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Related papers: Extension of the HF program to partially filled f-…

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The internal structure of stripes in the two dimensional Hubbard model is studied by going beyond the Hartree-Fock approximation. Partially filled stripes, consistent with experimental observations, are stabilized by quantum fluctuations,…

Strongly Correlated Electrons · Physics 2009-10-31 E. Louis , F. Guinea , M. P. Lopez-Sancho , J. A. Verges

Some general features of the spectrum of the Hartree-Fock-Bogoliubov equations are examined. Special attention is paid to the asymptotic behavior of the single quasiparticle wave functions (s.qp.w.fs.), matter density distribution and…

Nuclear Theory · Physics 2007-05-23 Aurel Bulgac

In electronic structure theory, the availability of analytical derivative is one of the desired features for a method to be useful in practical applications, as it allows for geometry optimization as well as computation of molecular…

Chemical Physics · Physics 2017-03-08 Takashi Tsuchimochi , Seiichiro Ten-no

A new electronic structure model is developed in which the ground state energy of a molecular system is given by a Hartree-Fock-like expression with parametrized one- and two-electron integrals over an extended (minimal + polarization) set…

Chemical Physics · Physics 2014-02-11 Dimitri N. Laikov

We derive a zero-range pseudopotential that includes all possible terms up to sixth order in derivatives. Within the Hartree-Fock approximation, it gives the average energy that corresponds to a quasi-local nuclear Energy Density Functional…

Nuclear Theory · Physics 2011-06-06 F. Raimondi , B. G. Carlsson , J. Dobaczewski

A new effective interaction PKA1 with $\rho$-tensor couplings for the density-dependent relativistic Hartree-Fock (DDRHF) theory is presented. It is obtained by fitting selected empirical ground state and shell structure properties. It…

Nuclear Theory · Physics 2008-11-26 Wen Hui Long , Hiroyuki Sagawa , Nguyen Van Giai , Jie Meng

In this article, we demonstrate the restricted Hartree-Fock electronic structure computation of the molecule $H_3^+$ through computational algebra. We approximate the Hartree-Fock total energy by a polynomial composed of LCAO coefficients…

Computational Physics · Physics 2024-05-15 Ichio Kikuchi , Akihito Kikuchi

We present two improvements to the tight-binding approximation of time-dependent density functional theory (TD-DFTB): Firstly, we add an exact Hartree-Fock exchange term, which is switched on at large distances, to the ground state…

Chemical Physics · Physics 2015-10-28 Alexander Humeniuk , Roland Mitric

In the limit of infinite spatial dimensions a thermodynamically consistent theory, which is valid for arbitrary value of the Coulombic interaction ($U<\infty$), is built for the Hubbard model when the total auxiliary single-site problem…

Strongly Correlated Electrons · Physics 2014-02-17 A. M. Shvaika

A previously proposed computational procedure for constructing a set of nonorthogonal strongly localised one-electron molecular orbitals (O. Danyliv, L. Kantorovich - physics/0401107) is applied to a perfect $\alpha$-quartz crystal…

Chemical Physics · Physics 2009-11-10 Oleh Danyliv , Lev Kantorovich

A Hartree--Fock analysis of the ground-state electronic structure of the finite spherical jellium model is carried out for systems containing up to $520$ electrons in a positive background field with densities ranging from $10^{-3}$ to $1$.…

Materials Science · Physics 2025-12-09 Michael Píro , Jaroslav Hamrle

With the widespread use of self-consistent field methods, including Hartree-Fock and Density Functional Theory, the implications of accelerating these methods are immense. To this end, we develop a tensor hypercontraction construction with…

Chemical Physics · Physics 2025-08-27 Andreas Erbs Hillers-Bendtsen , Todd J. Martínez

Fractional-spin errors are inherent in all current approximate density functionals, including Hartree-Fock theory, and their origin has been related to strong static correlation effects. The conventional way to encode fractional-spin…

This article examines the time-dependent Hartree-Fock (TDHF) approximation of single-particle dynamics in systems of interacting fermions. We find the TDHF approximation to be accurate when there are sufficiently many particles and the…

Mathematical Physics · Physics 2007-05-23 Claude Bardos , Francois Golse , Alex D. Gottlieb , Norbert J. Mauser

Considering the emblematic Hartree-Fock (HF) energy expression with single Slater determinant and the ortho-normal molecular orbits (MO) in it, expressed as a linear combination (LC) of atomic orbits (LCAO) basis set functions, the HF…

Chemical Physics · Physics 2019-09-04 Sandor Kristyan

This paper reports an implementation of Hartree-Fock linear response with complex orbitals for computing electronic spectra of molecules in a strong external magnetic fields. The implementation is completely general, allowing for…

Chemical Physics · Physics 2019-02-01 Sangita Sen , Kai K. Lange , Erik I. Tellgren

We prove within the Hartree-Fock theory of pseudo-relativistic atoms that the maximal negative ionization charge and the ionization energy of an atom remain bounded independently of the nuclear charge Z and the fine structure constant…

Mathematical Physics · Physics 2010-11-12 Anna Dall'Acqua , Jan Philip Solovej

We introduce a new framework for the low-energy nuclear structure calculations, which describes the single-particle wave function as a superposition of localized Gaussians. It is a hybrid of the Hartree-Fock and antisymmetrized molecular…

Nuclear Theory · Physics 2024-08-01 Masaaki Kimura , Yasutaka Taniguchi

We introduce a framework for resolving electron-hole dynamics within wavefunction-based multiconfigurational time-dependent Hartree-Fock (MCTDHF) theory. Central to this framework is a time-domain generalization of the extended Koopmans'…

Atomic Physics · Physics 2026-01-13 Zhao-Han Zhang , Yang Li , Himadri Pathak , Takeshi Sato , Kenichi L. Ishikawa , Feng He

The f-electron spectral function of the Falicov-Kimball model is calculated via a Keldysh-based many-body formalism originally developed by Brandt and Urbanek. We provide results for both the Bethe lattice and the hypercubic lattice at half…

Strongly Correlated Electrons · Physics 2009-11-10 J. K. Freericks , V. Turkowski , V. Zlatic