marginally…

Soft Condensed Matter · Physics 2020-12-02 James M. Polson , Cameron G. Hastie

We consider the problem of an ideal polymer confined in a droplet. When the droplet radius is smaller than the (unconfined) polymer radius of gyration, the polymer entropy will depend on the droplet shape. We compute the resulting surface…

Condensed Matter · Physics 2009-10-28 M. Goulian , S. T. Milner

We investigate the tight packing of nematic polymers inside a confining hard sphere. We model the polymer {\sl via} the continuum Frank elastic free energy augmented by a simple density dependent part as well as by taking proper care of the…

Soft Condensed Matter · Physics 2010-05-05 Daniel Svenšek , Gregor Veble , Rudolf Podgornik

The massive field theory approach in fixed space dimensions $d=3$ is applied to investigate a dilute solution of long-flexible polymer chains in a good solvent between two parallel repulsive walls, two inert walls and for the mixed case of…

Soft Condensed Matter · Physics 2009-10-08 D. Romeis , Z. Usatenko

We consider a binary system of small and large spheres of finite size in a continuous medium interacting via a non-negative potential. We work in the canonical ensemble and compute upper and lower bound for the free energy at finite and…

Mathematical Physics · Physics 2023-10-24 Tong Xuan Nguyen , Giuseppe Scola , Dimitrios Tsagkarogiannis

We demonstrate that a highly charged polyelectrolyte confined in a spherical cavity undergoes reversible transformations between amorphous conformations to a four-fold symmetry morphology as a function of dielectric mismatch between the…

Soft Condensed Matter · Physics 2019-08-20 Trung Dac Nguyen , Monica Olvera de la Cruz