Related papers: Cold free radical molecules in the laboratory fram…
We studied the effects of cryogenic cooling of a 2-[3-(4-hydroxystyryl)-5, 5-dimethylcyclohex-2-enylidene] malononitrile (OH1) crystal on the generation of broadband THz pulses via collinear optical rectification of 1350 nm femtosecond…
The possibility of a significant slowdown of particles by removing them from a localized state in an electromagnetic potential well with a fixed spatial distribution is shown with a sufficiently slow decrease in the depth of this well with…
A method of slowing, accelerating, cooling, and bunching molecules and neutral atoms using time-varying electric field gradients is demonstrated with cesium atoms in a fountain. The effects are measured and found to be in agreement with…
Molecular cooling is essential for studying the formation of sub-structure of dissipative dark-matter halos that may host compact objects such as black holes. Here, we analyze the reaction rates relevant for the formation, dissociation, and…
The stereochemical properties of the ultracold ground state OH molecule in the presence of electric and magnetic fields are currently of considerable interest. For example, relevant quantities such as molecular alignment and orientation,…
The control of ultrafast molecular rotational motion has benefited from the development of innovative techniques in strong-field laser physics. Here, we theoretically demonstrate a novel type of coherent control by inducing rotation of an…
We have demonstrated that a supersonic beam of methyl radicals (CH$_3$) in the ground rotational state of both $para$ and $ortho$ species has been slowed down to standstill with a magnetic molecular decelerator, and successfully captured…
We describe a method for cooling neutral molecules that have magnetic and electric dipole moments using collisions with cold ions. An external magnetic field is used to split the ground rovibrational energy levels of the molecule. The…
We present a detailed analysis of the molecular kinetics of CHCl$_3$ in a range of temperatures covering the solid and liquid phases. Using nuclear quadrupolar resonance we determine the relaxation times for the molecular rotations in solid…
It has been roughly three decades since laser cooling techniques produced ultracold atoms, leading to rapid advances in a vast array of fields. Unfortunately laser cooling has not yet been extended to molecules because of their complex…
We investigate laser cooling of an ensemble of atoms in an optical cavity. We demonstrate that when atomic dipoles are sychronized in the regime of steady-state superradiance, the motion of the atoms may be subject to a giant frictional…
We consider a diatomic molecule driven by a linearly polarized laser pulse with a polarization axis rotating with a constant acceleration. This setup is referred to as optical centrifuge, and it is known to lead to high-angular momenta for…
We derive a novel lattice Hamiltonian, the \emph{Molecular Hubbard Hamiltonian} (MHH), which describes the essential many body physics of closed-shell ultracold heteronuclear molecules in their absolute ground state in a…
Molecules with heavy, radioactive nuclei promise extreme sensitivity to fundamental nuclear and particle physics. However, these nuclei are available in limited quantities, which challenges their use in precision measurements. Here we…
When molecules interact with intense light sources of femtosecond or shorter duration the rotational degrees of freedom are frozen during the response to the strong nonperturbative interaction. We show how the frozen degrees of freedom…
Optically pumped magnetometers (OPMs) based on alkali-atom vapors are ultra-sensitive devices for dc and low-frequency ac magnetic measurements. Here, in combination with fast-field-cycling hardware and high-resolution spectroscopic…
Atmospheric pressure steam/oxygen plasma is generated by a 88 Hz, 6kV AC power supply. The properties of the produced plasma are investigated by optical emission spectroscopy (OES). The relative intensity, rotational, vibrational,…
Cold supersonic beams of molecules can be slowed down using a switched sequence of electrostatic field gradients. The energy to be removed is proportional to the mass of the molecules. Here we report deceleration of YbF, which is 7 times…
The term `laser cooling' is applied to the use of optical means to cool the motional energies of either atoms and molecules, or micromirrors. In the literature, these two strands are kept largely separate; both, however suffer from severe…
Frontier orbitals, i.e., the highest occupied and lowest unoccupied orbitals of a molecule, generally determine molecular properties, such as chemical bonding and reactivities. Consequently, there has been a lot of interest in measuring…