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We show that high-resolution laser spectroscopy can probe surface interactions of gas confined in nano-cavities of porous materials. We report on strong line broadening and unfamiliar lineshapes due to tight confinement, as well as signal…

Atomic Physics · Physics 2010-01-13 Tomas Svensson , Zhijian Shen

We measure the resonance line shape of atomic vapor layers with nanoscale thickness confined between two sapphire windows. The measurement is performed by scanning a probe laser through resonance and collecting the scattered light. The line…

Atomic Physics · Physics 2015-11-18 K. A. Whittaker , J. Keaveney , I. G. Hughes , A. Sargsyan , D. Sarkisyan , C. S. Adams

A nanometer-thin-cell (in the direction of laser beam propagation) has been elaborated with the thickness of the atomic vapor column varying smoothly in the range of $L = \unit[50-1500]{nm}$. The cell allows one to study the behavior of the…

Atomic Physics · Physics 2016-04-20 A. Sargsyan , Y. Pashayan-Leroy , C. Leroy , D. Sarkisyan

We report on precision spectroscopy of sub-wavelength confined molecular gases. This was obtained by rovibrational selective reflection of $\mathrm{NH_3}$ and $\mathrm{SF_6}$ gases using a quantum cascade laser at $\lambda\approx 10.6 \mu…

This paper presents our current measurements in a vapor nanocell aiming at a test of the distance-dependence of the atom-surface interaction, when simple asymptotic descriptions may turn to be not valid. A state-of-the-art of atom-surface…

A new nano-cell with smoothly varying longitudinal thickness of the atomic vapour layer L in the range of 350 - 5100 nm allowing to study the resonant absorption of D1 and D2 lines of Cs atoms for thicknesses changing from L = Lambda/2 to L…

Atomic Physics · Physics 2007-12-30 A. Sargsyan , D. Sarkisyan , Y. Pashayan-Leroy , C. Leroy , P. Moroshkin , A. Weis

Miniaturizing and integrating atomic vapor cells is widely investigated for the purposes of fundamental measurements and technological applications such as quantum sensing. Extending such platforms to the realm of molecular physics is a…

This chapter deals with atom-wall interaction occurring in the "long-range" regime (typical distances: 1-1000 nm), when the electromagnetic fluctuations of an isolated atom are modified by the vicinity with a surface. Various regimes of…

Atomic Physics · Physics 2007-05-23 Daniel Bloch , Martial Ducloy

We measure the modification of the transmission spectra of cold $^{87}$Rb atoms in the proximity of an optical nanofiber (ONF). Van der Waals interactions between the atoms an the ONF surface decrease the resonance frequency of atoms closer…

Atomic Physics · Physics 2018-03-21 B. D. Patterson , P. Solano , P. S. Julienne , L. A. Orozco , S. L. Rolston

We investigate theoretically dark resonance spectroscopy for a dilute atomic vapor confined in a thin (micro-metric) cell. We identify the physical parameters characterizing the spectra and study their influence. We focus on a Hanle-type…

Quantum Physics · Physics 2009-11-13 Horacio Failache , Lorenzo Lenci , Arturo Lezama , Daniel Bloch , Martial Ducloy

The development of nanotechnology and atom optics relies on understanding how atoms behave and interact with their environment. Isolated atoms can exhibit wave-like (coherent) behaviour with a corresponding de Broglie wavelength and phase…

Atomic Physics · Physics 2009-11-11 John D. Perreault , Alexander D. Cronin

Molecular self-assembly, the function of biomembranes, and the performance of organic solar cells rely on molecular interactions on the nanoscale. The understanding and design of such intrinsic or engineered heterogeneous functional soft…

Chemical Physics · Physics 2013-12-30 Benjamin Pollard , Eric A. Muller , Karsten Hinrichs , Markus B. Raschke

We demonstrate a method for measuring atom-surface interactions using transmission spectroscopy of thermal vapors confined in a wedged nano-cell. The wedged shape of the cell allows complementary measurements of both the bulk atomic vapor…

The nanoscale interaction between single emitters and plasmonic structures is traditionally studied by relying on near-perfect, deterministic, nanoscale-control. This approach is ultra-low throughput thus rendering systematic studies…

Chemical Physics · Physics 2019-04-29 Lisa Saemisch , Matz Liebel , Niek van Hulst

The van der Waals atom-surface attraction, scaling as C3 z-3 for z the atom-surface distance, is expected to be valid in the distance range 1-1000 nm, covering 8-10 orders of magnitudes in the interaction energy. A Cs vapour nanocell allows…

In atom optics a material structure is commonly regarded as an amplitude mask for atom waves. However, atomic diffraction patterns formed using material gratings indicate that material structures also operate as phase masks. In this study a…

Atomic Physics · Physics 2007-05-23 John D. Perreault , Alexander D. Cronin , T. A. Savas

Laser interaction with uniform and nanostructured near-critical plasmas has been investigated by means of 2D particle-in-cell simulations. The effect of a nanostructure (modeled as a collection of solid-density nanospheres) on energy…

Plasma Physics · Physics 2017-11-21 Luca Fedeli , Arianna Formenti , Carlo Enrico Bottani , Matteo Passoni

Molecular beams of rare gas atoms and D_2 have been diffracted from 100 nm period SiN_x transmission gratings. The relative intensities of the diffraction peaks out to the 8th order depend on the diffracting particle and are interpreted in…

Quantum Physics · Physics 2016-09-08 R. E. Grisenti , W. Schoellkopf , J. P. Toennies , G. C. Hegerfeldt , T. Koehler

We report the optical imaging of a single atom with nanometer resolution using an adaptive optical alignment technique that is applicable to general optical microscopy. By decomposing the image of a single laser-cooled atom, we identify and…

Atomic Physics · Physics 2016-09-21 J. D. Wong-Campos , K. G. Johnson , B. Neyenhuis , J. Mizrahi , C. Monroe

The ability to confine light into tiny spatial dimensions is important for applications such as microscopy, sensing and nanoscale lasers. While plasmons offer an appealing avenue to confine light, Landau damping in metals imposes a…

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