Related papers: Optical frequency standard with $Sr^+$: A theoreti…
We report on spectroscopy of the low-lying electronic transitions in $^{224}$Ra$^+$. The ion's low charge to mass ratio and convenient wavelengths make $^{224}$Ra$^+$ a promising optical clock candidate. We measured the frequencies of the…
Electrometry is performed using Rydberg states to evaluate the quadratic Stark shift of the $5s^2$ $^1\textrm{S}_0-5s5p$ $^3\textrm{P}_0$ clock transition in strontium. By measuring the Stark shift of the highly excited…
We report precision measurement of the unperturbed ${^{3}}D_1$ microwave transition frequencies in $^{176}\mathrm{Lu}^+$ to a fractional uncertainty of $4\times10^{-14}$. We find the $|F,m_F\rangle=|8,0\rangle$ to $|7,0\rangle$ hyperfine…
We report the first direct frequency comparison between two multi-ion optical clocks based on the S$_{1/2}$ to D$_{5/2}$ transition in \Ca and \Sr ions. Using linear chains of up to nine \Ca ions and six \Sr ions, we demonstrate improved…
Motivated by the prospect of an optical frequency standard based on 43Ca+, we calculate the blackbody radiation (BBR) shift of the 4s_1/2-3d_5/2 clock transition, which is a major component of the uncertainty budget. The calculations are…
Transition frequencies of atoms and ions are among the most accurately accessible quantities in nature, playing important roles in pushing the frontiers of science by testing fundamental laws of physics, in addition to a wide range of…
It is shown that the dynamic differential scalar polarisability of the $S_{1/2}-D_{5/2}$ transition in $^{138}$Ba$^+$ can be determined to an inaccuracy below $0.5\%$ across a wide wavelength range ($\lambda>700\,\mathrm{nm}$). This can be…
We report high-precision frequency ratio measurements between optical atomic clocks based on $^{27}$Al$^+$, $^{171}$Yb, and $^{87}$Sr. With total fractional uncertainties at or below $3.2 \times 10^{-18}$, these measurements meet an…
We propose In-like Pr10+ as a candidate for the development of a high-accuracy optical clock with high sensitivity to a time variation of the fine-structure constant, (\dot alpha}/alpha, as well as favorable experimental systematics. We…
We present a measurement of the absolute frequency of the 5s$^2$ $^1$S$_0$ to 5s5p $^3$P$_0$ transition in $^{87}$Sr, which is a secondary representation of the SI second. We describe the optical lattice clock apparatus used for the…
We analyze an optical atomic clock using two-photon $5S_{1/2} \rightarrow 4D_J$ transitions in rubidium. Four one- and two-color excitation schemes to probe the fine-structure states $4D_{3/2}$ and $4D_{5/2}$ are considered in detail. We…
Optical frequency comparison of the 40Ca+ clock transition \nu_{Ca} (2S1/2-2D5/2, 729nm) against the 87Sr optical lattice clock transition \nu_{Sr}(1S0-3P0, 698nm) has resulted in a frequency ratio \nu_{Ca} / \nu_{Sr} = 0.957 631 202 358…
We report on the first absolute transition frequency measurement at the 10^{-15} level with a single, laser-cooled 40Ca+ ion in a linear Paul trap. For this measurement, a frequency comb is referenced to the transportable Cs atomic fountain…
An optical atomic clock scheme is developed that utilizes two lasers to establish coherent coupling between the $5s^2 \phantom{}^1S_0$ ground state of $^{88}$Sr and the first excited state, $5s5p \phantom{}^3P_0$. The coupling is mediated…
By combining our theoretical calculation and recently measured electric quadrupole hyperfine structure constant of the $3d ^2D_{5/2}$ state in the singly ionized $^{43}$Ca, we determine its nuclear quadrupole moment to one percent accuracy.…
We report the first operation of a Ra$^{+}$ optical clock, a promising high-performance clock candidate. The clock uses a single trapped $^{226}$Ra$^{+}$ ion and operates on the $7s\ ^2S_{1/2}\rightarrow$ $6d\ ^2D_{5/2}$ electric quadrupole…
An atom exposed to an electric field will experience Stark shifts of its internal energy levels, proportional to their polarizabilities. In optical frequency metrology, the Stark shift due to background black-body radiation (BBR) modifies…
Improvements in atom-light coherence are foundational to progress in quantum information science, quantum optics, and precision metrology. Optical atomic clocks require local oscillators with exceptional optical coherence due to the…
Recent experimental progress in cooling, trapping, and quantum logic spectroscopy of highly-charged ions (HCIs) made HCIs accessible for high resolution spectroscopy and precision fundamental studies. Based on these achievements, we explore…
The hyperfine structure of the S1/2-D5/2 quadrupole transition at 729 nm in 43Ca+ has been investigated by laser spectroscopy using a single trapped 43Ca+ ion. We determine the hyperfine structure constants of the metastable level as…