Related papers: Laser Control of Atomic Motion inside Diatomic Mol…
We provide a complete toolkit for coherent control experiments on the nano-scale. By exploiting the second harmonic emission from single (150 nm) nonlinear nano-particles, we show that ultrafast femtosecond laser pulses can be compressed…
Observing the motion of the nuclear wavepackets during a molecular reaction, in both space and time, is crucial for understanding and controlling the outcome of photoinduced chemical reactions. We have imaged the motion of a vibrational…
Femtosecond time-resolved x-ray diffraction is employed to study the dynamics of the periodic lattice distortion (PLD) associated with the charge-density-wave (CDW) in K0.3MoO3. Using a multi-pulse scheme we show the ability to extend the…
The coupling of laser light to matter can exert sub-cycle coherent control over material properties, with optically induced currents and magnetism shown to be controllable on ultrafast femtosecond time scales. Here, by employing laser light…
We present the first calculation of coherent backscattering with inelastic scattering by saturated atoms. We consider the scattering of a quasi-monochromatic laser pulse by two distant atoms in free space. By restricting ourselves to…
Quantum coherence in quantum optics is an essential part of optical information processing and light manipulation. Alkali metal vapors, despite the numerous shortcomings, are traditionally used in quantum optics as a working medium due to…
The kinetic energy distribution of D$^+$ ions resulting from the interaction of a femtosecond laser pulse with D$_2$ molecules is calculated based on the rescattering model. From analyzing the molecular dynamics, it is shown that the…
Centre-of-mass atomic motion in an optical lattice near the resonance is shown to be a chaotic walking due to the interplay between coherent internal atomic dynamics and spontaneous emission. Statistical properties of chaotic atomic motion…
We describe the mechanism by which a metamaterial surface can act as an ideal phase-controlled rotatable linear polarizer. With equal-power linearly polarized beams incident on each side of the surface, varying the relative phase rotates…
Questions are raised about certain experimental and theoretical claims that atoms may be stabilized into their bound states, and prevented from achieving full ionization, by the application of adiabatic, ultraintense, high-frequency laser…
How fast can a laser pulse ionize an atom? We address this question by considering pulses that carry a fixed time-integrated energy per-area, and finding those that achieve the double requirement of maximizing the ionization that they…
For sufficiently short relativistic-intensity laser pulses, the disparity in time scales for electron and ion motion causes ions to behave as a fixed, neutralizing background. As the pulse duration or intensity is increased, ion motion…
We introduce an approach to determining the required waveforms to coherently control the optical energy localization in plasmonic nanosystems. This approach is based on the impulsive localized excitation of the nanosystem and time reversal…
We investigate quantum control of a single atom in an optical tweezer trap created by a tightly focused optical beam. We show that longitudinal polarization components in the dipole trap arising from the breakdown of the paraxial…
We have found a new hidden symmetry of time reversal light-atom interaction in the photon echo quantum memory with Raman atomic transition. The time-reversed quantum memory creates generalized conditions for ideal compression/decompression…
A fraction of a laser beam array, whose unknown phase relationships must be set to prescribed values, is launched into a scattering media with random transmission. The resulting output speckle pattern is sampled by an array of photodiodes…
We report generation of cascaded rotational Raman scattering up to 58th orders in coherently excited CO_2 molecules. The high-order Raman scattering, which produces a quasiperiodic frequency comb with more than 600 sidebands, is obtained…
We solve the problem concerning a time optimal return of a particle with a prescribed velocity to the origin by applying a magnitude-bounded force. The equations of controlled motion are derived and explicitly integrated, and the optimal…
The optimal control of two-level systems by time-dependent laser fields is studied using a variational theory. We obtain, for the first time, general analytical expressions for the optimal pulse shapes leading to global maximization or…
The dynamics of atomic levels resonantly coupled by a coherent and intense short high-frequency laser pulse is discussed and it is advocated that this dynamics is sensitively probed by measuring the spectra of the particles emitted. It is…