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An approach to electron correlation effects in atoms that uses quantum trajectories is presented. A comparison with the exact quantum mechanical results for 1D Helium atom shows that the major features of the correlated ground state…

Atomic Physics · Physics 2025-02-07 Ivan P. Christov

High-harmonic generation (HHG) from liquids offers a potential pathway to attosecond spectroscopy in chemically complex and disordered environments, yet fundamental questions remain open: whether liquid harmonic emission preserves…

Quasi-free field-driven electron trajectories are a key element of strong-field dynamics. Upon recollision with the parent ion, the energy transferred from the field to the electron may be released as attosecond duration XUV emission in the…

We investigate the photoionization dynamics of atoms subjected to intense, ultrashort laser pulses through the use of quantum trajectories. This method provides a unique and consistent framework for examining electron dynamics within a…

Atomic Physics · Physics 2024-08-01 Taylor Moon , Klaus Bartschat , Nicolas Douguet

High-harmonic generation (HHG) involves the up-conversion of a high-intensity driving field into its harmonic orders. This process is intrinsically non-classical, requiring from quantum mechanics for a complete explanation as, under…

Quantum Physics · Physics 2024-09-25 Javier Rivera-Dean

Beyond their use as numerical tools, quantum trajectories can be ascribed a degree of reality in terms of quantum measurement theory. In fact, they arise naturally from considering continuous observation of a damped quantum system. A…

Quantum Physics · Physics 2009-11-10 H. M. Wiseman

Quantum trajectory calculations for electrons are a useful tool in the field of molecular dynamics, e.g. to understand processes in ultrafast spectroscopy. They have, however, two limitation: On the one hand, such calculations are typically…

Chemical Physics · Physics 2021-09-29 Axel Schild

Stochastic perturbation of two-level atoms strongly driven by a coherent light field is analyzed by the quantum trajectory method. A new method is developed for calculating the resonance fluorescence spectra from numerical simulations. It…

Quantum Physics · Physics 2009-11-07 A. Karpati , P. Adam , W. Gawlik , B. Lobodzinski , J. Janszky

We report attosecond-scale probing of the laser-induced dynamics in molecules. We apply the method of high-harmonic spectroscopy, where laser-driven recolliding electrons on various trajec- tories record the motion of their parent ion.…

Both the physical picture of the dynamics of atoms and molecules in intense infrared fields and its theoretical description use the concept of electron trajectories. Here we address a key question which arises in this context: Are…

Atomic Physics · Physics 2015-10-28 L. I. Plimak , Misha Yu. Ivanov

The evolution of electron wavepackets determines the course of many physical and chemical phenomena and attosecond spectroscopy aims to measure and control such dynamics in real-time. Here, we investigate radial electron wavepacket motion…

Atomic Physics · Physics 2015-09-04 Niranjan Shivaram , Xiao-Min Tong , Henry Timmers , Arvinder Sandhu

We investigate how short and long electron trajectory contributions to high harmonic emission and their interferences give access to intra-molecular dynamics. In the case of unaligned molecules, we show experimental evidences that the long…

We analyze the attosecond electron dynamics in hydrogen molecular ion driven by an external intense laser field using ab-initio numerical simulations of the corresponding time-dependent Schr{\"{o}}dinger equation and Bohmian trajectories.…

Chemical Physics · Physics 2015-05-20 Norio Takemoto , Andreas Becker

A trajectory in the Schroedinger wave for an electron in an attractive Coulomb potential with the dynamical behavior is proposed and illustrated for a scattering and a bound state. The scattering cross section derived from the trajectories…

Atomic Physics · Physics 2007-05-23 Yoshio Nishiyama

It is shown that all of the basic properties of the hydrogen atom can be consistently described in terms of classical electrodynamics instead of taking the electron to be a particle; we consider an electrically charged classical wave field,…

General Physics · Physics 2017-03-08 Sergey Rashkovskiy

We calculate the transient absorption of an isolated attosecond pulse by helium atoms subject to a delayed infrared (\ir) laser pulse. With the central frequency of the broad attosecond spectrum near the ionization threshold, the absorption…

Atomic Physics · Physics 2015-06-12 Shaohao Chen , Mengxi Wu , Mette B. Gaarde , Kenneth J. Schafer

We develop a non-relativistic quantum field theory of electrons and nuclei based on the Coulomb Hamiltonian. We derive the exact equations of motion and write these equations in the form of Hedin's equations for all species of identical…

Quantum Physics · Physics 2024-12-12 Ville J. Härkönen

The concerted motion of two or more bound electrons governs atomic and molecular non-equilibrium processes and chemical reactions. It is thus a long-standing scientific dream to measure the dynamics of two bound correlated electrons in the…

We scrutinize the behavior of eigenvalues of an electron of Helium atom as it interacts with electric field directed along $z$-axis and exposed to linearly polarized intense laser field radiation. In order to achieve this, we freeze one…

High-harmonic generation (HHG) is a nonlinear process in which a material sample is irradiated by intense laser pulses, causing the emission of high harmonics of the incident light. HHG has historically been explained by theories employing…

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