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Optical atomic clocks with unrivaled precision and accuracy have advanced the frontier of precision measurement science and opened new avenues for exploring fundamental physics. A fundamental limitation on clock precision is the Standard…

Quantum Physics · Physics 2025-11-11 Y. A. Yang , Maya Miklos , Yee Ming Tso , Stella Kraus , Joonseok Hur , Jun Ye

Optical transitions of highly charged ions can be very sensitive to hypothetical beyond-the-Standard-Model phenomena. Those near the $5s-4f$ level crossing, where the $5s$ and $4f$ are degenerate are especially promising. We present…

We report the observation of the higher order frequency shift due to the trapping field in a $^{87}$Sr optical lattice clock. We show that at the magic wavelength of the lattice, where the first order term cancels, the higher order shift…

Atomic Physics · Physics 2016-08-16 Anders Brusch , Rodolphe Le Targat , Xavier Baillard , Mathilde Fouché , Pierre Lemonde

We present a comprehensive study of the frequency shifts associated with the lattice potential for a Sr lattice clock. By comparing two such clocks with a frequency stability reaching $5\times 10^{-17}$ after a one hour integration time,…

We show that optical spectroscopy of Rydberg states can provide accurate {\em in situ} thermometry at room-temperature. Transitions from a metastable state to Rydberg states with principal quantum numbers of 25 to 30 have 200 times larger…

Quantum Physics · Physics 2011-08-24 Vitali D. Ovsiannikov , Andrei Derevianko , Kurt Gibble

Accurate calculations of electric dipole polarizabilities ($\alpha_d$), quadrupole moments ($\Theta$), and quadrupole polarizabilities ($\alpha_q$) for the clock states of the singly charged calcium (Ca$^+$) and ytterbium (Yb$^+$) ions are…

Atomic Physics · Physics 2025-02-11 YanMei Yu , B. K. Sahoo

The frequency comb created by a femtosecond mode-locked laser and a microstructured fiber is used to phase coherently measure the frequencies of both the Hg^+ and Ca optical standards with respect to the SI second as realized at NIST. We…

The energy levels and electric dipole ($E1$) matrix elements of the ground state and low-lying excited states of Be atoms are calculated using the relativistic configuration interaction plus core polarization (RCICP) method. The static and…

Atomic Physics · Physics 2023-03-30 Lei Wu , Xia Wang , Ting Wang , Jun Jiang , Chenzhong Dong

Optical frequency standards, lasers stabilized to atomic or molecular transitions, are widely used in length metrology and laser ranging, provide a backbone for optical communications and lie at the heart of next-generation optical atomic…

We demonstrate a technique to measure hyperfine structure using a frequency-stabilized diode laser and an acousto-optic modulator locked to the frequency difference between two hyperfine peaks. We use this technique to measure hyperfine…

Atomic Physics · Physics 2007-05-23 Umakant D. Rapol , Anusha Krishna , Vasant Natarajan

Precision measurements of the Lu$^+$ $^3D_1$ and $^3D_2$ quadrupole moments have been carried out giving $\Theta(^3D_1)=0.63862(74)\,e a_0^2$ and $\Theta(^3D_2)=0.8602(14)\,e a_0^2$, respectively. The measurements utilize the differential…

Atomic Physics · Physics 2020-11-04 R. Kaewuam , T. R. Tan , Zhiqiang Zhang , K. J. Arnold , M. S. Safronova , M. D. Barrett

A full evaluation of the uncertainty budget for the ytterbium ion optical clock at the National Physical Laboratory (NPL) was performed on the electric octupole (E3) $^2\mathrm{S}_{1/2}\,\rightarrow\, ^2\mathrm{F}_{7/2}$ transition. The…

The pursuit of better atomic clocks has advanced many research areas, providing better quantum state control, new insights in quantum science, tighter limits on fundamental constant variation, and improved tests of relativity. The record…

By varying the density of an ultracold $^{88}$Sr sample from $10^9$ cm$^{-3}$ to $> 10^{12}$ cm$^{-3}$, we make the first definitive measurement of the density-related frequency shift and linewidth broadening of the $^1S_0$ - $^3P_1$…

Atomic Physics · Physics 2009-11-10 Tetsuya Ido , Thomas H. Loftus , Martin M. Boyd , Andrew D. Ludlow , Kevin W. Holman , Jun Ye

Optical clocks have extremely attractive applications in many fields, including time-frequency metrology, validation of fundamental physical principles, and relativistic geodesy. The 467 nm octupole transition in 171Yb+ ion exhibits…

Atomic Physics · Physics 2025-10-14 Xuanjian Wang , Jian Cao , Hualin Shu , Yi Yuan , Zehao Li , Pengcheng Fang , Qunfeng Chen , Xueren Huang

Hyperfine structure $A$ and $B$ factors of the atomic $5s\,5p\,\; ^3\rm{P}_2 \rightarrow 5s\,6s\,\; ^3\rm{S}_1$ transition are determined from collinear laser spectroscopy data of $^{107-123}$Cd and $^{111m-123m}$Cd. Nuclear magnetic…

The electric dipole-forbidden, quadrupole 6S1/2 <-> 5D3/2 transition in Ba+ near 2051 nm, with a natural linewidth of 13 mHz, is attractive for potential observation of parity non-conservation, and also as a clock transition for a barium…

We perform detailed calculations of the electronic structure of the Os$^{16+}$ ion and demonstrate that it has several metastable states which can be used for very accurate optical clocks. The clocks are highly sensitive to manifestations…

Atomic Physics · Physics 2024-02-21 V. A. Dzuba , V. V. Flambaum

A black-body radiation (BBR) shifts of (nsnp ^3P_0) - (ns^2 ^1S_0) clock transition in divalent atoms Mg, Ca, Sr, and Yb are evaluated. A theory of multipolar BBR shifts is developed and its implications are discussed. At room temperatures,…

Atomic Physics · Physics 2009-11-11 Sergey G. Porsev , Andrei Derevianko

We propose and experimentally demonstrate a scheme which effects hyperfine averaging during a Ramsey interrogation of a clock transition. The method eliminates the need to average over multiple optical transitions, reduces the sensitivity…

Quantum Physics · Physics 2020-03-04 R. Kaewuam , T. R. Tan , K. J. Arnold , S. R. Chanu , Zhiqiang Zhang , M. D. Barrett