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Short-range corrections to long-range selected configuration interaction calculations are derived from perturbation theory considerations and applied to harmonium (with two to six electrons for some low-lying states). No fitting to…

Chemical Physics · Physics 2024-07-19 Anthony Scemama , Andreas Savin

We present a review of recent works devoted to the variation of the fine structure constant alpha, strong interaction and fundamental masses. There are some hints for the variation in quasar absorption spectra, Big Bang nucleosynthesis, and…

Atomic Physics · Physics 2009-08-18 V. V. Flambaum

We perform ab initio calculations of isotope shifts for isotopes of cesium (from A=123 to A=137) and francium (from A=207 to A=228). These calculations start from the relativistic Hartree-Fock method and make use of several techniques to…

Atomic Physics · Physics 2009-11-11 V. A. Dzuba , W. R. Johnson , M. S. Safronova

A systematic study of energy spectra throughout the rare-earth region (even-even nuclei from $_{58}$Ce to $_{74}$W) is carried out in the framework of the interacting boson model (IBM), leading to an accurate description of the…

Nuclear Theory · Physics 2012-04-06 S. Zerguine , P. Van Isacker , A. Bouldjedri

Background: Atomic spectral lines from different isotopes display a small shift in energy, commonly referred to as the line isotope shift. One of the components of the isotope shift is the field shift, which depends on the extent and the…

Atomic Physics · Physics 2016-11-03 A. Papoulia , B. G. Carlsson , J. Ekman

Alchemical transformations showed that perturbation theory can be applied also to changes in the atomic nuclear charges of a molecule. The alchemical path that connects two different chemical species involves the conceptualization of a…

Chemical Physics · Physics 2024-03-27 Giorgio Domenichini

Relativistic configuration-interaction calculations have been performed for the energy levels of the low-lying and core-excited states of beryllium-like argon, Ar$^{14+}$. These calculations include the one-loop QED effects as obtained by…

Atomic Physics · Physics 2015-09-30 V. A. Yerokhin , A. Surzhykov , S. Fritzsche

Even when starting with a very poor initial guess, the iterative configuration interaction (iCI) approach can converge from above to full CI very quickly by constructing and diagonalizing a small Hamiltonian matrix at each…

Chemical Physics · Physics 2020-01-07 Ning Zhang , Wenjian Liu , Mark R. Hoffmann

Vibrational energy transfer of the amide I mode of N-methylacetamide (NMA) is studied theoretically using the vibrational configuration interaction method. A quartic force field of NMA is constructed at the B3LYP/6-31G+(d) level of theory…

Biomolecules · Quantitative Biology 2009-11-13 Hiroshi Fujisaki , Kiyoshi Yagi , Kimihiko Hirao , John E. Straub

We calculate excitation energies for low states of nobelium, including states with open $5f$ subshell. An efficient version of the many-electron configuration-interaction method for treating the atom as a sixteen external electrons system…

Atomic Physics · Physics 2019-03-13 V. A. Dzuba , V. V. Flambaum , M. G. Kozlov

Relativistic Hartree-Fock method together with many-body perturbation theory and configuration interaction techniques are used to calculate relativistic energy shifts for frequencies of the strong electric dipole transitions of C III, C IV,…

Atomic Physics · Physics 2007-10-26 I. M. Savukov , V. A. Dzuba

We predict the strong enhancement in the photoabsorption of small Mg clusters in the region of 4-5 eV due to the resonant excitation of the plasmon oscillations of cluster electrons. The photoabsorption spectra for neutral Mg clusters…

Atomic and Molecular Clusters · Physics 2007-05-23 Ilia A. Solovyov , Andrey V. Solovyov , Walter Greiner

The theory of phase transitions is based on the consideration of "idealized" models, such as the Ising model: a system of magnetic moments living on a cubic lattice and having only two accessible states. For simplicity the interaction is…

Statistical Mechanics · Physics 2011-12-22 H Chamati , S Romano

The shift in chemical equilibria due to isotope substitution is often exploited to gain insight into a wide variety of chemical and physical processes. It is a purely quantum mechanical effect, which can be computed exactly using…

Statistical Mechanics · Physics 2014-07-04 Michele Ceriotti , Thomas E. Markland

The reaction dynamics of axisymmetric deformed $^{24}$Mg + $^{24}$Mg collisions have been investigated systematically by an isospin-dependent quantum molecular dynamics (IDQMD) model. It is found that different deformations and orientations…

Nuclear Theory · Physics 2014-11-21 X. G. Cao , G. Q. Zhang , X. Z. Cai , Y. G. Ma , W. Guo , J. G. Chen , W. D. Tian , D. Q. Fang , H. W. Wang

We calculate the light-induced collisional loss of laser-cooled and trapped magnesium atoms for detunings up to 50 atomic linewidths to the red of the ^1S_0-^1P_1 cooling transition. We evaluate loss rate coefficients due to both radiative…

Atomic Physics · Physics 2009-11-07 M. Machholm , Paul S. Julienne , K. -A. Suominen

We study the electron correlation effects in the calculations of isotope shifts in Na and Mg+ using the relativistic coupled-cluster method. The trends of the correlation effects are explicitly discussed and comparison of the present…

Atomic Physics · Physics 2010-07-29 B. K. Sahoo

We calculate the shift, due to interatomic interactions, of an optical transition in an atomic Fermi gas trapped in an optical lattice, as in recent experiments of Campbell {\it et al.}, Science {\bf 324}, 360 (2009). Using a pseudospin…

Quantum Gases · Physics 2010-01-11 Zhenhua Yu , C. J. Pethick

We perform accurate calculations of the dependence of transition frequencies in two valence electron atoms and ions on a variation of the fine structure constant, alpha. The relativistic Hartree-Fock method is used with many-body…

Atomic Physics · Physics 2009-02-05 E. J. Angstmann , V. A. Dzuba , V. V. Flambaum

Theories unifying gravity with other interactions suggest spatial and temporal variation of fundamental ``constants'' in the Universe. A change in the fine structure constant, alpha, could be detected via shifts in the frequencies of atomic…