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The local interaction of charges and light in organic solids is the basis of distinct and fundamental effects. We here observe, at the single molecule scale, how a focused laser beam can locally shift by hundreds-time their natural…

Accurate molecular imaging via high-order harmonic generation relies on comparing the harmonic emission from a molecule and an adequate reference system. However, an ideal reference atom with the same ionization properties as the molecule…

Atomic Physics · Physics 2015-05-28 Elmar V. van der Zwan , Manfred Lein

Non-sequential double recombination (NSDR) high-order harmonic generation (HHG) is studied in a molecular system. We observe a unique molecular two-electron effect with a characteristic cutoff in the HHG spectrum at higher energies than…

Atomic Physics · Physics 2016-06-08 Kenneth K. Hansen , Lars Bojer Madsen

In order to elucidate the correlated motion of atomic electrons, we investigate the attosecond-scale dynamics of their entanglement arising due to nonsequential ionization driven by a strong, linearly-polarized laser field. The calculation…

Atomic Physics · Physics 2024-03-18 Daniel Younis , Songbo Xie , Joseph H. Eberly

With a semiclassical quasi-static model we achieve an insight into the complex dynamics of two correlated electrons under the combined influence of a two-center Coulomb potential and an intense laser field. The model calculation is able to…

Atomic and Molecular Clusters · Physics 2009-11-13 J. Liu , D. F. Ye , J. Chen , X. liu

We investigate the high harmonic generation (HHG) in solids driven by laser fields with different ellipticities. The HHG spectra show a two-plateau structure within the energy gap between the valence band and the first conduction band.…

Optics · Physics 2018-06-01 Liang Li , Pengfei Lan , Xiaosong Zhu , Tengfei Huang , Peixiang Lu

We develop a green light source with low spatial coherence via intracavity frequency doubling of a solid-state degenerate laser. The second harmonic emission supports many more transverse modes than the fundamental emission, and exhibit…

We investigate the effect of phase modulation of laser beams on the coherent and incoherent non-linear signals arising from the interaction of femtosecond pulses with matter. We observe that two collinear beams, whose phases are modulated…

Optics · Physics 2015-05-29 Khadga Jung Karki , Loni Kringle , Andrew H. Marcus , Tõnu Pullerits

We examine correlated electron and doubly charged ion momentum spectra from strong field double ionization of Neon employing intense elliptically polarized laser pulses. An ellipticity-dependent asymmetry of correlated electron and ion…

We show that spatially structured radiation generates second harmonic in a two-dimensional system even if the system is homogeneous and isotropic. The effect originates from non-locality of electric response to structured electromagnetic…

Mesoscale and Nanoscale Physics · Physics 2025-04-23 A. A. Gunyaga , M. V. Durnev , S. A. Tarasenko

We investigate high-order harmonic generation in inhomogeneous media for reduced dimensionality models. We perform a phase-space analysis, in which we identify specific features caused by the field inhomogeneity. We compute high-order…

Atomic Physics · Physics 2016-05-25 C. Zagoya , M. Bonner , H. Chomet , E. Slade , C. Figueira de Morisson Faria

We extend the semiclassical two-step model for strong-field ionization that describes quantum interference and accounts for the Coulomb potential beyond the semiclassical perturbation theory to the hydrogen molecule. In the simplest case of…

Atomic Physics · Physics 2019-03-27 N. I. Shvetsov-Shilovski , M. Lein , K. Tőkési

We perform a systematic analysis of intra-channel quantum interference in laser-induced nonsequential double ionization with linearly polarized bichromatic fields, focusing on the recollision-excitation with subsequent ionization (RESI)…

Atomic Physics · Physics 2025-08-06 S. Hashim , D. Habibović , C. Figueira de Morisson Faria

High-order harmonic generation from atomic systems is considered in the crossed fields of a relativistically strong infrared laser and a weak attosecond-pulse train of soft x-rays. Due to one-photon ionization by the x-ray pulse, the…

Atomic Physics · Physics 2009-11-13 Michael Klaiber , Karen Z. Hatsagortsyan , Carsten Müller , Christoph H. Keitel

We demonstrate a two-dimensional time-domain spectroscopy method to extract amplitude and phase modifications of excited atomic states caused by the interaction with ultrashort laser pulses. The technique is based on Fourier analysis of the…

Atomic Physics · Physics 2015-06-19 Alexander Blättermann , Christian Ott , Andreas Kaldun , Thomas Ding , Thomas Pfeifer

We analize the dipole spectrum of a two-level atom excited by a non-resonant intense monochromatic field, under the electric dipole approximation and beyond the rotating wave approximation. We show that the apparently complex spectral…

Optics · Physics 2010-03-25 A. Picón , L. Roso , J. Mompart , O. Varela , V. Ahufinger , R. Corbalán , L. Plaja

High-order harmonic generation (HHG) with relativistically strong laser pulses is considered employing electron ionization-recollisions from multiply charged ions in counterpropagating, linearly polarized attosecond pulse trains. The…

Atomic Physics · Physics 2015-05-19 Markus C. Kohler , Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel

Using a master-equation approach for the description of coherent and incoherent dynamics in `artificial atoms and molecules', we present a theoretical analysis of situations where intense laser fields lead to pronounced renormalizations of…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Ulrich Hohenester , Filippo Troiani , Elisa Molinari

Here we experimentally map the dynamics of electron plasma waves in laser solid interaction. We do time resolved measurements of second harmonic and hard X-ray generation from interaction of intense ($10^{16} W cm^{-2}$, 100 fs, 800nm)…

Plasma Physics · Physics 2007-05-23 Arvinder S. Sandhu , G. Ravindra Kumar , S. Sengupta , A. Das , P. K. Kaw

In our earlier work on harmonic generation with complex light [Nature Communications 15, 6878 (2024)], we demonstrated how the harmonic spectrum of a complex laser beam in a nonlinear medium can be obtained through the judicious application…

Optics · Physics 2025-11-17 Raoul Trines , Holger Schmitz , Martin King , Paul McKenna , Robert Bingham
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