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We demonstrate experimentally a method of varying the degree of directionality in laser-induced molecular rotation. To control the ratio between the number of clockwise and counter-clockwise rotating molecules (with respect to a fixed…

Chemical Physics · Physics 2021-05-05 Alexander A. Milner , Valery Milner

The bulk polarization is a $\mathbb{Z}_2$ topological invariant characterizing non-interacting systems in one dimension with chiral or particle-hole symmetries. We show that the bulk polarization can always be determined from the…

Mesoscale and Nanoscale Physics · Physics 2021-05-26 Carlos Ortega-Taberner , Maria Hermanns

We consider a method for obtaining information on polarization of astronomical objects radiation at diffraction limited resolution - differential speckle polarimetry. As an observable we propose to use averaged cross spectrum of two…

Instrumentation and Methods for Astrophysics · Physics 2015-06-12 Boris Safonov

A method and codes for two-step correlation calculation of heavy-atom molecules have been developed, employing the generalized relativistic effective core potential and relativistic coupled cluster (RCC) methods at the first step, followed…

Chemical Physics · Physics 2009-11-07 A. N. Petrov , N. S. Mosyagin , T. A. Isaev , A. V. Titov , V. F. Ezhov , E. Eliav , U. Kaldor

The yield of strong-field ionization, by a linearly polarized probe pulse, is studied experimentally and theoretically, as a function of the relative orientation between the laser field and the molecule. Experimentally, carbonyl sulfide,…

We study interaction of generic asymmetric molecules with a pair of strong time-delayed short laser pulses with crossed linear polarizations. We show that such an excitation not only provides unidirectional rotation of the most polarizable…

Chemical Physics · Physics 2018-02-28 E. Gershnabel , I. Sh. Averbukh

Coulomb interactions that occur in electronic structure calculations are correlated by allowing basis function components of the interacting densities to polarize, thereby reducing the magnitude of the interaction. Exchange integrals of…

Chemical Physics · Physics 2022-05-16 Jerry L. Whitten

Super-resolution localization microscopy is based on determining the positions of individual fluorescent markers in a sample. The major challenge in reaching an ever higher localization precision lies in the limited number of collected…

Optics · Physics 2020-08-05 Daniel Böning , Franz-Ferdinand Wieser , Vahid Sandoghdar

In this perspective, the various measures of electron correlation used in wavefunction theory, density functional theory and quantum information theory are briefly reviewed. We then focus on a more traditional metric based on dominant…

Chemical Physics · Physics 2023-04-07 Róbert Izsák , Aleksei V Ivanov , Nick S. Blunt , Nicole Holzmann , Frank Neese

A program for molecular calculations with B functions is reported and its performance is analyzed. All the one- and two-center integrals, and the three-center nuclear attraction integrals are computed by direct procedures, using previously…

Chemical Physics · Physics 2016-02-19 E. O. Steinborn , H. H. H. Homeier , I. Ema , R. Lopez , G. Ramirez

We develop a direct derivation for the primary contribution to the vibrational polarizability for molecules, clusters and other finite systems. The vibrational polarizability is then calculated within the generalized gradient approximation…

Other Condensed Matter · Physics 2007-05-23 Mark R. Pederson , Tunna Baruah , Philip B. Allen , Christian Schmidt

We suggest measuring the one-particle density matrix of a trapped ultracold atomic cloud by scattering fast atoms in a pure momentum state off the cloud. The lowest-order probability for the process, resulting in a pair of outcoming fast…

Soft Condensed Matter · Physics 2007-05-23 A. B. Kuklov , B. V. Svistunov

The morphology of spectral line polarization is the most valuable observable to investigate the magnetic and dynamic solar atmosphere. However, in order to develop solar diagnosis, it is fundamental to understand the different kinds of…

Solar and Stellar Astrophysics · Physics 2019-07-03 Edgar S. Carlin

In this work, we present a new computational approach to characterize and classify molecular packing in the solid states. The key idea is to project each neighboring molecule (or short contact) from the centered molecule into a unit sphere…

Materials Science · Physics 2025-06-06 Qiang Zhu , Weilun Tang , Shinnosuke Hattori

The tensor polarization of particles and nuclei becomes constant in the coordinate system rotating with the same angular velocity as the spin and rotates in the lab frame with the above angular velocity. The general equation defining the…

High Energy Physics - Phenomenology · Physics 2015-07-07 Alexander J. Silenko

Chemotactic cells establish cell polarity in the absence of external guidance cues. Such self-organized polarity is induced by spontaneous symmetry breaking in the intracellular activities, which produces an emergent memory effect…

Cell Behavior · Quantitative Biology 2015-06-16 Tetsuya Hiraiwa , Akihiro Nagamatsu , Naohiro Akuzawa , Masatoshi Nishikawa , Tatsuo Shibata

Control of molecular rotations by laser fields is an active area of research focusing on the alignment/orientation of otherwise isotropic molecular samples. Oriented molecules are useful in many applications, such as molecular orbital…

Chemical Physics · Physics 2020-07-03 Long Xu , Ilia Tutunnikov , Erez Gershnabel , Yehiam Prior , Ilya Sh. Averbukh

We demonstrate theoretically and experimentally that the three-dimensional orientation of a single fluorescent nano-emitter can be determined by polarization analysis of the emitted light (while excitation polarization analysis provides…

The simultaneous treatment of static and dynamical correlations in strongly-correlated electron systems is a critical challenge. In particular, finding a universal scheme for identifying a single-particle orbital basis that minimizes the…

Quantum Physics · Physics 2024-08-07 Ke Liao , Lexin Ding , Christian Schilling

For $\pi^0\eta$-photoproduction on the nucleon formal expressions are developed for the five-fold differential cross section and the recoil polarization including beam and target polarizations. The polarization observables are described by…

Nuclear Theory · Physics 2011-02-28 A. Fix , H. Arenhövel
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