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Molecular spin systems based on photoexcited triplet pairs formed via singlet fission (SF) are attractive as carriers of quantum information because of their potentially pure and controllable spin polarization, but developing systems that…

Mesoscale and Nanoscale Physics · Physics 2022-11-09 Gajadhar Joshi , Ryan D. Dill , Karl J. Thorley , John E. Anthony , Obadiah G. Reid , Justin C. Johnson

A numerical modeling of the radiation emitted from a Luminescent dye embedded in a finite one-dimensional photonic crystal is presented. The Photonic Band Structure and the Photonic Density of States are derived using classical…

Optics · Physics 2010-12-30 J. Manzanares-Martinez , P. Castro-Garay

The blue emission of polyfluorene (PF) based light-emitting diodes (LEDs) is known to degrade due to a low energy green emission, which hitherto has been attributed to oxidative defects. By studying the electroluminescence from ethyl-hexyl…

Soft Condensed Matter · Physics 2015-05-13 M. Arif , S. Mukhopadhyay , S. Ramasesha , S. Guha

Effects associated with the change in the local density of photonic states in a periodic structure based on alternating \textit{a}-Si$_{1-x}$C$_x$:H and \textit{a}-SiO$_2$ amorphous layers forming a one-dimensional (1D) photonic crystal…

Mesoscale and Nanoscale Physics · Physics 2017-07-21 Mikhail V. Rybin , Alexander V. Zherzdev , Nikolay A. Feoktistov , Alexander B. Pevtsov

We study numerically the slow (subradiant) decay of the fluorescence of motionless atoms after a weak pulsed excitation. We show that, in the linear-optics regime and for an excitation detuned by several natural linewidths, the slow decay…

Quantum Physics · Physics 2021-08-10 Y. A. Fofanov , I. M. Sokolov , R. Kaiser , W. Guerin

Polarization mode dispersion (PMD) in optical fibers poses a major challenge for maintaining the fidelity of quantum states for quantum communications. In this work, a comprehensive model linking the probability of quantum measurement…

We experimentally show that the rate of singlet fission in tetracene films has a superlinear dependence on the density of photo-excited singlet excitons with ultrafast transient absorption spectroscopy. The spectrotemporal features of…

Materials Science · Physics 2014-10-01 Bo Zhang , Chunfeng Zhang , Rui Wang , Zhanao Tan , Yunlong Liu , Wei Guo , Xiaoling Zhai , Xiaoyong Wang , Min Xiao

Cesium lead halide nanocrystals and quantum dots are prominent materials for different types of applications because of their remarkable photophysical properties. However, they are also known to exhibit the same effects observed for…

The aim of this paper is to present the analysis of influence of defects in 1D photonic crystal (PC) on the density of states and simultaneously spontaneous emission, in both spatial and frequency domains. In our investigations we use an…

Optics · Physics 2009-12-22 A. Rudziński , A. Tyszka-Zawadzka , P. Szczepański

Fluorescence lifetimes of nitrogen-vacancy color centers in individual diamond nanocrystals were measured at the interface between a glass substrate and a strongly scattering medium. Comparison of the results with values recorded from the…

Quantum Physics · Physics 2015-05-18 P. V. Ruijgrok , R. Wüest , A. A. Rebane , A. Renn , V. Sandoghdar

Investigations that probe defects one at a time offer a unique opportunity to observe properties and dynamics that are washed out of ensemble measurements. Here we present confocal fluorescence measurements of individual defects in Al-doped…

Materials Science · Physics 2015-06-18 N. R. Jungwirth , Y. Y. Pai , H. S. Chang , E. R. MacQuarrie , G. D. Fuchs

Variation in fluorescence intensity from rhodamine 6G dye was investigated. A small volume of dye solution was optically excited with a 0.4 mW, 532nm wavelength cw-laser light. The dye was dissolved in methanol and glycerol for a…

Optics · Physics 2023-10-16 S. M. Iftiquar , H. Zilay

A photonic molecule (PM) is a miniature diffractive optical structure composed of resonance microcavities called atoms (e.g., cylinders or spheres) supporting a set of high-quality eigenmodes. All atoms in a PM are coupled by the…

Optics · Physics 2022-11-29 Yury E. Geints

Colloidal semiconductor quantum dots (QDs) are excellent luminescent nanomaterials for a broad range of optoelectronic applications. Their photoluminescence blinking, however, hinders their practical use in many aspects. It has been shown…

Optics · Physics 2024-02-27 Zhiyuan Wang , Jianwei Tang , Jiahao Han , Juan Xia , Tianzi Ma , Xue-Wen Chen

We introduce the concept of optical control of the fluorescence yield of CdSe quantum dots through plasmon-induced structural changes in random semicontinuous nanostructured gold films. We demonstrate that the wavelength- and polarization…

Photo-luminescence intermittency (blinking) in semiconductor nanocrystals (NCs), a phenomenon ubiquitous to single-emitters, is generally considered to be temporally random intensity fluctuations between bright (On) and dark (Off) states.…

Mesoscale and Nanoscale Physics · Physics 2020-01-29 Amitrajit Mukherjee , Korak Kumar Ray , Chinmay Phadnis , Arunasish Layek , Soumya Bera , Arindam Chowdhury

Triplet excited states in organic semiconductor materials and devices are notoriously difficult to detect and study with established spectroscopic methods. Yet, they are a crucial intermediate step in next-generation organic light emitting…

Applied Physics · Physics 2021-11-24 Jeannine Grüne , Vladimir Dyakonov , Andreas Sperlich

Coherence phenomena in four-level atomic system, cyclicly driven by three coherent fields, are investigated thoroughly at zero and weak magnetic fields. Each strongly interacting atomic state is converted to a triplet due to a dynamical…

Optics · Physics 2016-09-20 F. Ghafoor , R. G. Nazmitdinov

Tin-phthalocyanine molecules adsorbed on a NaCl ultrathin film on Au(111) exhibit electrofluorescence excited by a current across a scanning tunneling microscope junction. Exploring the dependence of the molecular monomer photon yield on…

Mesoscale and Nanoscale Physics · Physics 2026-03-03 Maximilian Kögler , Nicolas Néel , Jörg Kröger

Single cesium lead bromide (CsPbBr3) nanocrystals show strong photoluminescence blinking, with on- and off- dwelling times following power-law distributions. We investigate the memory effect in the photoluminescence blinking of single…