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A simple scheme of population and detection of low-lying electronic quadrupole modes in free small deformed metal clusters is proposed. The scheme is analyzed in terms of the TDLDA (time-dependent local density approximation) calculations.…

Atomic and Molecular Clusters · Physics 2014-02-04 V. O. Nesterenko , P. -G. Reinhard , T. Halfmann , L. I. Pavlov

We analyze particular two-photon processes as possible means to explore electronic quadrupole states in free small deformed atomic clusters. The analysis is done in the time-dependent local density approximation (TDLDA). It is shown that…

Atomic and Molecular Clusters · Physics 2011-05-26 V. O. Nesterenko , P. -G. Reinhard , Th. Halfmann , E. Suraud

We apply the time-dependent local density approximation (TDLDA) to calculate dipole excitations in small carbon clusters. A strong low-frequency mode is found which agrees well with observation for clusters C_n with n in the range 7-15. The…

Chemical Physics · Physics 2009-10-30 K. Yabana , G. F. Bertsch

Various ways to analyze the dynamical response of clusters and molecules to electromagnetic perturbations exist. Particularly rich information can be obtained from measuring the properties of electrons emitted in the course of the…

Atomic and Molecular Clusters · Physics 2015-06-11 P. Wopperer , P. M. Dinh , P. -G. Reinhard , E. Suraud

The existence and nature of a new mode of electronic collective excitations (quadrupole plasmons) in confined one-dimensional electronic systems have been predicted by an eigen-equation method. The eigen-equation based on the time-dependent…

Mesoscale and Nanoscale Physics · Physics 2015-06-18 Reng-lai Wu , Yabin Yu , Hong-jie Xue

Infrared quadrupole modes (IRQM) of the valence electrons in light deformed sodium clusters are studied by means of the time-dependent local-density approximation (TDLDA). IRQM are classified by angular momentum components $\lambda\mu =$20,…

Atomic and Molecular Clusters · Physics 2009-02-05 V. O. Nesterenko , P. -G. Reinhard , W. Kleinig , D. S. Dolci

We discuss the calculation of collective excitations in atomic clusters using the time-dependent local density approximation. In principle there are many formulations of the TDLDA, but we have found that a particularly efficient method for…

Atomic and Molecular Clusters · Physics 2009-10-30 G. F. Bertsch , K. Yabana

A remarkable orbital quadrupole magnetic resonance, so-called twist mode, is predicted in alkali metal clusters where it is represented by $I^{\pi}=2^-$ low-energy excitations of valence electrons with strong M2 transitions to the ground…

Mesoscale and Nanoscale Physics · Physics 2008-11-26 V. O. Nesterenko , J. R. Marinelli , F. F. de Souza Cruz , W. Kleinig , P. -G. Reinhard

The electronic structure and optical properties of metallic nanoshells are investigated using a jellium model and the Time Dependent Local Density Approximation (TDLDA). An efficient numerical implementation enables applications to…

Materials Science · Physics 2009-11-10 P. Nordlander , E. Prodan

We have carried out a unified microscopic study of electric monopole, quadrupole and magnetic dipole excitations in fast rotating nuclei undergoing backbending, with special attention at the magnetic excitations. We found, among other…

Nuclear Theory · Physics 2007-05-23 J. Kvasil , N. Lo Iudice , R. G. Nazmitdinov , A. Porrino , F. Knapp

Collective plasma excitations in moir\'e flat bands display unique properties reflecting strong electron-electron interactions and unusual carrier dynamics in these systems. Unlike the conventional two-dimensional plasmon modes, dispersing…

Mesoscale and Nanoscale Physics · Physics 2020-11-06 Ali Fahimniya , Cyprian Lewandowski , Leonid Levitov

The collective electronic excitation in planar sodium clusters is studied by time-dependent density functional theory calculations. The formation and development of the resonances in photoabsorption spectra are investigated in terms of the…

Mesoscale and Nanoscale Physics · Physics 2013-06-17 Bao-Ji Wang , San-Huang Ke

Electron-positron clusters are studied using a quantum hydrodynamic model that includes Coulomb and exchange interactions. A variational Lagrangian method is used to determine their stationary and dynamical properties. The cluster static…

Plasma Physics · Physics 2012-12-03 Giovanni Manfredi , Paul-Antoine Hervieux , Fernando Haas

We describe the structure of the time-harmonic electromagnetic field of a vertical Hertzian electric dipole source radiating over an infinite, translation invariant two-dimensional electron system. Our model for the electron flow takes into…

Mesoscale and Nanoscale Physics · Physics 2020-11-18 Vera Andreeva , Denis A. Bandurin , Mitchell Luskin , Dionisios Margetis

We perform a detailed study of the phase transitions and mechanisms of electron localization in the extended Hubbard model using the dynamical cluster approximation on a $2\times 2$ cluster. We explore the interplay of charge order and Mott…

Strongly Correlated Electrons · Physics 2021-08-25 Hanna Terletska , Sergei Iskakov , Thomas Maier , Emanuel Gull

Time-dependent density-functional theory (TDDFT) is widely used to describe electronic excitations in complex finite systems with large numbers of atoms, such as biomolecules and nanocrystals. The first part of this paper will give a simple…

Materials Science · Physics 2008-08-15 C. A. Ullrich , V. Turkowski

We investigate the impact of dissipation on the energy balance in the electron dynamics of metal clusters excited by strong electro-magnetic pulses. The dynamics is described theoretically by Time-Dependent Density-Functional Theory (TDDFT)…

Mesoscale and Nanoscale Physics · Physics 2017-02-01 M. Vincedon , E. Suraud , P. -G. Reinhard

Toroidal dipole moments, which consist of enclosed circulating currents aligned along paths within a torus shape, can be experimentally achieved in metamaterials using various geometrical configurations. Here, we investigate the excitation…

Optics · Physics 2024-06-12 Tiago José Arruda

The random-phase-approximation (RPA) method with separable residual forces (SRPA) is proposed for the description of multipole electric oscillations of valence electrons in deformed alkali metal clusters. Both the deformed mean field and…

Atomic and Molecular Clusters · Physics 2009-11-07 W. Kleinig , V. O. Nesterenko , P. G. Reinhard

A novel approach to electronic correlations and magnetism of crystals based on realistic electronic structure calculations is reviewed. In its simplest form it is a combination of the ``local density approximation'' (LDA) and the dynamical…

Strongly Correlated Electrons · Physics 2007-05-23 A. I. Lichtenstein , M. I. Katsnelson , G. Kotliar
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