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Density functional theory has been used to study the adsorption of molecular H2 on a graphene layer. Different adsorption sites on top of atoms, bonds and the center of carbon hexagons have been considered and compared. We conclude that the…

Chemical Physics · Physics 2009-11-06 J. S. Arellano , L. M. Molina , A. Rubio , J. A. Alonso

Using density functional theory calculations, we show that the binding strength of a graphene monolayer on Pd(111) can vary between physisorption and chemisorption depending on its orientation. By studying the interfacial charge transfer,…

Materials Science · Physics 2013-03-29 B. B. Kappes , A. Ebnonnasir , S. Kodambaka , C. V. Ciobanu

According to previous interpretations of experimental data, sodium-scandium double-cation borohydride NaSc(BH$_4$)$_4$ crystallizes in the crystallographic space group $Cmcm$ where each sodium (scandium) atom is surrounded by six scandium…

Materials Science · Physics 2014-04-01 Tran Doan Huan , Maximilian Amsler , Silvana Botti , Miguel A. L. Marques , Stefan Goedecker

Within the framework of a model representing the potential of a graphene sheet U(z) as an electro-neutral layer formed by smeared carbon atoms, the effect of this potential on spectral characteristics of atoms adsorbed on a graphene sheet…

Atomic Physics · Physics 2013-10-02 A. S. Baltenkov , V. A. Pikhut

We have studied the adsorption of Li atoms at the hollow sites of graphene nanoribbons (zigzag and armchair), graphene, and fullerenes by means of density functional theory calculations including local and semilocal functionals. The binding…

Materials Science · Physics 2015-05-14 Chananate Uthaisar , Veronica Barone , Juan E. Peralta

We present a density functional study of the structural and electronic properties of small Cu_n (n=1,4) aggregates on defect-free MgO(100). The calculations employ a slab geometry with periodic boundary conditions, supercells with up to 76…

Materials Science · Physics 2009-10-30 V. Musolino , A. Selloni , R. Car

We present a comparative study of metal-organic interface properties obtained from dispersion corrected density functional theory calculations based on two different approaches: the periodic slab supercell technique and cluster models with…

We investigate the effects of Na adsorption on the electronic structure of bare and Ir cluster superlattice covered epitaxial graphene on Ir(111) using angle-resolved photoemission spectroscopy and scanning tunneling microscopy. At Na…

Sodium chloride (NaCl), or rocksalt, is well characterized at ambient pressure. Due to the large electronegativity difference between Na and Cl atoms, it has highly ionic chemical bonding, with stoichiometry 1:1 dictated by charge balance,…

Formation of clusters of interlayer interstitial carbon atoms in graphite is studied by means of molecular dynamics simulation. It is shown that the deformation potential is attractive for interstitials located in one interlayer region and…

Materials Science · Physics 2007-05-23 V. F. Elesin , L. A. Openov

Analytical relationships for the surface and curvature energies of oblate and prolate semi-spheroidal atomic clusters have been obtained. By modifying the cluster shape from a spheroid to a semi-spheroid the most stable shape was changed…

Atomic and Molecular Clusters · Physics 2007-09-18 D. N. Poenaru , R. A. Gherghescu , A. V. Solov'yov , W. Greiner

Carbon foams are hypothetical carbon allotropes that contain graphite-like (sp$^2$ carbon) segments, connected by sp$^3$ carbon atoms, resulting in porous structures. In this work the DFTB (Density Functional based Tight-Binding) method…

Materials Science · Physics 2013-02-15 Gotthard Seifert , Agnieszka Kuc , Thomas Heine

Compositional effects in NaK alloy clusters have been studied using bond order length strength notation and density functional theory calculations. The results reveal binding energy shifts of the NaK alloy clusters under different elemental…

Materials Science · Physics 2019-08-08 Jing Zhao , Maolin Bo

Based on first principles calculation, the electronic properties of graphene on metal (Ti, Ca, Ni, Mn, Co, Fe, Cr, K) modified SiO2 substrate have been studied. The results of binding energies supported graphene indicate that the metal…

Mesoscale and Nanoscale Physics · Physics 2012-03-02 L. Shen , F. Jiang , M. Xiao , R. Zhang , M. X. Yu , L. Miao , J. J. Jiang

At ambient pressure, sodium, chlorine, and their only known compound NaCl, have well-understood crystal structures and chemical bonding. Sodium is a nearly-free-electron metal with the bcc structure. Chlorine is a molecular crystal,…

We present density functional theory (DFT) calculations for 6H-SiC$\{0001\}$ surfaces with different surface stackings and terminations. We compare the relative stability of different $(0001)$ and $(000\bar1)$ surfaces in terms of their…

Materials Science · Physics 2011-02-11 Jochen Rohrer , Eleni Ziambaras , Per Hyldgaard

We study the atomic oxygen adsorption on Pb(111) surface by using density-functional theory within the generalized gradient approximation and a supercell approach. The atomic and energetic properties of purely on-surface and subsurface…

Materials Science · Physics 2009-11-13 Bo Sun , Ping Zhang , Zhigang Wang , Suqing Duan , Xian-Geng Zhao , Xuchun Ma , Qi-Kun Xue

Stable and metastable metallic nanoparticles exhibit unique properties compared to the bulk, with potentially important applications for catalysis. This is in particular the case for the AgPt alloy that can exhibit the ordered L1$_1$…

Materials Science · Physics 2023-07-11 F. Ait Hellal , J. Puibasset , C. Andreazza-Vignolle , P. Andreazza

Likely candidates for the global potential energy minima of (H$_{2}$O)$_{n}$ clusters with $n\leq21$ on the (0001)-surface of graphite are found using basin-hopping global optimization. The potential energy surfaces are constructed using…

Atomic and Molecular Clusters · Physics 2007-10-10 B. S. Gonzalez , J. Hernandez-Rojas , J. Breton , J. M. Gomez Llorente

Two-dimensional materials composed of transition metal carbides and nitrides (MXenes) are poised to revolutionize energy conversion and storage. In this work, we used density functional theory (DFT) to investigate adsorption of Mg and Na…

Materials Science · Physics 2021-12-01 G. Chaney , D. Çakır , F. M. Peeters , C. Ataca