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Canonical semiclassical methods can be used to develop an intuitive definition of tunneling time through potential barriers. An application to atomic ionization is given here, considering both static and time-dependent electric fields. The…

Quantum Physics · Physics 2019-01-23 Bekir Baytas , Martin Bojowald , Sean Crowe

Attosecond science has opened up new frontiers in our understanding of processes happening on the intrinsic timescale of electrons. The ability to manipulate and observe phenomena at the attosecond level has yielded groundbreaking insights…

Quantum Physics · Physics 2024-11-08 Lidice Cruz-Rodriguez , Diptesh Dey , Antonia Freibert , Philipp Stammer

The full-dimensional time-dependent Schrodinger equation for the electronic dynamics of single-electron systems in intense external fields is solved directly using a discrete method. Our approach combines the finite-difference and Lagrange…

Atomic Physics · Physics 2009-11-10 Liang-You Peng , J F McCann , Daniel Dundas , K T Taylor , I D Williams

A new quantum dynamical model has been developed to describe the dissociative ionization of deuterium molecular ions by intense laser pulses ($\tau=10$ fs, $\lambda=200$ nm and $I=3\times10^{13}$ W/cm$^{2}$). We calculated the ionization…

Atomic and Molecular Clusters · Physics 2017-02-08 Attila Tóth , Sándor Borbély , Zsolt G. Kiss , Gábor J. Halász , Ágnes Vibók

The interaction of a short, few-cycle light pulse and an atom which is prepared initially in a superposition of two stationary states is shown to exhibit strong signatures of atomic coherence. For a given waveform of the laser pulse,…

Atomic Physics · Physics 2017-01-04 Viktor Ayadi , Mihaly G. Benedict , Peter Dombi , Peter Foldi

Short-time filtering of the photoionization amplitude extracted straight from the numerical solution of the time-dependent Schr\"{o}dinger equation (TDSE) is used to identify dominant pathways that form photoelectron spectra in strong…

Atomic Physics · Physics 2020-10-21 V. A. Tulsky , D. Bauer

We analyze the photoelectron angular distribution in two-pathway interference between non\-resonant one-photon and resonant two-photon ionization of neon. We consider a bichromatic femtosecond XUV pulse whose fundamental frequency is tuned…

The electron motion in atoms and molecules is at the heart of all phenomena in nature that occur outside the nucleus. Recently, ultrafast electron and X-ray imaging tools have been developed to image the ultrafast dynamics of matter in real…

Precision study of few-electron, high-$Z$ ions is a privileged field for probing high-field, bound-state quantum electrodynamics (BSQED). However, the accuracy of such tests is plagued by nuclear uncertainties, which are often larger than…

Atomic Physics · Physics 2021-05-05 Nancy Paul , Guojie Bian , Toshiyuki Azuma , Shinji Okada , Paul Indelicato

We propose a new technique to fully characterize the temporal structure of extreme ultraviolet pulses by ionizing a bound coherent electronic wavepacket. The populated energy levels make it possible to interfere different spectral…

Optics · Physics 2016-07-19 Stefan Pabst , Jan Marcus Dahlström

Attosecond science is well developed for atoms and promising results have been obtained for molecules and solids. Here, we review the first steps in developing attosecond time-resolved measurements in liquids. These advances provide access…

Other Condensed Matter · Physics 2020-09-11 H. J. Wörner , A. Schild , D. Jelovina , I. Jordan , C. Perry , T. T. Luu , Z. Yin

An alternative method to the density matrix formalism for the derivation of general expressions of the interaction of polarized atoms with polarized photons and electrons is presented. The expression for the cross-section describing the…

Quantum Physics · Physics 2015-06-26 A. Kupliauskiene

Reconstruction of Attosecond Beating By Interference of Two-photon Transitions (RABBITT) is a technique that can be used to determine the phases of atomic transition elements in photoionization processes. In the traditional RABBITT scheme,…

The purpose of this document is to describe the solution and implementation of the time-independent and time-dependent Schr\"odinger using pseudospectral methods. Currently, the description is for single particle systems interacting with a…

Quantum Physics · Physics 2024-04-08 Håkon Kristiansen , Einar Aurbakken

Focused laser fields with textured polarization on a sub-wavelength scale allow extracting information on electronic processes which are not directly accessible by homogeneous fields. Here, we consider photoionization in radially and…

Atomic Physics · Physics 2021-06-30 Jonas Wätzel , Jamal Berakdar

Quantum control and measurement are two sides of the same coin. To affect a dynamical map, well-designed time-dependent control fields must be applied to the system of interest. To read out the quantum state, information about the system…

Quantum Physics · Physics 2015-05-14 Ivan H. Deutsch , Poul S. Jessen

Quantum tunnelling of electrons can be confined to the sub-cycle time scale of strong light fields, contributing decisively to the extreme time resolution of attosecond science. Because tunnelling also enables atomic-scale spatial…

We investigate the angular distribution of electrons that are emitted in the ionization of hydrogen-like ions by twisted photons. Analysis is performed based on the first-order perturbation theory and the non-relativistic Schr\"odinger…

We study experimentally the influence of the intensity of the infrared (IR) probe field on attosecond pulse train (APT) phase measurements performed with the RABITT method (Reconstruction of Attosecond Beating by Interference in Two-Photon…

Atomic Physics · Physics 2009-07-22 M. Swoboda , J. M. Dahlstrom , T. Ruchon , P. Johnsson , J. Mauritsson , K. J. Schafer , A. L'Huillier

We propose a protocol to probe the ultrafast evolution and dephasing of coherent electronic excitation in molecules in the time domain by the intrinsic streaking field generated by the molecule itself. Coherent electronic motion in the…