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We report the first full-dimensional potential energy surface (PES) and quantum mechanical close-coupling calculations for scattering of SiO due to H$_2$. The full-dimensional interaction potential surface was computed using the explicitly…

The accurate modeling of non-covalent interactions between helium and graphitic materials is important for understanding quantum phenomena in reduced dimensions, with the helium-benzene complex serving as the fundamental prototype. However,…

We present a quantum Monte Carlo study of the solvation and spectroscopic properties of the Mg doped helium clusters MgHe$_n$ with $n=2-50$. Three high level (MP4, CCSD(T) and CCSDT) MgHe interaction potentials have been used to study the…

Atomic and Molecular Clusters · Physics 2009-11-11 Massimo Mella , Gabriele Calderoni , Fausto Cargnoni

For the prototypical diatomic-molecule - diatomic molecule interactions H2-HX and H2-X2, where X = F, Cl, Br, quantum-chemical ab initio calculations are carried out on grids of the configuration space, which permit a spherical-harmonics…

We report a set of adiabatic potential energy surfaces (PESs) for diiodomethane, including the ground electronic state and all excited states accessible via single-photon absorption near 260 nm. Although constrained to four dimensions,…

Chemical Physics · Physics 2026-02-26 Yijue Ding

We present a first principles-quality potential energy surface (PES) describing the inter-atomic forces for hydrogen atoms interacting with free-standing graphene. The PES is a high-dimensional neural network potential that has been…

The NH2 + O reaction represents a critical oxidation pathway in ammonia and hydrazine combustion, yet significant discrepancies persist in reported kinetics. Here, we generate a full-dimensional ground-state potential energy surface (PES)…

Chemical Physics · Physics 2026-03-24 Ying Xing , Weijie Hua , Junxiang Zuo

A potential energy surface for the lowest quartet electronic state of lithium trimer is developed and used to study spin-polarized Li + Li_2 collisions at ultralow kinetic energies. The potential energy surface allows barrierless atom…

Chemical Physics · Physics 2009-11-13 Marko T. Cvitas , Pavel Soldan , Jeremy M. Hutson , Pascal Honvault , Jean-Michel Launay

New particles with masses in the sub-eV range have been predicted by various theories beyond the Standard Model. Some can induce new spin-spin interactions between fermions. Existing constraints on such interactions between nucleons with…

Atomic Physics · Physics 2011-03-04 Changbo Fu , W. M. Snow

Reaction probabilities as a function of total angular momentum and the resulting reaction cross-sections for the collision of open shell S($^1$D) atoms with para-hydrogen have been calculated in the kinetic energy range 0.09--10 meV (1--120…

Chemical Physics · Physics 2015-05-28 Manuel Lara , P. G. Jambrina , A. J. C. Varandas , J. -M. Launay , F. J. Aoiz

This work discusses a protocol for constructing highly accurate potential energy curves (PECs) for the lowest two states of Rb$_{2}^+$, i.e. $X\,{}^2{\Sigma}{_g^+}$ and $(1) {}^2\Sigma{_u^+}$, using an additivity scheme based on…

Atomic Physics · Physics 2022-09-21 Jan Schnabel , Lan Cheng , Andreas Köhn

Collisional excitation of light hydrides is important to fully understand the complex chemical and physical processes of atmospheric and astrophysical environments. Here, we focus on the NH(X3{\Sigma}-)-Ar van der Waals system. First, we…

Computational Physics · Physics 2019-06-28 D. Prudenzano , F. Lique , R. Ramachandran , L. Bizzocchi , P. Caselli

We report state-of-the-art ab initio calculations of the potential energy curve for the $a^3\Sigma_u^+$ state of the lithium dimer conducted to achieve spectroscopic accuracy ($<$1cm$^{-1}$) without any prior adjustment to fit the…

Chemical Physics · Physics 2021-01-27 Michał Lesiuk , Monika Musiał , Robert Moszynski

Full-dimensional reactive potential energy surfaces (PESs) for the OCS$^+$ cation are constructed to describe S$^+$ loss in the electronic ground state and seven low-lying electronically excited states. High-level \textit{ab initio}…

Chemical Physics · Physics 2026-05-15 Cangtao Yin , Stefan Willitsch , Markus Meuwly

Ab initio quantum chemistry calculations are performed for the mixed alkali triatomic system. Global minima of the ground and first excited doublet states of the trimer are found and Born-Oppenheimer potential energy surfaces of the Li atom…

Chemical Physics · Physics 2018-03-14 Patryk Jasik , Tymon Kilich , Jan Kozicki , Józef E. Sienkiewicz

Pairwise additive potentials for multielectronic atoms interacting with a LiF(001) surface are revisited by including an improved description of the electron density associated with the different lattice sites, as well as non-local electron…

Atomic Physics · Physics 2018-05-16 J. E. Miraglia , M. S. Gravielle

Quantum-mechanical close-coupling calculations for state-to-state cross sections and thermal rates are reported for H2+H2 collisions. Two recently developed potential energy surfaces (PES) for the H2-H2 system are applied, namely, the…

Chemical Physics · Physics 2009-11-11 Renat A. Sultanov , Dennis Guster

Collisions of metastable antiprotonic helium atoms with atoms of the medium induce, among other processes, transitions between hyperfine structure (HFS) states, as well as shifts and broadening of microwave M1 spectral lines. In order to…

Nuclear Theory · Physics 2019-11-26 A. V. Bibikov , G. Ya. Korenman , S. N. Yudin

We employ an accurate, ab initio potential energy surface (PES) which describes the electronic interaction energy between the molecular anion OH$^-$ ($^1\Sigma^+$) and the neutral rubidium atom Rb ($^2S$), to evaluate the elastic and…

Atomic Physics · Physics 2018-07-31 L. González-Sánchez , F. Carelli , F. A. Gianturco , R. Wester

The attractive branch of the interaction potentials with the surface of gold have been computed for a large variety of atomic systems: the hydrogen atom, noble gases (He, Ne, Ar, Kr, Xe), alkali atoms (Li, Na, K, Rb, Cs) and alkaline atoms…

Atomic Physics · Physics 2013-01-15 Grzegorz Łach , Maarten DeKieviet , Ulrich D. Jentschura