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Because molecules can have their orientation locked when embedded into a solid rare-gas matrix, their hyperfine structure is strongly perturbed relative to the freely rotating molecule. The addition of an electric field further perturbs the…

Atomic Physics · Physics 2018-10-03 A. C. Vutha , M. Horbatsch , E. A. Hessels

We describe a method for cooling neutral molecules that have magnetic and electric dipole moments using collisions with cold ions. An external magnetic field is used to split the ground rovibrational energy levels of the molecule. The…

Atomic Physics · Physics 2014-08-22 F. Robicheaux

A strong inhomogeneous static electric field is used to spatially disperse a supersonic beam of polar molecules, according to their quantum state. We show that the molecules residing in the lowest-lying rotational states can be selected and…

Recent experiments have demonstrated direct cooling and trapping of diatomic and triatomic molecules in magneto-optical traps (MOTs). However, even the best molecular MOTs to date still have density $10^{-5}$ times smaller than in typical…

Atomic Physics · Physics 2023-04-19 Thomas K. Langin , David DeMille

We consider collisions of electric and magnetic polar molecules, taking the OH radical as an example, subject to combined electric and magnetic static fields. We show that the relative orientation of the fields has an important effect on…

Atomic Physics · Physics 2013-07-16 Goulven Quéméner , John L. Bohn

We derive an equation for the cooling dynamics of the quantum motion of an atom trapped by an external potential inside an optical resonator. This equation has broad validity and allows us to identify novel regimes where the motion can be…

Quantum Physics · Physics 2009-11-11 Stefano Zippilli , Giovanna Morigi

The collisions between linear polar molecules, trapped in a microwave field with circular polarization, are theoretically analyzed. The microwave trap suggested by DeMille \cite{DeMille} seems to be rather advantageous in comparison with…

Atomic Physics · Physics 2015-05-13 Alexander V. Avdeenkov

We explore a technique for decelerating molecules using a static magnetic field and optical pumping. Molecules travel through a spatially varying magnetic field and are repeatedly pumped into a weak-field seeking state as they move towards…

Atomic Physics · Physics 2016-09-20 N. J. Fitch , M. R. Tarbutt

Recently, the spectral manipulation of single photons has been achieved through spatial-temporal modulation of the optical refractive index. Here, we generalize this mechanism to massive particles, i.e. realizing the acceleration or…

Optics · Physics 2022-04-26 Mai Zhang , Xie-hang Yu , Xin-Biao Xu , Guang-Can Guo , Chang-Ling Zou

Ultralight bosons such as axions and dark photons are well-motivated hypothetical particles, whose couplings to ordinary matter can be effectively constrained by stellar cooling. Limits on these interactions can be obtained by demanding…

High Energy Physics - Phenomenology · Physics 2026-04-13 Zhaoyu Bai , Vitor Cardoso , Yifan Chen , Yuyan Li , Jamie I. McDonald , Hyeonseok Seong

Strong-field ionization of polar molecules contains rich dynamical processes such as tunneling, excitation, and Stark shift. These processes occur on a sub-cycle time scale and are difficult to distinguish in ultrafast measurements. Here,…

Atomic Physics · Physics 2021-12-15 Jia-Yin Che , Chao Chen , Shang Wang , Guo-Guo Xin , Yan-Jun Chen

The increasing richness of data related to cold dense matter, from laboratory experiments to neutron-star observations, requires a framework for constraining the properties of such matter that makes use of all relevant information. Here, we…

High Energy Astrophysical Phenomena · Physics 2020-01-08 M. Coleman Miller , Cecilia Chirenti , Frederick K. Lamb

We describe an approach to optically trapping small, chemically stable molecules at cryogenic temperatures by buffer-gas loading a deep optical dipole trap. The ~10 K trap depth will be produced by a tightly-focused, 1064-nm cavity capable…

Accurately predicting the electronic energy deposition of ions in materials is an important challenge in both fundamental and applied research. While employing ab initio simulations to investigate electronic stopping of ions in matter holds…

Atoms in spatially dependent light fields are attracted to local intensity maxima or minima depending on the sign of the frequency difference between the light and the atomic resonance. For light fields confined in open high-Q optical…

Quantum Physics · Physics 2019-08-05 Arthur Jungkind , Wolfgang Niedenzu , Helmut Ritsch

Trapping ultracold molecules in conservative traps is essential for applications -- such as quantum state-controlled chemistry, quantum simulations, and quantum information processing. These applications require high densities or…

Atomic Physics · Physics 2022-11-29 Juliana J. Park , Yu-Kun Lu , Alan O. Jamison , Wolfgang Ketterle

A simple method to control molecular translation with a chemical reaction is demonstrated. Slow NO molecules have been produced by partially canceling the molecular beam velocity of NO$_2$ with the recoil velocity of the NO photofragment.…

Chemical Physics · Physics 2009-09-10 Bum Suk Zhao , So Eun Shin , Sung Tai Park , Xingnan Sun , Doo Soo Chung

Molecular cooling is essential for studying the formation of sub-structure of dissipative dark-matter halos that may host compact objects such as black holes. Here, we analyze the reaction rates relevant for the formation, dissociation, and…

Cosmology and Nongalactic Astrophysics · Physics 2022-08-09 Michael Ryan , James Gurian , Sarah Shandera , Donghui Jeong

We introduce a scheme for deep laser cooling of molecules based on robust dark states at zero velocity. By simulating this scheme, we show it to be a widely applicable method that can reach the recoil limit or below. We demonstrate and…

Atomic Physics · Physics 2019-07-24 L. Caldwell , J. A. Devlin , H. J. Williams , N. J. Fitch , E. A. Hinds , B. E. Sauer , M. R. Tarbutt

We present the design, construction, and characterisation of longitudinal- and transverse-field Zeeman slowers, based on arrays of permanent magnets, for slowing thermal beams of atomic Sr. The slowers are optimised for operation with…

Atomic Physics · Physics 2015-06-18 Ian R. Hill , Yuri B. Ovchinnikov , Elizabeth M. Bridge , E. Anne Curtis , Patrick Gill