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A novel polarization-modulation transient method has been developed for studying fast anisotropic relaxation in electronic excited states of polyatomic and biologically relevant molecules under excitation with femtosecond laser pulses. The…

Chemical Physics · Physics 2020-05-12 Ioanna Gorbunova , Nikolay Bezverkhnii , Maxim Sasin , Idris Gagzhiev , Oleg Vasyutinskii

Measurements of interactions between cold molecules and ultracold atoms can allow for a detailed understanding of fundamental collision processes. These measurements can be done using various experimental geometries including where both…

Atomic Physics · Physics 2020-03-25 N. J. Fitch , L. P. Parazzoli , H. J. Lewandowski

Maximizing nonlinear light-matter interactions is a primary motive for compressing laser pulses to achieve ultrashort transform limited pulses. Here we show how, by appropriately shaping the pulses, resonant multiphoton transitions can be…

Atomic Physics · Physics 2009-11-10 Nirit Dudovich , Barak Dayan , S. M. G. Faeder , Yaron Silberberg

The generation of ultra-strong attosecond pulses through laser-plasma interactions offers the opportunity to surpass the intensity of any known laboratory radiation source, giving rise to new experimental possibilities, such as quantum…

We demonstrate numerically a method of focusing two-photon field inside one-dimensional random media. The approach is based on coherent control of backscattering achieved by adaptive spectral pulse shaping. The spectral phases of a…

Optics · Physics 2016-03-02 Alex C. Han , Valery Milner

We formulate a robust optimal control algorithm to synthesize minimum energy pulses that can transfer a cold atom system into various momentum states. The algorithm uses adaptive linearization of the evolution operator and sequential…

We investigate the interactions between ultracold alkali metal atoms and closed-shell atoms using electronic structure calculations on the prototype system Rb+Sr. There are molecular bound states that can be tuned across atomic thresholds…

Atomic Physics · Physics 2015-05-19 Piotr S. Zuchowski , J. Aldegunde , Jeremy M. Hutson

Molecular polaritons are hybrid states of photonic and molecular character that form when molecules strongly interact with light. Strong coupling tunes energy levels and importantly, can modify molecular properties (e.g. photoreaction…

Chemical Physics · Physics 2023-02-14 Francesca Fassioli , Kyu Hyung Park , Sarah E. Bard , Gregory D. Scholes

Two-color photoassociation of ground state $^6$Li$^{87}$Rb molecules via the $\mathrm{B}^1\Pi$ electronic state using short pulses near a magnetic Feshbach resonance is studied theoretically. A near-resonant magnetic field is applied to mix…

Atomic Physics · Physics 2014-02-04 Marko Gacesa , Subhas Ghosal , Jason Byrd , Robin Côté

A pulse shaping algorithm for a matter wave with the purpose of controlling a binary reaction has been designed. The scheme is illustrated for an Eley-Rideal reaction where an impinging matter-wave atom recombines with an adsorbed atom on a…

Quantum Physics · Physics 2009-11-10 Solvejg Jorgensen , Ronnie Kosloff

High-harmonic generation is one of the most extreme nonlinear-optical processes observed to date. By focusing an intense laser pulse into a gas, the light-atom interaction that occurs during the process of ionising the atoms results in the…

Progress on researches in the field of molecules at cold and ultracold temperatures is reported in this review. It covers extensively the experimental methods to produce, detect and characterize cold and ultracold molecules including…

Quantum Physics · Physics 2015-05-13 Olivier Dulieu , Carlo Gabbanini

A key requirement for quantum technologies based on atoms, ions, and molecules, is the ability to realize precise phase- and amplitude-controlled quantum operations via coherent laser pulses. However, for generating pulses on the…

Quantum Physics · Physics 2025-12-30 Shuzhe Yang , Guido Masella , Vase Moeini , Amar Bellahsene , Chang Li , Tom Bienaimé , Shannon Whitlock

In recent years it became possible to align molecules in free space using ultrashort laser pulses. Here we explore two schemes for controlling molecule-surface scattering process, which are based on the laser-induced molecular alignment. In…

Chemical Physics · Physics 2015-05-28 Yuri Khodorkovsky , J. R. Manson , Ilya Sh. Averbukh

We report the production of ultracold 7Li85Rb molecules by photoassociation (PA) below the Li (2s 2S1/2) + Rb (5p 2P1/2) asymptote. We perform PA spectroscopy in a dual-species 7Li-85Rb magneto-optical trap (MOT) and detect the PA…

Atomic Physics · Physics 2014-05-06 Sourav Dutta , D. S. Elliott , Yong P. Chen

We demonstrate a method to make mixtures of ultracold atoms that does not make use of a two-species magneto-optical trap. We prepare two clouds of 87Rb atoms in distinct magnetic quadrupole traps and mix the two clouds by merging the traps.…

Other Condensed Matter · Physics 2007-05-23 Jesper Fevre Bertelsen , Henrik Kjaer Andersen , Sune Mai , Michael Budde

Scattering by atmospheric turbulence is one of the main challenges in creating long free-space optical links, and specifically links of entangled photons. Classical compensation methods are hard to apply to entangled photons, due to…

Quantum Physics · Physics 2022-02-18 Ronen Shekel , Ohad Lib , Yaron Bromberg , Alon Sardas

We study theoretically lattice modulation experiments with ultracold fermions in optical lattices. We focus on the regime relevant to current experiments when interaction strength is larger than the bandwidth and temperature is higher than…

Quantum Gases · Physics 2012-05-04 Akiyuki Tokuno , Eugene Demler , Thierry Giamarchi

Light shaping facilitates the preparation and detection of optical states and underlies many applications in communications, computing, and imaging. In this Letter, we generalize light shaping to the quantum domain. We show that patterns of…

Optics · Physics 2018-12-27 Hugo Defienne , Matthew Reichert , Jason W. Fleischer

We investigate the interaction of femtosecond laser pulses with spins including relativistic corrections. The time-ordered magneto-optical signals corresponding to a pump-probe configuration are calculated in the case of one electron…

Strongly Correlated Electrons · Physics 2012-01-04 Hélène Vonesch , Jean-Yves Bigot
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