Related papers: Photo-Chemical Applications of Phase-Modulus Inter…
We investigate the phase interference effects in the nonlinear Compton scattering via the collision between an high-energy electron and the laser in the intermediate intensity region, and reveal that the importance of interference effects…
Ionization of atoms and molecules in laser fields can lead to various interesting interference structures in the photoelectron spectrum. For the case of a super-intense extreme ultraviolet laser pulse, we identify a novel petal-like…
An ab initio simulation of strong-field photodissociation of diatomic molecules was developed, inspired by recent dissociation experiments of F2-. The transition between electronic states was modeled, including the laser pulse and…
We develop a time-dependent theory to investigate electron dynamics and photoionization processes of diatomic molecules interacting with strong laser fields including electron-electron correlation effects. We combine the recently formulated…
We show that if the laser is intense enough, it may always ionize an atom or induce transitions between discrete energy levels of the atom, no matter what is its frequency. It means in the quantum transition of an atom interacting with an…
We employ heterodyne interferometry to investigate the effect of a single organic molecule on the phase of a propagating laser beam. We report on the first phase-contrast images of individual molecules and demonstrate a single-molecule…
We study the photonic interactions between two distant atoms which are coupled by an optical element (a lens or an optical fiber) focussing part of their emitted radiation onto each other. Two regimes are distinguished depending on the…
The advent of ultrashort soft x-ray pulse sources permits the use of established gas phase spectroscopy methods to investigate ultrafast photochemistry in isolated molecules with element and site specificity. In the present study, we…
We investigate photon merging and splitting processes in inhomogeneous, slowly varying electromagnetic fields. Our study is based on the three-photon polarization tensor following from the Heisenberg-Euler effective action. We put special…
Next generation of ultra-intense laser facilities will lead to novel physical conditions ruled by collective and quantum electrodynamics effects, such as synchrotron-like emission of high-energy photons and electron-positron pair…
We model energy transfer between two coupled four-level chromophores with arbitrarily spaced energy levels. Our analysis takes into account the crucial---yet often ignored---process of initial excitation by light that is incident on the…
The coherence of light from independent ensembles of elementary atomic emitters plays a paramount role in diverse areas of modern optics. We demonstrate the interference of photons scattered from independent ensembles of warm atoms in…
Understanding and controlling the electronic as well as ro-vibrational motion and, thus, the entire chemical dynamics in molecules is the ultimate goal of ultrafast laser and imaging science. In photochemistry, laser-induced dissociation…
Time synchronization and phase shaping of single photons both play fundamental roles in quantum information applications that rely on multi-photon quantum interference. Phase shaping typically requires separate modulators with extra…
The dynamics of atomic levels resonantly coupled by a coherent and intense short high-frequency laser pulse is discussed and it is advocated that this dynamics is sensitively probed by measuring the spectra of the particles emitted. It is…
Loss is a critical roadblock to achieving photonic quantum-enhanced technologies. We explore a modular platform for implementing integrated photonics experiments and consider the effects of loss at different stages of these experiments,…
The local interaction of charges and light in organic solids is the basis of distinct and fundamental effects. We here observe, at the single molecule scale, how a focused laser beam can locally shift by hundreds-time their natural…
We investigate dynamics of atomic and molecular systems exposed to intense, shaped chaotic fields and a weak femtosecond laser pulse theoretically. As a prototype example, the photoionization of a hydrogen atom is considered in detail. The…
Laser-induced electron diffraction is an evolving tabletop method, which aims to image ultrafast structural changes in gas-phase polyatomic molecules with sub-{\AA}ngstr\"om spatial and femtosecond temporal resolution. Here, we provide the…
The development of attosecond technology has enabled the real-time observation of coherent electron motion in atoms, molecules and condensed phases. Experimentally, it is now possible to generate laser pulses of durations of only a few tens…