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Related papers: Enhanced Molecular Orientation Induced by Molecula…

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We show that a 450 fs nonresonant, moderately intense, linearly polarized laser pulse can induce field-free molecular axis alignment of methyliodide molecules dissolved in a helium nanodroplet. Time-resolved measurements reveal rotational…

Chemical Physics · Physics 2015-06-12 Dominik Pentlehner , Jens H. Nielsen , Alkwin Slenczka , Klaus Mølmer , Henrik Stapelfeldt

We have theoretically investigated the molecular orientation by a asymmetric potential created by the superposition of two-color laser fields. The time-dependent Schrodinger equation is solved numerically for different field parameters. We…

Quantum Physics · Physics 2022-12-22 E. A. Koval

We show that a laser pulse designed as an adiabatic ramp followed by a kick allows one to reach a perfect postpulse molecular alignment, free of saturation. The mechanism is based on an optimized distribution of the energy between a weakly…

Quantum Physics · Physics 2009-11-13 S. Guerin , A. Rouzee , E. Hertz

We investigate to which extend a THz laser pulse can be used to produce field-free molecular orientation at high temperature. We consider laser pulses that can be implemented with the state of the art technology and we show that the…

Quantum Physics · Physics 2015-06-05 M. Lapert , D. Sugny

We point out that the non-adiabatic orientation of quantum rotors, produced by ultrashort laser pulses, is remarkably enhanced by introducing dipolar interaction between the rotors. This enhanced orientation of quantum rotors is in contrast…

Quantum Physics · Physics 2009-11-10 Hiroyuki Shima , Tsuneyoshi Nakayama

The impact of nonadiabatic laser-induced molecular alignment on filamentation is numerically studied. Weak and strong field model of impulsive molecular alignment are compared in the context of nonlinear pulse propagation. It is shown that…

Optics · Physics 2014-12-03 N. Berti , P. Béjot , J. -P. Wolf , O. Faucher

In this paper, we studied the optimal alignment and anti-alignment of O2 molecules by femtosecond laser pulse under different input energy. The results show that there is an energy limit in molecular alignment. The optimal molecular…

Optics · Physics 2023-03-16 Yue-Xun Li , Tao Du

We consider solid surface scattering of molecules that were subject to strong non-resonant ultrashort laser pulses just before hitting the surface. The pulses modify the rotational states of the molecules, causing their field free…

Chemical Physics · Physics 2015-06-12 Yuri Khodorkovsky , J. R. Manson , Ilya Sh. Averbukh

Control of molecular rotations by laser fields is an active area of research focusing on the alignment/orientation of otherwise isotropic molecular samples. Oriented molecules are useful in many applications, such as molecular orbital…

Chemical Physics · Physics 2020-07-03 Long Xu , Ilia Tutunnikov , Erez Gershnabel , Yehiam Prior , Ilya Sh. Averbukh

This study shows the unexpected and counter-intuitive possibility of simultaneously orienting a molecule while delocalizing its molecular axis in a plane in field-free conditions. The corresponding quantum states are characterized and…

Quantum Physics · Physics 2022-10-26 D. Sugny

Photoassociation of ultracold atoms is shown to lead to alignment of the product molecules along the excitation laser polarization axis. We theoretically investigate pulsed photoassociation of $^{87}Rb$ atoms into a specific weakly-bound…

Quantum Physics · Physics 2017-11-15 S. Kallush , J. L. Carini , P. L. Gould , R. Kosloff

The transition between two distinct mechanisms for the laser-induced field-free orientation of CO molecules is observed via measurements of orientation revival times and subsequent comparison to theoretical calculations. In the first…

We show that a linear molecule subjected to a short specific elliptically polarized laser field yields postpulse revivals exhibiting alignment alternatively located along the orthogonal axis and the major axis of the ellipse. The effect is…

Quantum Physics · Physics 2007-05-23 D. Daems , S. Guérin , E. Hertz , H. R. Jauslin , B. Lavorel , O. Faucher

We present an analysis of two experimental approaches to controlling the directionality of molecular rotation with ultrashort laser pulses. The two methods are based on the molecular interaction with either a pair of pulses (a "double kick"…

Optics · Physics 2015-06-11 C. Bloomquist , S. Zhdanovich , A. A. Milner , V. Milner

We consider injection and subsequent acceleration of electrons in narrow plasma channels irradiated by linearly and radially polarized ultraintense laser pulses. Using three-dimensional particle-in-cell simulations, we show that radially…

We introduce a new optical tool - a "two-dimensional optical centrifuge", capable of aligning molecules in extreme rotational states. Unlike the conventional centrifuge, which confines the molecules in the plane of their rotation, its…

Chemical Physics · Physics 2016-05-18 A. A. Milner , A. Korobenko , V. Milner

We introduce a new scheme for controlling the sense of molecular rotation. By varying the polarization and the delay between two ultrashort laser pulses, we induce unidirectional molecular rotation, thereby forcing the molecules to rotate…

Quantum Physics · Physics 2015-05-13 Sharly Fleischer , Yuri Khodorkovsky , Yehiam Prior , Ilya Sh. Averbukh

We report the observation of macroscopic field-free orientation, i.e. more than 73 % of CO molecules pointing in the same direction. This is achieved through an all-optical scheme operating at high particle densities ($>10^{17}$cm$^{-3}$)…

Chemical Physics · Physics 2014-07-09 P. M. Kraus , D. Baykusheva , H. J. Wörner

Orientation states of two coupled polar molecules controlled by laser pulses are studied theoretically. By varying the period of a series of periodically applied laser pulse, transition from regular to chaotic behavior may occur. Schmidt…

Quantum Physics · Physics 2007-05-23 Ying-Yen Liao , Yueh-Nan Chen , Der-San Chuu

The use of bichromatic counter-rotating laser field is known to generate high-order harmonics with non-zero ellipticity. By combining such laser field with a plasmonic-enhanced spatially inhomogeneous field, we propose a way to influence…