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Electrostatic velocity filtering and guiding is an established technique to produce high fluxes of cold polar molecules. In this paper we clarify different aspects of this technique by comparing experiments to detailed calculations. In the…

Chemical Physics · Physics 2009-01-14 M. Motsch , L. D. van Buuren , C. Sommer , M. Zeppenfeld , G. Rempe , P. W. H. Pinkse

An inhomogeneous electric field is used to study the deflection of a supersonic beam of water molecules. The deflection profiles show strong broadening accompanied by a small net displacement towards higher electric fields. The profiles are…

Chemical Physics · Physics 2009-11-13 Ramiro Moro , Jaap Bulthuis , Jonathon Heinrich , Vitaly V. Kresin

The properties of amorphous solid water at and near the calorimetric glass transition temperature, $T_{g}$, of 136 K have been debated for years. One hypothesis is that water turns into a "true" liquid at $T_{g}$ (i.e., it becomes ergodic)…

Soft Condensed Matter · Physics 2025-03-03 Greg A. Kimmel , Megan K. Dunlap , Kirill Gurdumov , R. Scott Smith , Loni Kringle , Bruce D. Kay

Stark effect is calculated by the perturbation theory method separately for the ortho and para water molecules. At room temperature, a 30%-difference in the energy change is found for the two species put in electric field. This implies a…

Chemical Physics · Physics 2007-05-23 S. N. Andreev , V. P. Makarov , V. I. Tikhonov , A. A. Volkov

A method of slowing, accelerating, cooling, and bunching molecules and neutral atoms using time-varying electric field gradients is demonstrated with cesium atoms in a fountain. The effects are measured and found to be in agreement with…

Atomic Physics · Physics 2009-10-31 Jason A. Maddi , Timothy P. Dinneen , Harvey Gould

We describe the generation and properties of a cryogenic beam of $^7$Li$_2$ dimers from sublimation of a neon matrix where lithium atoms have been implanted via laser ablation of solid precursors of metallic lithium or lithium hydride…

The Stark interaction of polar molecules with an inhomogeneous electric field is exploited to select slow molecules from a room-temperature reservoir and guide them into an ultrahigh vacuum chamber. A linear electrostatic quadrupole with a…

Chemical Physics · Physics 2009-11-07 S. A. Rangwala , T. Junglen , T. Rieger , P. W. H. Pinkse , G. Rempe

Carbon monoxide molecules in their electronic, vibrational, and rotational ground state are highly attractive for trapping experiments. The optical or ac electric traps that can be envisioned for these molecules will be very shallow,…

Isotopically layered amorphous solid water films were used to measure the diffusivity of deeply supercooled liquid water near the glass transition. The films, composed of separate layers of oxygen 16 and oxygen 18 labeled water, were grown…

Soft Condensed Matter · Physics 2025-02-06 R. Scott Smith , Wyatt A. Thornley , Greg A. Kimmel , Bruce D. Kay

We have simulated structure and dynamics of water in the grooves of a DNA duplex using moleculear dynamics simulations. We find signatures of a dynamical transition in both translational and orientational dynamics of water molecules in both…

Soft Condensed Matter · Physics 2008-09-23 Debasmita Biswal , Biman Jana , Subrata Pal , Biman Bagchi

The static and dynamical properties of heavy water have been studied at ambient conditions with extensive Car-Parrinello molecular-dynamics simulations in the canonical ensemble, with temperatures ranging between 325 K and 400 K.…

Soft Condensed Matter · Physics 2007-05-23 P. H-L. Sit , Nicola Marzari

Any evolving system can change of state via thermal mechanisms (hopping a barrier) or via quantum tunneling. Most of the time, efficient classical mechanisms dominate at high temperatures. This is why an increase of the temperature can…

Materials Science · Physics 2014-02-14 M. Minissale , E. Congiu , S. Baouche , H. Chaabouni , A. Moudens , F. Dulieu , M. Accolla , S. Cazaux , G. Manico , V. Pirronello

We predict that it is possible to cool rotational, vibrational and translational degrees of freedom of molecules by coupling a molecular dipole transition to an optical cavity. The dynamics is numerically simulated for a realistic set of…

Quantum Physics · Physics 2007-08-13 Giovanna Morigi , Pepijn W. H. Pinkse , Markus Kowalewski , Regina de Vivie-Riedle

Raising the temperature of a material enhances the thermal motion of particles. Such an increase in thermal energy commonly leads to the melting of a solid into a fluid and eventually vaporises the liquid into a gaseous phase of matter.…

We propose a general method to cool the translational motion of molecules. Our method is an extension of single photon atomic cooling which was successfully implemented in our laboratory. Requiring a single event of absorption followed by a…

Chemical Physics · Physics 2015-05-13 Edvardas Narevicius , S. Travis Bannerman , Mark G. Raizen

We present the detection of four rotational emission lines of water vapor, from energy levels Eu/k= 101 - 454 K, in the gravitationally lensed z=3.9 QSO host galaxy APM08279+5255. While the lowest H2O lines are collisionally excited in…

Cosmology and Nongalactic Astrophysics · Physics 2015-05-28 Paul P. van der Werf , Alicia Berciano Alba , Marco Spaans , Edo Loenen , Rowin Meijerink , Dominik Riechers , Pierre Cox , Axel Weiss , Fabian Walter

A novel concept of membrane process in thermal-driven system is proposed for water desalination. By means of molecular dynamics simulations, we show fast water transport through graphene galleries at a temperature gradient. Water molecules…

Soft Condensed Matter · Physics 2018-10-29 Bo Chen , Haifeng Jiang , Huidong Liu , Kang Liu , Xiang Liu , Xuejiao Hu

The development of the magneto-optical trap revolutionized the fields of atomic and quantum physics by providing a simple method for the rapid production of ultracold, trapped atoms. A similar technique for producing a diverse set of dense,…

Atomic Physics · Physics 2014-04-17 Matthew T. Hummon , Mark Yeo , Benjamin K. Stuhl , Alejandra L. Collopy , Yong Xia , Jun Ye

We conducted series of experiments on observing a Stark-type effect in superfluid $^4$He in presence of relative laminar flows of the normal and superfluid components. It is designed a measurement cell which allows us to simultaneously…

Employing a two-stage cryogenic buffer gas cell, we produce a cold, hydrodynamically extracted beam of calcium monohydride molecules with a near effusive velocity distribution. Beam dynamics, thermalization and slowing are studied using…

Atomic Physics · Physics 2017-09-13 Hsin-I Lu , Julia Rasmussen , Matthew J. Wright , Dave Patterson , John M. Doyle
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