Related papers: Measuring the gain dynamics in a conjugated polyme…
A pulsed source of entangled photons is desirable for some applications. Yet, such a source has intrinsic problems arising from the simultaneous arrival of the signal and noise photons to the detectors. These problems are analyzed and…
The water flow through the poly(acrylamide) gel under a constant water pressure is measured by newly designed apparatus. The time evolution of the water flow in the gel, is calculated based on the collective diffusion model of the polymer…
The optimization of material gain in optically pumped dye-doped polymer thin films is an important task in the development of organic solid-state lasers. In this work, we present a theoretical model that accommodates the influence of…
A gain-assisted plasmonic waveguide with two detuned resonators is investigated in the plasmon-induced transparency window. Phase map is employed to study power transmittance and group delay for varying gain coefficients and frequency…
High-gain optical parametric amplification is an important nonlinear process used both as a source of coherent infrared light and as a source of nonclassical light. In this work, we experimentally demonstrate an approach to optical…
We have used the variable stripe technique and pump-probe spectroscopy to investigate both gain and the dynamics of amplified spontaneous emission from CdSe quantum dot structures. We have found modal gain coefficients of 75 and 32 1/cm for…
We study the dynamics of the pump mode in the down-conversion Hamiltonian using the cumulant expansion method, perturbation theory, and the full numerical simulation of systems with a pump mean photon number of up to one hundred thousand.…
We investigate the universality of entanglement kinetics in polymer melts. We compare predictions of a recently developed constitutive equation for disentanglement to molecular dynamics simulations of both united-atom polyethylene and…
A simple and effective single-shot pump-probe technique is reported for studying the ultrafast dynamic processes in various materials. Using only two commercial gratings, a large time window of ~ 95.58 ps is spatially encoded in a single…
We report experimental evidence of electrostatic inhibition of fast electrons, generated in a highly resistive material upon irradiation with an intense ultra-short ($10^{16} W/cm^{2}$, $100 fmsec$) laser pulse. The experiment involves…
Deeply sub-wavelength two-dimensional films may exhibit extraordinarily strong nonlinear effects. Here we show that 2D films exhibit the remarkable property of a phase-controllable nonlinearity, i.e., the amplitude of the nonlinear…
We present an experimental method allowing to quantify slip at the wall in viscous polymer fluids, based on the observation of the evolution under simple shear flow of a photobleached pattern within a fluorescent labeled polymer melt. This…
Pump-probe microscopy is an emerging nonlinear imaging technique based on high repetition rate lasers and fast intensity modulation. Here we present new methods for pump-probe microscopy that keep the beam intensity constant and instead…
While time-resolved pump-probe differential reflectivity and transmitivity measurements are routinely used to monitor the population relaxation dynamics on the subpicosecond time scale, it is also known that the signal in the negative delay…
Conjugated polymers can be reversibly doped by electrochemical means. This doping introduces new sub-bandgap optical absorption bands in the polymer while decreasing the bandgap absorption. To study this behavior, we have prepared an…
We propose, analyze, and evaluate a technique for the joint measurement of time-frequency entanglement between two photons. In particular, we show that the frequency sum and time difference of two photons could be simultaneously measured…
Two-photon lasers require materials with large two-photon gain (2PG) coefficients and low linear and nonlinear losses. Our previous demonstration of large enhancement of two-photon absorption in semiconductors for very different photon…
Hot carrier dynamics in a dispersionless plasmonic structures over a broad wavelength are studied by pump-probe measurements with 45 fs time resolution. The role of direct excited as well as plasmon generated hot carriers on low energy…
In this study, using only a single pulse, pump-probe measurement with a large time window of more than 100 ps is implemented. A commercial grating is used to encode a time window of ~ 56 ps in a single pulse; therefore, there is no need for…
Recent experiments have demonstrated that the glass transition temperature of thin polymer films can be shifted as compared to the same polymer in the bulk, the amplitude and the sign of this effect depending on the interaction between the…