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Molecules have vibrational, rotational, spin-orbit and hyperfine degrees of freedom or quantum states, each of which responds in a unique fashion to external electromagnetic radiation. The control over superpositions of these quantum states…

Quantum Physics · Physics 2024-04-29 Svetlana Kotochigova , Qingze Guan , Eite Tiesinga , Vito Scarola , Brian DeMarco , Bryce Gadway

High harmonic spectroscopy has the potential to combine attosecond temporal with sub-Angstrom spatial resolution of the early nuclear and multielectron dynamics in molecules. It involves strong field ionization of the molecule by the IR…

Atomic Physics · Physics 2013-08-08 Valeria Serbinenko , Olga Smirnova

Orientation states of two coupled polar molecules controlled by laser pulses are studied theoretically. By varying the period of a series of periodically applied laser pulse, transition from regular to chaotic behavior may occur. Schmidt…

Quantum Physics · Physics 2007-05-23 Ying-Yen Liao , Yueh-Nan Chen , Der-San Chuu

We provide an exact analytic description of decelerating, stopping and re-accelerating optical solitons in atomic media. By virtue of this solution we describe in detail how spatially localized optical memory bits can be written down, read…

Quantum Physics · Physics 2007-05-23 I. P. Vadeiko , A. V. Rybin , A. R. Bishop

We investigate the effect of incoherent perturbations on atomic photoionization due to a femtosecond mid-infrared laser pulse by solving the time-dependent stochastic Schr\"odinger equation. For a weak laser pulse which causes almost no…

Quantum Physics · Physics 2009-11-13 Kamal P. Singh , Jan M. Rost

Neutral atoms trapped by laser light are amongst the most promising candidates for storing and processing information in a quantum computer or simulator. The application certainly calls for a scalable and flexible scheme for addressing and…

We study theoretically inelastic spectrum of coherent backscattering of laser light by two atoms. For an intense laser field, there are frequency domains of not only constructive but also destructive (self-)interference of the inelastic…

Quantum Physics · Physics 2009-11-13 Vyacheslav Shatokhin

We formulate a theory of slow polaritons in atomic gases and apply it to the slowing down, storing, and redirecting of laser pulses in an EIT medium. The normal modes of the coupled matter and radiation are determined through a full…

Quantum Physics · Physics 2009-11-07 G. Juzeliunas , H. J. Carmichael

The coherent interaction with ultrashort light pulses is a powerful strategy for monitoring and controlling the dynamics of wave packets in all states of matter. As light presents an oscillation period of a few femtoseconds ($T=2.6$~fs in…

We investigate, using the stochastic limit method, the coherent quantum control of a 3-level atom in $\Lambda$-configuration interacting with two laser fields. We prove that, in the generic situation, this interaction entangles the two…

Quantum Physics · Physics 2024-04-30 L. Accardi , S. V. Kozyrev , A. N. Pechen

Half-cycle laser pulse is applied on an absorbed molecule to investigate its alignment and orientation behavior. Crossover from field-free to hindered rotation motion is observed by varying the angel of hindrance of potential well. At small…

Atomic Physics · Physics 2007-05-23 Y. Y. Liao , Y. N. Chen , D. S. Chuu

The acceleration of ions in the interaction of circular polarized laser pulses with overdense plasmas is investigated. For circular polarization laser pulses, the quasi-equilibrium for electrons is established due to the light pressure and…

Accelerator Physics · Physics 2007-12-26 X. Q. Yan , C. Lin , Z. M. Sheng , Z. Y. Guo , B. C. Liu , Y. R. Lu , J. X. Fang , J. E. Chen

In attosecond streaking, an electron is released by a short xuv pulse into a strong near infrared laser field. When the laser coupling between two states in the target is weak relative to the detuning, the streaking technique, which allows…

Atomic Physics · Physics 2015-05-19 Jan Conrad Baggesen , Lars Bojer Madsen

Vacuum-stimulated Raman transitions are driven between two magnetic substates of a rubidium-87 atom strongly coupled to an optical cavity. A magnetic field lifts the degeneracy of these states, and the atom is alternately exposed to laser…

Quantum Physics · Physics 2007-05-23 T. Wilk , S. C. Webster , H. P. Specht , G. Rempe , A. Kuhn

Energy coupling during relativistically intense laser-matter interactions is encoded in the attosecond motion of strongly driven electrons at the pre-formed plasma-vacuum boundary. Studying and controlling this motion can reveal details…

Two-photon optical transitions combined with long-range dipole-dipole interactions can be used for the coherent manipulation of collective metastable states composed of different atoms. We show that it is possible to induce optical…

Quantum Physics · Physics 2007-05-23 M. D. Lukin , P. R. Hemmer

We present a modified optimal control scheme based on the Krotov method, which allows for strict limitations on the spectrum of the optimized laser fields, without losing monotonic convergence of the algorithm. The method guarantees a close…

Quantum Physics · Physics 2008-08-18 Caroline Gollub , Markus Kowalewski , Regina de Vivie-Riedle

We propose and computationally study a method for simultaneously orienting the angular momentum of asymmetric top molecules along: 1) a laboratory-fixed direction; 2) the molecular intermediate moment of inertia axis; 3) the laser field…

Quantum Physics · Physics 2022-11-21 Emil J. Zak

We explore the laser-induced ionization dynamics of N2 and CO2 molecules subjected to a few-cycle, linearly polarized, 800\,nm laser pulse using effective two-dimensional single active electron time-dependent quantum simulations. We show…

Atomic Physics · Physics 2012-10-02 Michel Peters , Tung Nguyen-Dang , Eric Charron , Arne Keller , Osman Atabek

The ionization of atoms with sequences of attosecond pulses gives rise to excited ionic states that are entangled with the emitted photoelectron. Still, the ionic ensemble preserves some coherence that can be controlled through the laser…

Atomic Physics · Physics 2023-03-15 Saad Mehmood , Eva Lindroth , Luca Argenti