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The dispersion component of the van der Waals (vdW) interaction in low-dimensional metals is known to exhibit anomalous "Type-C non-additivity" [Int. J. Quantum Chem. 114, 1157 (2014)]. This causes dispersion energy behavior, at…

Mesoscale and Nanoscale Physics · Physics 2023-08-24 John F. Dobson , Alberto Ambroselli

We devise a nonlocal correlation energy functional that describes the entire range of dispersion interactions in a seamless fashion using only the electron density as input. The new functional is considerably simpler than its predecessors…

Chemical Physics · Physics 2010-12-27 Oleg A. Vydrov , Troy Van Voorhis

The dynamical conductivity of interacting multiband electronic systems derived in Ref.[1] is shown to be consistent with the general form of the Ward identity. Using the semiphenomenological form of this conductivity formula, we have…

Mesoscale and Nanoscale Physics · Physics 2015-01-09 I. Kupcic

The density functional theory (DFT) interaction energy of a dimer is rigorously derived from the monomer densities. To this end, the supermolecular energy bifunctional is formulated in terms of mutually orthogonal sets of orbitals of the…

Van der Waals heterostructures have recently emerged as an exciting platform for investigating the effects of strong electronic correlations, including various forms of magnetic or electrical orders. Here, we perform an unbiased exact…

Strongly Correlated Electrons · Physics 2024-07-15 Ahmed Abouelkomsan , Emil J. Bergholtz , Shubhayu Chatterjee

The phases of A$_2$Mn$_8$O$_{16}$ hollandite group oxides emerge from the competition between ionic interactions, Jahn-Teller effects, charge ordering, and magnetic interactions. Their balanced treatment with feasible computational…

Materials Science · Physics 2017-12-06 Merzuk Kaltak , Marivi Fernandez-Serra , Mark S Hybertsen

We use the truncated-unity functional renormalization group (TUFRG) to study many-body instabilities of correlated electrons in graphene doped near the van Hove singularity (VHS). The system is described by an extended Hubbard model…

Strongly Correlated Electrons · Physics 2025-09-25 Jin-Ju Ri , Song-Jin O , Chol-Su O

An outstanding challenge of theoretical electronic structure is the description of van der Waals (vdW) interactions in molecules and solids. Renewed interest in resolving this is in part motivated by the technological promise of layered…

Materials Science · Physics 2016-01-20 Luke Shulenburger , Andrew D. Baczewski , Zhen Zhu , Jie Guan , David Tomanek

Motivated by recent experiments on correlated van der Waals materials, including twisted and rhombohedral graphene and twisted WSe$_2$, we perform an analytical and numerical study of the effects of strong on-site and short-range…

Strongly Correlated Electrons · Physics 2024-12-16 Patrick H. Wilhelm , Andreas M. Läuchli , Mathias S. Scheurer

Various strong coupling theories of the one-component plasma have successfully predicted the thermodynamic and structural properties by separating the Coulomb potential into short- and long-ranged parts in {\itshape ad hoc} ways. Moreover,…

Statistical Mechanics · Physics 2018-11-07 Hiroshi Frusawa

Polyphenols are natural molecules of crucial importance in many applications, of which tannic acid (TA) is one of the most abundant and established. Most high-value applications require precise control of TA interactions with the system of…

Molecular dimers are widely utilized as a tool to investigate the structure-property relationships behind the complex photophysical processes of condensed-phase systems, where structural tuning remains a challenge. This approach often…

We derive electronic structure models for weakly interacting bilayers such as graphene-graphene and graphene-hexagonal boron nitride, based on density functional theory calculations followed by Wannier transformation of electronic states.…

Mesoscale and Nanoscale Physics · Physics 2016-06-28 Shiang Fang , Efthimios Kaxiras

The processing and material properties of commercial organic semiconductors, for e.g. fullerenes is largely controlled by their precise arrangements, specially intermolecular symmetries, distances and orientations, more specifically,…

Mesoscale and Nanoscale Physics · Physics 2020-12-02 Saunak Das , Johannes Fiedler , Oliver Staufert , Michael Walter , Stefan Yoshi Buhmann , Martin Presselt

By comparing with recently available experimental data from several groups, we critically discuss the manifestation of continuum many body interaction effects in twisted bilayer graphene (tBLG) with small twist angles and low carrier…

Mesoscale and Nanoscale Physics · Physics 2020-06-02 Sankar Das Sarma , Fengcheng Wu

We review recent theoretical progress on the charge dynamics of doped carriers in high-temperature cuprate superconductors. Advances in this field have clarified that doped charges in cuprates exhibit remarkably rich collective behavior,…

Strongly Correlated Electrons · Physics 2026-04-22 Hiroyuki Yamase

We report quadruple configuration interaction calculations within the extended Pariser$-$Parr$-$Pople Hamiltonian on the excited states of aggregates of polyenes, crystalline acenes, and covalently linked dimers of acene molecules. We…

Strongly Correlated Electrons · Physics 2015-04-03 Karan Aryanpour , Alok Shukla , Sumit Mazumdar

We consider a system of particles interacting via a purely repulsive, soft-core potential recently introduced to model effective pair interactions between dendrimers, which is expected to lead to the formation of crystals with multiple…

Soft Condensed Matter · Physics 2015-05-11 Davide Pini

A previously proposed non-canonical coupled-perturbed Kohn-Sham density functional theory (KS-DFT)/Hartree-Fock (HF) treatment for spin-orbit coupling is here generalized to infinite periodic systems. The scalar-relativistic periodic…

Van der Waals heterostructures of atomically thin layers with rotational misalignments, such as twisted bilayer graphene, feature interesting structural moir\'e superlattices. Due to the quantum coupling between the twisted atomic layers,…