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The structure and photoexcitation dynamics of high lying doubly excited states of the strontium atom with high angular momenta are studied in the vicinity of the Sr$^+(N=5)$ threshold. The spectra recorded using resonant multiphoton…

Atomic Physics · Physics 2023-02-08 M. Génévriez , U. Eichmann

We report on the observation of electromagnetically induced transparency (EIT) and absorption (EIA) of highly excited Rydberg states in thermal Cs vapor using a four-step excitation scheme. The advantage of this four-step scheme is that the…

Exploring controllable interactions lies at the heart of quantum science. Neutral Rydberg atoms provide a versatile route toward flexible interactions between single quanta. Previous efforts mainly focused on the excitation…

Quantum Physics · Physics 2021-02-02 Xiao-Feng Shi

The influence of negative-energy states (NES) on forbidden magnetic-dipole $ns_{1/2}-(n+1)s_{1/2}$ transitions in alkali-metal atoms is investigated. We find that the NES contributions are significant in almost all cases and for rubidium…

Atomic Physics · Physics 2009-10-31 I. M. Savukov , A. Derevianko , H. G. Berry , W. R. Johnson

Rydberg atoms with dipole-dipole interactions provide intriguing platforms to explore exotic quantum many-body physics. Here we propose a novel scheme with laser-assisted dipole-dipole interactions to realize synthetic magnetic field for…

Mesoscale and Nanoscale Physics · Physics 2022-08-09 Tian-Hua Yang , Bao-Zong Wang , Xin-Chi Zhou , Xiong-Jun Liu

We report on the observation of interactions between ultracold Rydberg atoms and ions in a Paul trap. The rate of observed inelastic collisions, which manifest themselves as charge transfer between the Rydberg atoms and ions, exceeds that…

Atomic Physics · Physics 2019-07-03 N. V. Ewald , T. Feldker , H. Hirzler , H. Fürst , R. Gerritsma

The energy dependence of the rates of the reactions between He$^+$ and ammonia (NY$_3$, Y= {H,D}), forming NY$_2^+$, Y and He as well as NY$^+$, Y$_2$ and He, and the corresponding product branching ratios have been measured at low…

We demonstrate the interaction-induced blockade effect in an ultracold $^{88}$Sr gas via studying the time dynamics of a two-photon excitation to the triplet Rydberg series $5\mathrm{s}n\mathrm{s}\, ^3\textrm{S}_1$ for five different…

We investigate the implementation of a controlled-Z gate on a pair of Rydberg atoms in spatially separated dipole traps where the joint excitation of both atoms into the Rydberg level is strongly suppressed (the Rydberg blockade). We follow…

A three-level atomic medium can be made transparent to a resonant probe field in the presence of a strong control field acting on an adjacent atomic transition to a long-lived state, which can be represented by a highly excited Rydberg…

Quantum Physics · Physics 2017-03-16 David Petrosyan

Quantum information processing with neutral atoms relies on Rydberg excitation for entanglement generation. While the use of heavy divalent or open-shell elements, such as strontium or ytterbium, has benefits due to their optically active…

We analyze in detail the possibility to use charge-dipole interaction between a single polar molecule or a 1D molecular array and a single Rydberg atom to read out rotational populations. The change in the Rydberg electron energy is…

Quantum Physics · Physics 2016-10-05 Elena Kuznetsova , Seth T. Rittenhouse , H. R. Sadeghpour , Susanne F. Yelin

We explore a single-photon approach to Rydberg state excitation and Rydberg blockade. Using detailed theoretical models, we show the feasibility of direct excitation, predict the effect of background electric fields, and calculate the…

We have observed Stueckelberg oscillations in the dipole-dipole interaction between Rydberg atoms with an externally applied radio-frequency field. The oscillating RF field brings the interaction between cold Rydberg atoms in two separated…

Using the Brink-Axel hypothesis we derive the rate $R$ for nuclear dipole excitation by a laser pulse carrying $N \gg 1$ photons with average energy $\hbar \omega_0 \approx 5$ MeV. As expected $R \propto (\hbar \omega_0)^3$. The rate is…

Nuclear Theory · Physics 2020-05-06 Adriana Pálffy , Paul-Gerhard Reinhard , Hans A. Weidenmüller

Excitation of two identical species in a cluster by the absorption of two photons of the same energy is strongly suppressed since the excitation of one subunit blocks the excitation of the other one due to the binding Coulomb interaction.…

Atomic and Molecular Clusters · Physics 2013-01-11 Ph. V. Demekhin , K. Gokhberg , G. Jabbari , S. Kopelke , A. I. Kuleff , L. S. Cederbaum

We investigate a long-range interaction between $64D_{5/2}$ Rydberg-atom pairs and antiblockade effect employing a two-color excitation scheme. The first color (pulse A) is set to resonantly excite the Rydberg transition and prepare a few…

Atomic Physics · Physics 2020-02-25 Suying Bai , Xuedong Tian , Xiaoxuan Han , Yuechun Jiao , Jinhui Wu , Jianming Zhao , Suotang Jia

A three level ladder system is analyzed and the coherence of initially electric-dipole forbidden transition is calculated. Due to the presence of two laser fields the initially dipole forbidden transition becomes dynamically permitted due…

Optics · Physics 2014-02-13 Gennady A. Koganov , Reuben Shuker

We describe a method for controlling many-body states in extended ensembles of Rydberg atoms, forming crystalline structures during laser excitation of a frozen atomic gas. Specifically, we predict the existence of an excitation number…

Atomic Physics · Physics 2015-05-14 T. Pohl , E. Demler , M. D. Lukin

Rydberg atoms with principal quantum number n >> 1 have exaggerated atomic properties including dipole-dipole interactions that scale as n^4 and radiative lifetimes that scale as n^3. It was proposed a decade ago to take advantage of these…

Quantum Physics · Physics 2015-03-13 M. Saffman , T. G. Walker , K. Molmer