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Nonlinear terahertz (THz) spectroscopy relies on the interaction of matter with few-cycle THz pulses of electric field amplitudes up to megavolts/centimeter (MV/cm). In condensed-phase molecular systems, both resonant interactions with…

Chemical Physics · Physics 2021-12-08 Klaus Reimann , Michael Woerner , Thomas Elsaesser

Using a 3D fully-vectorial nonlinear time-domain analysis we numerically investigate the generation of terahertz radiation by pumping a photonic crystal microcavity out of resonance. High quality factors and a quadratic susceptibility lead…

Optics · Physics 2009-11-11 Andrea Di Falco , Claudio Conti , Gaetano Assanto

Photoinduced Kerr rotation by more than $\pi /2$ radians is demonstrated in planar quantum well microcavity in the strong coupling regime. This result is close to the predicted theoretical maximum of $\pi $. It is achieved by engineering…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 R. V. Cherbunin , M. Vladimirova , K. V. Kavokin , A. V. Mikhailov , N. E. Kopteva , P. G. Lagoudakis , A. V. Kavokin

We analyse the correlation and spectral properties of two-photon states resonantly transmitted by a non-linear optical microcavity. We trace the correlation properties of transmitted two-photon states to the decay spectrum of multi-photon…

Quantum Physics · Physics 2014-10-01 Y. Sherkunov , David M. Whittaker , Henning Schomerus , Vladimir Fal'ko

The problem of pattern formation in resonantly-enhanced near-field lithography by the use of dielectric or plasmonic planar resonators is investigated. Sub-diffraction-limited bright or dark spots can be produced by taking advantage of the…

Optics · Physics 2008-04-22 Mankei Tsang , Demetri Psaltis

Dynamic phase-only beam shaping with a liquid crystal spatial light modulator is a powerful technique for tailoring the beam's intensity profile or wave front. While shaping and controlling the light field is a highly researched topic,…

Nonlinear processes can offer pathways to next-generation sensors and frequency mixing devices to overcome modern imaging, detection, and communication challenges. In this article, we report on strong second and third-order nonlinear…

We demonstrate third harmonic generation in plasmonic antennas made of highly doped germanium and designed to be resonant in the mid infrared. Owing to the near-field enhancement, the result is an ultrafast, sub-diffraction, coherent light…

In recent years, electro-optic sampling, which is based on Pockel's effect between an electromagnetic mode and a copropagating, phase-matched ultrashort probe, has been largely used for the investigation of broadband quantum states of…

Quantum Physics · Physics 2023-10-03 Francesca Fabiana Settembrini , Alexa Herter , Jèrôme Faist

We show that a dimer made of two gold nanospheres exhibits a remarkable efficiency for second-harmonic generation under femtosecond optical excitation. The detectable nonlinear emission for the given particle size and excitation wavelength…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 A. Slablab , L. Le Xuan , M. Zielinski , Y. de Wilde , V. Jacques , D. Chauvat , J. -F. Roch

Periodically structured materials can sustain both optical and mechanical excitations which are tailored by the geometry. Here we analyze the properties of dispersively coupled planar photonic and phononic crystals: optomechanical crystals.…

While two-dimensional (2D) materials have intriguing second-order nonlinearities with ultrahigh coefficient and electrical tunability, their atomic layer thicknesses hinder explorations of other optical frequency-conversions (OFCs) than…

We consider theoretically nonlinear effects in a semiconductor quantum well embedded inside a photonic microcavity. Two-photon absorption by a 2p exciton state is considered and investigated; the matrix element of two-photon absorption is…

Mesoscale and Nanoscale Physics · Physics 2016-12-21 A. A. Pervishko , T. C. H. Liew , V. M. Kovalev , I. G. Savenko , I. A. Shelykh

A new and efficient method for orientation echo spectroscopy is presented and realized experimentally. The excitation scheme utilizes concerted rotational excitations by both ultrashort terahertz and near-IR pulses and its all-optical…

Chemical Physics · Physics 2022-12-07 Ran Damari , Amit Beer , Sharly Fleischer

One challenge of using nonlinear optical phenomena for practical applications is the need to perform phase-matching. Recently, epsilon-near-zero materials have been shown to demonstrate strong optical nonlinearities, in addition to their…

Optics · Physics 2024-07-30 Kyle Wynne , Marjan Bazian , Mark C. Harrison

A technique for obtaining efficient bulk second order susceptibility in non centro-symmetric Photonic Crystals (PC) made from centro-symmetric materials is discussed. The effect is based on the electric quadrupole effect, strong…

Optics · Physics 2009-11-07 A. Feigel , Z. Kotler , B. Sfez

Plasmon modes of a two-dimensional lattice of long conducting circular wires are investigated by using an embedding technique to solve Maxwell's equations rigorously. The frequency-dependent density of states is calculated for various…

Materials Science · Physics 2007-05-23 J. M. Pitarke , J. E. Inglesfield , N. Giannakis

We investigate the effect of phase modulation of laser beams on the coherent and incoherent non-linear signals arising from the interaction of femtosecond pulses with matter. We observe that two collinear beams, whose phases are modulated…

Optics · Physics 2015-05-29 Khadga Jung Karki , Loni Kringle , Andrew H. Marcus , Tõnu Pullerits

Out-of-plane gap solitons in 2D photonic crystals are optical beams localized in the plane of periodicity of the medium and delocalized in the orthogonal direction, in which they propagate with a nonzero velocity. We study such gap solitons…

Pattern Formation and Solitons · Physics 2012-02-17 Tomas Dohnal , Willy Doerfler

We study the formation of second harmonic double-resonance cones in hyperbolic metamaterials. An electric dipole on the surface of the structure induces second harmonic light to propagate into two distinct volume plasmon-polariton channels:…