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High order harmonic generation from clusters is a controversial topic: conflicting theories exist, with different explanations for similar experimental observations. From an experimental point of view, separating the contributions from…

Atomic and Molecular Clusters · Physics 2015-06-12 H. Ruf , C. Handschin , R. Cireasa , N. Thiré , A. Ferré , S. Petit , D. Descamps , E. Mével , E. Constant , V. Blanchet , B. Fabre , Y. Mairesse

We develop a quasi-classical theory of high harmonic generation in semiconductors based on an interband current that has been transformed from Bloch to Wannier basis. The Wannier quasi-classical approach reveals a complete picture of the…

Mesoscale and Nanoscale Physics · Physics 2020-06-18 Andrew M. Parks , Guilmot Ernotte , Adam Thorpe , Chris R. McDonald , Paul B. Corkum , Marco Taucer , Thomas Brabec

Recent years have witnessed significant developments in the study of nonlinear properties of various optical materials at the nanoscale. However, in most cases experimental results on harmonic generation from nanostructured materials are…

A formalism in terms of Hertz potentials is presented describing sum-frequency generation in a uniaxial non-linear crystal. A scheme is proposed consisting in aligning the side-walk propagation of extraordinary waves in combination with…

Optics · Physics 2011-06-23 Shahen Hacyan

Quantum geometry of the electron wave function plays a significant role in the linear and non-linear responses of crystalline materials. Here, we study quantum geometry induced second harmonic generation. We identify non-linear responses…

Mesoscale and Nanoscale Physics · Physics 2022-12-13 Pankaj Bhalla , Kamal Das , Dimitrie Culcer , Amit Agarwal

Nonlinear optical generation has been a well-established way to realize frequency conversion in nonlinear optics, whereas previous studies were just focusing on the scalar light fields. Here we report a concise yet efficient experiment to…

Optics · Physics 2018-11-20 Li Zhang , Fei Lin , Xiaodong Qiu , Lixiang Chen

We present experimental results on the observation of a bulk second-order nonlinear susceptibility derived from both free-space and integrated measurements in silicon nitride. Phase-matching is achieved through dispersion engineering of the…

Rigorous electrodynamical simulations based on the nonlinear Drude model are performed to investigate the influence of strong coupling on high harmonic generation by periodic metal gratings. It is shown that a thin dispersive material with…

Mesoscale and Nanoscale Physics · Physics 2019-08-13 Elena Drobnyh , Ruth Pachter , Maxim Sukharev

Second-order nonlinear optical response allows to detect different properties of the system associated with the inversion symmetry breaking. Here, we use a second harmonic generation effect to investigate the alignment of a…

Mesoscale and Nanoscale Physics · Physics 2020-07-03 E. A. Stepanov , S. V. Semin , C. R. Woods , M. Vandelli , A. V. Kimel , K. S. Novoselov , M. I. Katsnelson

The generation of harmonics by atoms interacting with two circularly polarized and frequency related laser fields is addressed through ab initio numerical simulations. A detailed charaterization of a few specific harmonics is given. In…

Atomic Physics · Physics 2009-11-10 F. Ceccherini , N. Davini , D. Bauer , F. Cornolti

Second-harmonic generation is of paramount importance in several fields of science and technology, including frequency conversion, self-referencing of frequency combs, nonlinear spectroscopy and pulse characterization. Advanced…

A hologram is an optical element storing phase and possibly amplitude information enabling the reconstruction of a three dimensional image of an object by illumination and scattering of a coherent beam of light, and the image is generated…

Optics · Physics 2016-09-21 Euclides Almeida , Ora Bitton , Yehiam Prior

Optical interference holography has been proved to be a useful technique in fabricating periodic photonic crystals in which electromagnetic waves are forbidden in certain frequency bandgaps. Compared to periodic crystals quasicrystals,…

Optics · Physics 2009-11-13 Wing Yim Tam

A new scheme for non-destructive characterization of quasi-phase-matching grating structures and temperature gradients via inverse Fourier theory using second-harmonic-generation experiments is proposed. We show how it is possible to…

Pattern Formation and Solitons · Physics 2007-05-23 Steffen K. Johansen , Pascal Baldi

The second-order nonlinear optical coefficients associated with chirality differ in sign for the two mirror-image forms (enantiomers) of a chiral material. Structures comprised of alternating stacks of the enantiomers can therefore be used…

Chemical Physics · Physics 2019-05-16 Bertrand Busson , Martti Kauranen , Colin Nuckolls , Thomas Katz , André Persoons

Second-harmonic emission at a frequency that is twice the laser frequency is an important diagnostic for nonlinear laser-plasma interaction. It is forbidden for centrosymmetric materials such as the bulk of sapphire. The symmetry, however,…

Quasicrystals, realized in metal alloys, are a class of lattices exhibiting symmetries that fall outside the usual classification for periodic crystals. They do not have translational symmetry and yet the lattice points are well ordered.…

Optics · Physics 2009-11-13 Jun Xu , Rui Ma , Xia Wang , Wing Yim Tam

High-harmonic generation (HHG) in crystalline solids have been examined so far on the basis of one-body energy-band structures arising from electron itineracy in a periodic potential. Here, we show emergence of HHG signals which are…

Strongly Correlated Electrons · Physics 2020-04-22 Shohei Imai , Atsushi Ono , Sumio Ishihara

The discovery of second harmonic generation in 1961 marked the birth of nonlinear optics, unlocking a range of applications from frequency conversion to quantum light generation. Yet, phase matching in bulk nonlinear crystals remains a key…

Quasicrystals,characterized by long-range order without translational symmetry,have catalyzed transformative advances in various fields,including optics in terms of field quasicrystals.Here,we present the first demonstration of photonic…

Optics · Physics 2024-07-15 Min Lin , Xinxin Gou , Zhenwei Xie , Aiping Yang , Luping Du , Xiaocong Yuan