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We present analytical formulas for the calculation of the two-center two-electron integrals in the basis of Slater geminals and products of Slater orbitals. Our derivation starts with establishing a inhomogeneous fourth-order ordinary…

Quantum Physics · Physics 2012-12-07 Michał Lesiuk , Robert Moszynski

In this paper, which constitutes the first part of the series, we consider calculation of two-centre Coulomb and hybrid integrals over Slater-type orbitals (STOs). General formulae for these integrals are derived with no restrictions on the…

Quantum Physics · Physics 2015-01-09 Michał Lesiuk , Robert Moszynski

In previous work, the necessary integrals arising from correlated wavefunctions were expressed in forms suitable for numerical integration. For the evaluation of $r_{12}$ and $1/r_{12}$ integrals an analytic formula is derived.…

Mathematical Physics · Physics 2012-07-26 E. V. Rothstein

In this study, using the analytical and recurrence relations suggested by the authors in previous works, the new efficient and reliable program procedure for the overlap integrals over Slater type orbitals (STOs) is presented. The proposed…

Chemical Physics · Physics 2015-05-13 I. I. Guseinov , B. A. Mamedov

Recently published formulas for the surface and regular solid spherical harmonics and for the expansion of the product of two normalized associated Legendre functions with different centers in ellipsoidal coordinates (Telhat Ozdogan, Metin…

Chemical Physics · Physics 2007-05-23 I. I. Guseinov

The purpose of this paper is to extend the explicit geometric evaluation of semisimple orbital integrals for smooth kernels for the Casimir operator obtained by the first author to the case of kernels for arbitrary elements in the center of…

Differential Geometry · Mathematics 2022-08-12 Jean-Michel Bismut , Shu Shen

A simple method is outlined for analytic evaluation of the basic 2-electron atomic integral with integrand containing products of atomic s-type Slater orbitals and exponentially correlated function of the form $r_{ij}…

Atomic Physics · Physics 2016-09-02 Bholanath Padhy

The auxiliary functions provide efficient computation of integrals arising at the self-consistent field (SCF) level for molecules using Slater-type bases. This applies both in relativistic and non-relativistic electronic structure theory.…

Chemical Physics · Physics 2017-11-29 A. Bagci , P. E. Hoggan

We derive direct single-stage numerical evaluation of the electronic overlap integral between arbitrary atomic orbitals (including STOs). Integration is over cartesian co-ordinates, and replaces previous sums over 'special' functions. The…

Chemical Physics · Physics 2016-04-21 Michael J Caola

The simple method outlined in our earlier paper [B.Padhy, Orissa Journal of Physics, vol.19, No.1, p.1, February 2012] has been utilized here for analytic evaluation of three different five-electron atomic integrals with integrands…

Atomic Physics · Physics 2016-09-03 Bholanath Padhy

Multicentric integrals that involve a continuum state cannot be evaluated with the usual quantum chemistry tools and require a special treatment. We consider an initial molecular bound state described by multicenter spherical or cartesian…

Quantum Physics · Physics 2021-11-17 Abdallah Ammar , Arnaud Leclerc , Lorenzo Ugo Ancarani

We present a general methodology to evaluate matrix elements of the effective core potentials (ECPs) within one-electron basis set of Slater-type orbitals (STOs). The scheme is based on translation of individual STO distributions in the…

Chemical Physics · Physics 2017-05-17 Michal Lesiuk , Aleksandra M. Tucholska , Robert Moszynski

In this paper methods for calculations of multi-center integrals of squared Coulomb potentials and Slater-type orbitals (STO) are derived. These integrals are necessary for accurate lower bounds to energy levels of molecular systems. All…

Chemical Physics · Physics 2022-02-10 Sohei Ashida

Single-center two-electron integration is an important core technology in ab initio calculation of atomic and molecular structures. Therefore, this paper reviews and optimizes the method of Zhao et al., and draws a conclusion: Because this…

Quantum Physics · Physics 2023-06-27 Lian-Peng Zhao

An improved algorithm to evaluate the nonrelativistic three-electron Hylleraas-Configuration Interaction (Hy-CI) kinetic energy integrals over Slater orbitals and the Hamiltonian in Hylleraas coordinates is shown. The resulting analytical…

Atomic Physics · Physics 2016-01-29 Maria Belen Ruiz

Starting from one-range addition theorems for Slater-type functions, which are expansion in terms of complete and orthonormal functions based on the generalized Laguerre polynomials, Guseinov constructed addition theorems that are…

Mathematical Physics · Physics 2011-07-26 Ernst Joachim Weniger

In this study, the one-center expansion formulas in terms of complete orthonormal sets of -exponential type orbitals (-ETOs,) are established for the Slater type orbitals (STOs) and Coulomb-Yukawa like correlated interaction potentials…

Chemical Physics · Physics 2013-02-12 I. I. Guseinov

Matrix elements between nonorthogonal Slater determinants represent an essential component of many emerging electronic structure methods. However, evaluating nonorthogonal matrix elements is conceptually and computationally harder then…

Chemical Physics · Physics 2024-06-19 Hugh G. A. Burton

By the use of complete orthonormal sets of nonrelativistic scalar orbitals introduced by the author in previous papers the new complete orthonormal basis sets for two- and four-component spinor wave functions, and Slater spinor orbitals…

Chemical Physics · Physics 2008-12-16 I. I. Guseinov

We present a computer code that analytically evaluates the matrix elements of the microscopic nuclear Hamiltonian and unity operator between Slater determinants of displaced gaussian single particle orbits. Such matrix elements appear in…

Nuclear Theory · Physics 2009-10-22 K. Varga