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Electrons colliding with spatially fixed ions in strong laser fields are investigated by solving the time-dependent Schr\"odinger equation. Considering first simple one-dimensional model systems, the mechanisms and energy spectra of fast…

Atomic Physics · Physics 2015-10-28 S. Bauch , M. Bonitz

Photoelectron spectra obtained from the ab initio solution of the time-dependent Schr\"odinger equation can be in striking disagreement with predictions by the strong-field approximation (SFA) not only at low energy but also around twice…

Atomic Physics · Physics 2016-12-14 Th. Keil , S. V. Popruzhenko , D. Bauer

Wave self-focusing in molecular systems subject to thermal effects, such as thin molecular films and long biomolecules, can be modeled by stochastic versions of the Discrete Self-Trapping equation of Eilbeck, Lomdahl and Scott, and this can…

Pattern Formation and Solitons · Physics 2009-11-11 Brenton LeMesurier , Barron Whitehead

Two non-equidistant grid implementations of infinite range exterior complex scaling are introduced that allow for perfect absorption in the time dependent Schr\"odinger equation. Finite element discrete variables grid discretizations…

Computational Physics · Physics 2015-09-17 Markus Weinmüller , Michael Weinmüller , Jonathan Rohland , Armin Scrinzi

Mesoscopic systems and large molecules are often modeled by graphs of one-dimensional wires, connected at vertices. In this paper we discuss the solutions of the Schr\"odinger equation on such graphs, which have been named "quantum…

Mesoscale and Nanoscale Physics · Physics 2020-04-01 Amnon Aharony , Ora Entin-Wohlman

In this work, we propose an efficient and robust multigrid method for solving the time-fractional heat equation. Due to the nonlocal property of fractional differential operators, numerical methods usually generate systems of equations for…

Numerical Analysis · Mathematics 2017-08-28 Francisco J. Gaspar , Carmen Rodrigo

We present the numerical implementation of the time-dependent complete-active-space self-consistent-field (TD-CASSCF) method [Phys. Rev. A, 88, 023402 (2013)] for atoms driven by a strong linearly polarized laser pulse. The present…

Given access to accurate solutions of the many-electron Schr\"odinger equation, nearly all chemistry could be derived from first principles. Exact wavefunctions of interesting chemical systems are out of reach because they are NP-hard to…

Chemical Physics · Physics 2021-03-26 David Pfau , James S. Spencer , Alexander G. de G. Matthews , W. M. C. Foulkes

We improve the complex scaling method (CSM) to obtain virtual states, which were previously challenging in the conventional CSM. Our approach solves the Schr\"odinger equation in the momentum space as an eigenvalue problem by choosing the…

High Energy Physics - Phenomenology · Physics 2024-02-22 Yan-Ke Chen , Lu Meng , Zi-Yang Lin , Shi-Lin Zhu

One of the unitary forms of the quantum mechanical time evolution operator is given by Cayley's approximation. A numerical implementation of the same involves the replacement of second derivatives in Hamiltonian with the three-point…

Quantum Physics · Physics 2023-09-07 Ankit Kumar

We present a stochastic method for solving the time-dependent Schr\"odinger equation, generalizing a ground-state full configuration interaction Quantum Monte Carlo method. By performing the time-integration in the complex plane close to…

Strongly Correlated Electrons · Physics 2018-08-08 Kai Guther , Werner Dobrautz , Olle Gunnarsson , Ali Alavi

We review two common numerical schemes for Coulomb potential evaluation that differ only in their radial part of the solutions in the spherical harmonic expansion (SHE). One is based on finite-difference method (FDM) while the other is…

Chemical Physics · Physics 2022-05-25 Po-Hao Chang , Zachary Buschmann , Rajendra R. Zope

A fast and stable numerical method is formulated to compute the time evolution of a wave function in a magnetic field by solving the time-dependent Schroedinger equation. This computational method is based on the finite element method in…

Computational Physics · Physics 2009-11-06 Naoki Watanabe , Masaru Tsukada

We show that the method of factorizing the evolution operator to fourth order with purely positive coefficients, in conjunction with Suzuki's method of implementing time-ordering of operators, produces a new class of powerful algorithms for…

Nuclear Theory · Physics 2009-11-07 S. A. Chin , C. R. Chen

A matrix inverse free method to solve time-dependent Schrodinger equation is presented. The method is not subject to form of Hamiltonian and adopting real space grid system such as structured and unstructured grid, and achieves the order N…

Computational Physics · Physics 2007-05-23 Katsuhiro Watanabe , Akihito Kikuchi

Over the last three decades numerous numerical methods for solving the time-dependent Schr\"{o}dinger equation within the single-active electron approximation have been developed for studying ionization of atomic targets exposed to an…

Atomic Physics · Physics 2020-08-12 B. Fetić , W. Becker , D. B. Milošević

This paper improves the convergence and robustness of a multigrid-based solver for the cross sections of the driven Schroedinger equation. Adding an Coupled Channel Correction Step (CCCS) after each multigrid (MG) V-cycle efficiently…

Computational Physics · Physics 2015-09-18 Siegfried Cools , Wim Vanroose

I consider the nonaxisymmetric linear theory of a rotating, isothermal magnetohydrodynamic (MHD) shear flow. The analysis is performed in the shearing box, a local model of a thin disk, using a decomposition in terms of shearing waves,…

Astrophysics · Physics 2011-02-11 Bryan M. Johnson

The Helmholtz equation arises when modeling wave propagation in the frequency domain. The equation is discretized as an indefinite linear system, which is difficult to solve at high wave numbers. In many applications, the solution of the…

Computational Engineering, Finance, and Science · Computer Science 2017-12-19 Eran Treister , Eldad Haber

We consider the interaction of hydrogen-like atoms with a strong laser field and show that the strong field approximation and all its variants may be grouped into a set of families of approximation schemes. This is done by introducing an…

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