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Related papers: Photoionization and vacancy decay of endohedral at…

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It is demonstrated that the fullerene shell affects dramatically the radiative and Auger vacancy decay of an endohedral atom A@C60. The collectivized electrons of the C60 shell add new possibilities for radiative and non-radiative decays…

Atomic Physics · Physics 2022-06-13 M. Ya. Amusia , A. S. Baltenkov

In this Letter, we investigate the time delay of photoelectrons by fullerenes shell in endohedrals. We present general formulas in the frame of the random phase approximation with exchange (RPAE) applied to endohedrals A@CN that consist of…

Atomic and Molecular Clusters · Physics 2020-10-28 M. Ya. Amusia , L. V. Chernysheva

We discuss the influence of a single or double fullerenes shell upon photoionization and vacancy decay of an atom, stuffed inside the fullerenes construction. The main manifestations of this influence are additional structures in the…

Atomic Physics · Physics 2009-06-23 M. Ya. Amusia

We study the interconnection between the results of two qualitatively different approximate calculations of photoionization cross sections, $\sigma_{n\ell}$, for neutral atoms ($A$) or their cations ($A^+$), centrally confined inside a…

Atomic Physics · Physics 2024-09-19 V. K. Dolmatov , L. V. Chernysheva , V. G. Yarzhemsky

We have calculated photoionization cross-section of endohedral atoms A@CN. We took into account the polarizability of the fullerene electron shell CN that modifies the incoming photon beam and the one-electron wave functions of the caged…

Atomic and Molecular Clusters · Physics 2019-03-27 M. Ya. Amusia , L. V. Chernysheva

We concentrate here on photon absorption as well as electron and positron scattering upon endohedrals that consist of a fullerenes shell and an inner atom A. The aim is to understand the effect of fullerene electron shell in formation of…

Atomic and Molecular Clusters · Physics 2018-02-12 M. Ya. Amusia , A. F. Ioffe

We demonstrate rather interesting manifestations of co-existence of resonance features in characteristics of the photoionization of 3d-electrons in Xe, Cs and Ba endohedral atoms. It is shown that for all of the considered atoms the…

Atomic Physics · Physics 2009-11-13 M. Ya. Amusia , A. S. Baltenkov , L. V. Chernysheva

We demonstrate for the first time that the effect of fullerene shell upon photoionization of the "caged" atom in an endohedral can result in formation of Giant Endohedral Resonances or GER. This is illustrated by the concrete case of Xe@C60…

Chemical Physics · Physics 2009-11-13 M. Ya. Amusia , A. S. Baltenkov , L. V. Chernysheva

Our previous studies [J. Phys. B 53, 125101 (2020); Euro. Phys. J. D 74, 191 (2020)] have predicted that the atom-fullerene hybrid photoionization properties for X = Cl, Br and I endohedrally confined in C60 are different before and after…

Atomic and Molecular Clusters · Physics 2022-03-14 Esam Ali , Taylor O'Brien , Andrew Dennis , Mohamed El-Amine Madjet , Steven T. Manson , Himadri S. Chakraborty

We discuss the complicated resonance structure of the endohedral atom photoionization cross section. Very strong enhancement and interference patterns in the photoionization cross-section of the valent and subvalent subshells of noble gas…

Atomic Physics · Physics 2008-06-03 M. Ya. Amusia , L. V. Chernysheva

It is demonstrated that in photoabsorption by endohedral atoms some atomic Giant resonances are almost completely destroyed while the others are totally preserved due to different action on it of the fullerenes shell. As the first example…

Atomic and Molecular Clusters · Physics 2007-12-20 M. Ya. Amusia , A. S. Baltenkov , L. V. Chernysheva

The photoionization of a two-shell endohedral A@CN1@CN2 is considered. Formulas are presented for cross-sections and angular anisotropy parameters, both dipole and non-dipole. The effect of the fullerenes shell upon photoelectron from atom…

Atomic and Molecular Clusters · Physics 2013-05-29 M. Ya. Amusia , L. V. Chernysheva , E. Z. Liverts

We demonstrate that the Auger decay rate in an endohedral atom is very sensitive to the atom's location in the fullerene cage. Two additional decay channels appear in an endohedral system: (a) the channel due to the change in the electric…

Atomic and Molecular Clusters · Physics 2015-05-20 Andrey V. Korol , Andrey V. Solov'yov

Photoionization cross sections, photoelectron angular-asymmetry parameters and photoionization time delays for $A$@C$_{60}$ endohedral atoms are studied with account for both the individual and combined effects of dipole static polarization…

Atomic Physics · Physics 2018-09-11 V. K. Dolmatov

It is demonstrated by the example of the Xe atom stuffed inside the C60 fullerene, that the so-called confinement resonances in 4d subshell strongly affect the photoionization cross-section of outer 5p and subvalent 5s electrons near 4d…

Atomic Physics · Physics 2015-06-03 M. Ya. Amusia , L. V. Chernysheva

Photoionization calculations of the endofullerene molecule Cl@$C_{60}$ with an open-shell chlorine atom are performed in the time-dependent local density approximation (TDLDA) based on a spherical jellium model. Cross sections for…

Atomic and Molecular Clusters · Physics 2021-06-08 Dakota Shields , Ruma De , Mohamed El-Amine Madjet , Steven T. Manson , Himadri S. Chakraborty

Photoionization from atom-C60 hybrid levels in halogen endufullerene molecules, Cl@C60, Br@C60 and I@C60, are calculated using a linear response density functional method. Both the ordinary electron-configuration where the open shell…

Atomic and Molecular Clusters · Physics 2021-06-08 Dakota Shields , Ruma De , Esam Ali , Mohamed E Madjet , Steven T Manson , Himadri S. Chakraborty

In this Letter, we investigate the variation of endohedral A@CN potential due to addition at the center of it a positive charge, for example, in the process of atom A photoionization. Using a reasonable model to describe the fullerenes…

Atomic and Molecular Clusters · Physics 2019-10-29 M. Ya. Amusia , A. S. Baltenkov , L. V. Chernysheva

Using $He@C_{60}$ as an example, we demonstrate that static potential of the fullerene core essentially alters the cross section of the two-electron ionization differential in one-electron energy $d\sigma ^{++}(\omega )/d\epsilon $. We…

Atomic Physics · Physics 2009-11-11 M. Ya. Amusia , E. Z. Liverts , V. B. Mandelzweig

We demonstrate the prominent modification of the outer shell photoionization cross-section in noble gas (NG) endohedral atoms NG@F under the action of the fullerene F electron shell. This shell leads to two important effects, namely to…

Atomic and Molecular Clusters · Physics 2009-11-13 M. Ya. Amusia , A. S. Baltenkov , L. V. Chernysheva
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