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We demonstrate the ability to coherently control ultracold atomic Rb collisions using frequency-chirped light on the nanosecond time scale. For certain center frequencies of the chirp, the rate of inelastic trap-loss collisions induced by…

Atomic Physics · Physics 2009-11-13 M. J. Wright , J. A. Pechkis , J. L. Carini , S. Kallush , R. Kosloff , P. L. Gould

We describe experiments and associated quantum simulations involving the production of ultracold $^{87}$Rb$_{2}$ molecules with nanosecond pulses of frequency-chirped light. With appropriate chirp parameters, the formation is dominated by…

Atomic Physics · Physics 2016-06-07 J. L. Carini , S. Kallush , R. Kosloff , P. L. Gould

We present results on coherent control of ultracold trap-loss collisions using 40 ns pulses of nonlinearly frequency-chirped light. The chirps, either positive or negative, sweep ~1 GHz in 100 ns and are centered at various detunings below…

Atomic Physics · Physics 2015-05-28 J. A. Pechkis , J. L. Carini , C. E. Rogers , P. L. Gould , S. Kallush , R. Kosloff

We have studied the effects of chirped femtosecond laser pulses on the formation of ultracold molecules in a Rb magneto-optical trap. We have found that application of chirped femtosecond pulses suppressed the formation of 85Rb-2 and 87Rb-2…

Atomic Physics · Physics 2009-11-11 Benjamin L. Brown , Alexander J. Dicks , Ian A. Walmsley

We show how to emulate a conventional pump-probe scheme using a single frequency-chirped ultrashort UV pulse to obtain a time-resolved image of molecular ultrafast dynamics. The chirp introduces a spectral phase in time that encodes the…

Chemical Physics · Physics 2017-05-03 Denis Jelovina , Johannes Feist , Fernando Martín , Alicia Palacios

We demonstrate that judicious shaping of a nanosecond-time-scale frequency chirp can dramatically enhance the formation rate of ultracold $^{87}$Rb$_{2}$ molecules. Starting with ultracold $^{87}$Rb atoms, we apply pulses of…

Atomic Physics · Physics 2016-02-26 J. L. Carini , S. Kallush , R. Kosloff , P. L. Gould

We use frequency-chirped light on the nanosecond time scale to produce ultracold $^{87}$Rb$_{2}$ molecules in the lowest triplet state via the process of photoassociation. Comparing to quantum simulations of the molecular formation, we…

Atomic Physics · Physics 2015-06-11 J. L. Carini , J. A. Pechkis , C. E. Rogers , P. L. Gould , S. Kallush , R. Kosloff

Scattering resonances due to the dipole-dipole interaction between ultracold molecules, induced by static or microwave fields, are studied theoretically. We develop a method for coupled-channel calculations that can efficiently impose many…

Quantum Gases · Physics 2023-07-11 Tijs Karman

Photoassociation of ultracold atoms induced by chirped picosecond pulses is analyzed in a non-perturbative treatment by following the wavepackets dynamics on the ground and excited surfaces. The initial state is described by a Boltzmann…

Atomic and Molecular Clusters · Physics 2009-06-10 Eliane Luc-Koenig , Mihaela Vatasescu , Francoise Masnou-Seeuws

Ultrafast electronic dynamics are typically studied using pulsed lasers. We demonstrate a complementary experimental approach: quantum simulation of ultrafast dynamics using trapped ultracold atoms. Counter-intuitively, this technique…

Two atoms in an ultracold gas are correlated at short inter-atomic distances due to threshold effects where the potential energy of their interaction dominates the kinetic energy. The correlations manifest themselves in a distinct nodal…

Atomic Physics · Physics 2011-04-15 Christiane P. Koch , Ronnie Kosloff

Photoassociation of ultracold atoms is shown to lead to alignment of the product molecules along the excitation laser polarization axis. We theoretically investigate pulsed photoassociation of $^{87}Rb$ atoms into a specific weakly-bound…

Quantum Physics · Physics 2017-11-15 S. Kallush , J. L. Carini , P. L. Gould , R. Kosloff

Using numerical simulations, we study propagation of linearly-chirped optical pulses in a homogeneously broadened two-level medium. We pay attention to the three main topics -- validity of the rotating-wave approximation (RWA), pulse…

Optics · Physics 2015-10-13 Denis Novitsky

We study the effect of the chirped laser pulse on the transmission and associated ion acceleration by the sub-wavelength target. In the chirped laser pulses, the pulse frequency has a temporal variation about its fundamental frequency,…

Plasma Physics · Physics 2018-11-06 Shivani Choudhary , Amol R. Holkundkar

The softness of elastic atomic collisions, defined as the average number of collisions each atom undergoes until its energy decorrelates significantly, can have a considerable effect on the decay dynamics of atomic coherence. In this paper…

Atomic Physics · Physics 2017-09-27 Jonathan Coslovsky , Gadi Afek , Alexander Mil , Ido Almog , Nir Davidson

We consider losses in collisions of ultracold molecules described by a simple statistical short-range model that explicitly accounts for the limited lifetime of classically chaotic collision complexes. This confirms that thermally sampling…

Atomic Physics · Physics 2021-11-05 Arthur Christianen , Gerrit C. Groenenboom , Tijs Karman

We employ a continuous dynamical decoupling scheme to suppress the decoherence induced by elastic collisions of cold atoms. Using a continuous echo pulse we achieve a thirty-fold increase in the coherence time of Rb87 atoms trapped in a…

Quantum Physics · Physics 2009-05-28 Yoav Sagi , Ido Almog , Nir Davidson

We study the effects of arbitrary laser pulse excitations on quantum correlation, entanglement and the role of quantum noise. The transient quantities are computed exactly using a method that provides exact solutions of the Langevin field…

Quantum Physics · Physics 2009-11-13 C. H. Raymond Ooi

At ultracold temperatures, the Pauli exclusion principle suppresses collisions between identical fermions. This has motivated the development of atomic clocks using fermionic isotopes. However, by probing an optical clock transition with…

Utilizing single-photon photoassociation, we have achieved ultracold rubidium molecules with a high number density that provides a new efficient approach toward molecular quantum degeneracy. A new detection mechanism for ultracold molecule…

Atomic Physics · Physics 2015-06-12 Jun-Ren Chen , Cheng-Yang Kao , Hung-Bin Chen , Yi-Wei Liu
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