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Single-shot ultrafast absorbance spectroscopy based on the frequency encoding of the kinetics is analyzed theoretically and implemented experimentally. The kinetics are sampled in the frequency domain using linearly chirped, amplified 33 fs…

Single-shot ultrafast absorbance spectroscopy based on the frequency encoding of the kinetics is analyzed theoretically and implemented experimentally. In Part II of the series, arbitrary thickness sample is analysed theroretically. The…

Single-shot ultrafast spectroscopy based on the frequency encoding of transient absorbance kinetics (FDSS) is demonstrated. These kinetics are sampled spectrally using linearly chirped pulses derived from a Ti:sapphire laser. A variable…

Optics · Physics 2007-05-23 Ilya A. Shkrob , Dmitri A. Oulianov , Robert A. Crowell

High time cadence Spectro Polarimetry allows the feasibility of studying magnetic field evolution coupled with the plasma flows. Such a high cadence solar spectropolarimetry if developed will allow one to study magnetic field evolution in…

Instrumentation and Methods for Astrophysics · Physics 2020-01-13 Harsh Mathur

We have developed a single-shot imaging technique that can capture ultrafast events occurring on femtosecond to picosecond time scales. The technique is based on an optical pump-probe method, in which multiple time-delayed femtosecond…

Instrumentation and Detectors · Physics 2018-11-14 Sarang Yeola , Donghoon Kuk , Ki-Yong Kim

Single-shot supercontinuum spectral interferometry (SSSI) is an optical technique that can measure ultrafast transients in the complex index of refraction. This method uses chirped supercontinuum reference/probe pulses that need to be…

Instrumentation and Detectors · Physics 2018-06-05 DinhDuy Tran Vu , Dogeun Jang , Ki-Yong Kim

Single-shot characterization techniques are crucial when dealing with shot-to-shot pulse-shape fluctuations (e.g., unstable laser systems, high-power, or with low repetition rate) since the scanning configurations cannot measure single…

Optics · Physics 2025-07-23 Cristian Barbero , Íñigo J. Sola , Benjamín Alonso

Few-shot fine-grained image classification aims to recognize subcategories with high visual similarity using only a limited number of annotated samples. Existing metric learning-based methods typically rely solely on spatial domain…

Computer Vision and Pattern Recognition · Computer Science 2026-04-17 Meijia Wang , Guochao Wang , Haozhen Chu , Bin Yao , Weichuan Zhang , Yuan Wang , Junpo Yang

Ultra-fast and multi-dimensional spectroscopy gives a powerful looking glass into the dynamics of molecular systems. In particular two-dimensional electronic spectroscopy (2DES) provides a probe of coherence and the flow of energy within…

Quantum Physics · Physics 2021-03-31 André Anda , Jared H. Cole

Single-molecule fluorescence spectroscopy is a powerful method that avoids ensemble averaging, but its temporal resolution is limited by the fluorescence lifetime to nanoseconds at most. At the ensemble level, two-dimensional spectroscopy…

Optics · Physics 2024-10-11 Sanchayeeta Jana , Simon Durst , Markus Lippitz

We have developed a single-shot terahertz time-domain spectrometer to perform optical-pump/terahertz-probe experiments in pulsed, high magnetic fields up to 30 T. The single-shot detection scheme for measuring a terahertz waveform…

Fourier-transform spectroscopy (FTS) has been widely used as a standard analytical technique over the past half-century. FTS is a simple and robust autocorrelation-based technique that is compatible with both temporally coherent and…

Instrumentation and Detectors · Physics 2018-11-21 Kazuki Hashimoto , Takuro Ideguchi

Ultrafast single-shot imaging techniques now reach frame rates of tens of tera-frame-per-second (Tfps) and long sequence depths but are often too complex for large-scale use, both in terms of image acquisition and reconstruction. We propose…

Spin noise spectroscopy has become a widespread technique to extract information on spin dynamics in atomic and solid-state systems, in a potentially non-invasive way, through the optical probing of spin fluctuations. Here we experimentally…

An apporach for the sensing of small amounts of chemical and biochemical material is presented. A frequency selective surface (FSS) made from asymmetric split ring resonators (aDSR) is excited with free space radiation. Due to interference…

Applied Physics · Physics 2021-04-13 Christian Debus , Peter Haring Bolívar

The mathematical theory of compressed sensing (CS) asserts that one can acquire signals from measurements whose rate is much lower than the total bandwidth. Whereas the CS theory is now well developed, challenges concerning hardware…

Information Theory · Computer Science 2013-07-18 Makhlad Chahid , Jerome Bobin , Hamed Shams Mousavi , Emmanuel Candes , Maxime Dahan , Vincent Studer

We propose a novel femtosecond stimulated Raman spectroscopy (FSRS) technique that combines entangled photons with interference detection to select matter pathways and enhance the resolution. Following photo excitation by an actinic pump,…

Quantum Physics · Physics 2014-07-15 Konstantin E. Dorfman , Frank Schlawin , Shaul Mukamel

Wavelength-tunable ultra-intense femtosecond lasers may enable breakthroughs in diverse areas of science spanning attosecond science, particle acceleration and beyond. Conventional crystal-based methods are limited by gain bandwidth and…

Optics · Physics 2026-03-13 Yunxiao He , Xiaonan Ning , Bo Guo , Jianfei Hua , Yuqiu Gu , Wei Lu

Fourier transform spectroscopy (FTS) has been widely used as an analytical tool for many applications in science and engineering. In this paper, we describe the operation principle and practical implementation of an FTS prototype. First,…

Instrumentation and Detectors · Physics 2023-02-02 Sohrab Sheikh-Sofla , Mohammad Neshat

Single-shot terahertz (THz) spectroscopy probes sub-picosecond, non-repetitive events by combining the advantages of laser absorption techniques with the phase-sensitive detection of interferometric methods. However, its usage as a…

Optics · Physics 2025-01-07 Charan R. Nallapareddy , Thomas C. Underwood
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