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Related papers: Coherent Control of Ultracold Collisions with Chir…

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We present results on coherent control of ultracold trap-loss collisions using 40 ns pulses of nonlinearly frequency-chirped light. The chirps, either positive or negative, sweep ~1 GHz in 100 ns and are centered at various detunings below…

Atomic Physics · Physics 2015-05-28 J. A. Pechkis , J. L. Carini , C. E. Rogers , P. L. Gould , S. Kallush , R. Kosloff

We use frequency-chirped light on the nanosecond time scale to produce ultracold $^{87}$Rb$_{2}$ molecules in the lowest triplet state via the process of photoassociation. Comparing to quantum simulations of the molecular formation, we…

Atomic Physics · Physics 2015-06-11 J. L. Carini , J. A. Pechkis , C. E. Rogers , P. L. Gould , S. Kallush , R. Kosloff

We report on the dynamics of ultracold collisions induced by near-resonant frequency-chirped light. A series of identical chirped pulses, separated by a variable delay, is applied to an ultracold sample of 85Rb, and the rate of inelastic…

Atomic Physics · Physics 2009-11-13 M. J. Wright , J. A. Pechkis , J. L. Carini , P. L. Gould

We describe experiments and associated quantum simulations involving the production of ultracold $^{87}$Rb$_{2}$ molecules with nanosecond pulses of frequency-chirped light. With appropriate chirp parameters, the formation is dominated by…

Atomic Physics · Physics 2016-06-07 J. L. Carini , S. Kallush , R. Kosloff , P. L. Gould

We have studied the effects of chirped femtosecond laser pulses on the formation of ultracold molecules in a Rb magneto-optical trap. We have found that application of chirped femtosecond pulses suppressed the formation of 85Rb-2 and 87Rb-2…

Atomic Physics · Physics 2009-11-11 Benjamin L. Brown , Alexander J. Dicks , Ian A. Walmsley

We demonstrate that judicious shaping of a nanosecond-time-scale frequency chirp can dramatically enhance the formation rate of ultracold $^{87}$Rb$_{2}$ molecules. Starting with ultracold $^{87}$Rb atoms, we apply pulses of…

Atomic Physics · Physics 2016-02-26 J. L. Carini , S. Kallush , R. Kosloff , P. L. Gould

Coherent control of atomic and molecular scattering relies on the preparation of colliding particles in superpositions of internal states, establishing interfering pathways that can be used to tune the outcome of a scattering process.…

Atomic Physics · Physics 2024-12-20 Adrien Devolder , Timur V. Tscherbul , Paul Brumer

Coherent control of ultrafast molecule making from colliding reactants is crucial for realizing coherent control of binary photoreactions (CCBP). To handle diverse excitation scenarios, feasibility with both weak and strong fields is…

Chemical Physics · Physics 2024-11-08 Moran Geva , Yonathan Langbeheim , Arie Landau , Zohar Amitay

Inelastic interaction between coherent light with constant frequency and free electrons enables periodic phase modulation of electron wave packets leading to periodic side-bands in the electron energy spectra. In this Letter we propose a…

Coherent wave control exploits the interference among multiple waves impinging on a system to suppress or enhance outgoing signals based on their relative phase and amplitude. This process inherently requires non-Hermiticity, in order to…

We consider controlled collisions between two ultracold atoms guided by external harmonic potentials. We derive analytical solutions of the Schroedinger equation for this system, and investigate the properties of eigenergies and eigenstates…

Quantum Gases · Physics 2009-10-30 Michał Krych , Zbigniew Idziaszek

We demonstrate for the first time coherent control of bond making, a milestone on the way to coherent control of photo-induced bimolecular chemical reactions. In strong-field multiphoton femtosecond photoassociation experiments, we find the…

We demonstrate and characterize that a carrier-envelope-phase (CEP)-controlled ultrashortchirped field is an efficient and robust mechanism to modify the dissociation dynamics of molecularhydrogen. Different dissociation pathways are…

Atomic Physics · Physics 2019-12-11 S. A. Karakaş , P. Rosenberger , M. F. Ciappina , M. F. Kling , İ. Yavuz

We consider the coherent control of ultracold molecule-molecule scattering, impacted by a dense set of rovibrational resonances. To characterize the resonance spectrum, a rudimentary model based on multichannel quantum defect theory has…

Atomic Physics · Physics 2023-01-18 Adrien Devolder , Timur V. Tscherbul , Paul Brumer

We show that quantum interference-based coherent control is a highly efficient tool for tuning ultracold molecular collision dynamics, and is free from the limitations of commonly used methods that rely on external electromagnetic fields.…

Atomic Physics · Physics 2021-04-21 Adrien Devolder , Paul Brumer , Timur V. Tscherbul

We study the effect of the chirped laser pulse on the transmission and associated ion acceleration by the sub-wavelength target. In the chirped laser pulses, the pulse frequency has a temporal variation about its fundamental frequency,…

Plasma Physics · Physics 2018-11-06 Shivani Choudhary , Amol R. Holkundkar

Quantum coherent control of bimolecular collisions beyond the ultracold regime can face a major challenge due to the incoherent addition of different partial wave contributions to the total scattering cross section. These contributions…

Atomic Physics · Physics 2023-06-26 Adrien Devolder , Paul Brumer , Timur Tscherbul

The dynamics of two traps with ultracold atoms and connected by Josephson type coupling, is shown to exhibit a transition from dispersive dynamics to localized coherent oscillations. This transition is controlled by coupling strength and…

Statistical Mechanics · Physics 2007-05-23 N. M. Bogoliubov , J. Timonen , M. B. Zvonarev

We show how to emulate a conventional pump-probe scheme using a single frequency-chirped ultrashort UV pulse to obtain a time-resolved image of molecular ultrafast dynamics. The chirp introduces a spectral phase in time that encodes the…

Chemical Physics · Physics 2017-05-03 Denis Jelovina , Johannes Feist , Fernando Martín , Alicia Palacios

Reciprocity is a universal principle that has a profound impact on many areas of physics. A fundamental phenomenon in condensed-matter physics, optical physics and acoustics, arising from reciprocity, is the constructive interference of…

Optics · Physics 2016-02-24 Y. Bromberg , B. Redding , S. M. Popoff , H. Cao
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