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Related papers: Nonlinear interferometric vibrational imaging

200 papers

Far field radiation pattern under tight focusing condition is investigated in Coherent Anti-stokes Raman Scattering (CARS) microscopy both in the forward (F-CARS) and backward (E-CARS) directions. While we assume no refraction index…

Optics · Physics 2009-11-11 D. Gachet , N. Sandeau , H. Rigneault

Currently, a large number of stored tissue samples are unavailable for spectroscopic study without the time consuming and destructive process of paraffin removal. Instead, a structurally sensitive technique, sum frequency generation, and a…

Medical Physics · Physics 2023-10-03 Bryan Semon , Michael Jaffe , Haifeng Wang , Lauren Priddy , Gombojav Ariunbold

Coherent Raman scattering (CRS) spectroscopy techniques have been widely developed and optimized for different applications in biomedicine and fundamental science. The most utilized CRS technique has been coherent anti-Stokes Raman…

Optics · Physics 2020-03-05 Pavel Kolesnichenko , Jonathan O. Tollerud , Jeffrey A. Davis

The success of non-linear optics relies largely on pulse-to-pulse consistency. In contrast, covariance based techniques used in photoionization electron spectroscopy and mass spectrometry have shown that wealth of information can be…

We describe a new optical diagnostic for determining the composition of gases by measuring the motion of atoms and molecules trapped within very deep optical lattices. This non-resonant method is analogous to conventional Raman scattering,…

Optics · Physics 2022-01-19 A. Gerakis , M. N. Shneider , P. F. Barker

We use a Langevin approach to analyze the quantum noise in Coherent Anti-Stokes Raman Spectroscopy (CARS) in several experimental scenarios: with continuous wave input fields acting simultaneously and with fast sequential pulsed lasers…

Statistical Mechanics · Physics 2009-11-10 Kunal K. Das , G. S. Agarwal , Yu. M. Golubev , M. O. Scully

We propose a full-vectorial numerical study of far field radiation patterns in coherent anti-Stokes Raman scattering (CARS) microscopy. We emphasis the particular role of the Raman depolarisation ratio of the observed medium and show how it…

Optics · Physics 2009-11-13 D. Gachet , N. Sandeau , H. Rigneault

Conventional femtosecond coherent laser spectroscopy predominantly focuses on the temporal phase coherence through time- or frequency-resolved methods. In this work, we suggest an alternative experimental framework based on spatial phase…

Coherent anti-Stokes Raman scattering (CARS) and, in particular, femtosecond adaptive spectroscopic techniques (FAST CARS) have been successfully used for molecular spectroscopy and microscopic imaging. Recent progress in ultrafast…

In Impulsive Stimulated Raman Scattering vibrational oscillations, coherently stimulated by a femtosecond Raman pulse, are real time monitored and read out as intensity modulations in the transmission of a temporally delayed probe pulse.…

Chemical Physics · Physics 2019-11-28 Giovanni Batignani , Carino Ferrante , Giuseppe Fumero , Tullio Scopigno

The key challenge of time-resolved Raman spectroscopy is the identification of the constituent species and the analysis of the kinetics of the underlying reaction network. In this work we present an integral approach that allows for…

Numerical Analysis · Mathematics 2017-09-15 Robert Luce , Peter Hildebrandt , Uwe Kuhlmann , Jörg Liesen

Early theoretical works on coherent anti-Stokes Raman scattering in optically active medium consider only heterodyne signal and subsequently, fourth- and fifth-rank tensor averages have been used. In this work, we presented a full signal…

Quantum Physics · Physics 2019-01-03 Tuguldur Kh. Begzjav , Marlan O. Scully , Girish S. Agarwal

We apply coherent anti-Stokes Raman Scattering (CARS) microscopy to characterize director structures in liquid crystals.

Soft Condensed Matter · Physics 2016-09-08 A. V. Kachynski , A. N. Kuzmin , P. N. Prasad , I. I. Smalyukh

This study presents a nonlinear signal processing method for accurate radar-based heartbeat interval estimation by exploiting the periodicity of higher-order harmonics inherent in heartbeat signals. Unlike conventional approaches that…

Signal Processing · Electrical Eng. & Systems 2025-07-29 Kohei Shimomura , Chi-Hsuan Lee , Takuya Sakamoto

We demonstrate the acquisition of stimulated Raman scattering spectra with the use of a single femtosecond pulse. High resolution vibrational spectra are obtained by shifting the phase of a narrow band of frequencies in the broadband input…

Optics · Physics 2015-05-20 Hadas Frostig , Ori Katz , Adi Natan , Yaron Silberberg

Removing distortions in coherent anti-Stokes Raman scattering (CARS) spectra due to interference with the nonresonant background (NRB) is vital for quantitative analysis. Popular computational approaches, the Kramers-Kronig relation and the…

Signal Processing · Electrical Eng. & Systems 2022-07-08 Charles H. Camp

To avoid decorrelation, conventional synthetic aperture radar interferometry (InSAR) requires that interferometric images should have a common spectral band and the same resolution after proper preprocessing. For a high-resolution (HR)…

Signal Processing · Electrical Eng. & Systems 2020-10-15 Huizhang Yang , Chengzhi Chen , Shengyao Chen , Feng Xi , Zhong Liu

High-gain resonant nonlinear Raman scattering on trapped cold atoms within a high-fineness ring optical cavity is simply explained under a nonlinear opto-mechanical mechanism, and a proposal using it to detect frequency of micro-trap on…

Atomic Physics · Physics 2014-03-24 Lin Zhang

The ability to enhance resonant signals and eliminate the non-resonant background is analyzed for Coherent Anti-Stokes Raman Scattering (CARS). The analysis is done at a specific frequency as well as for broadband excitation using…

Quantum Physics · Physics 2015-03-19 Fang Gao , Feng Shuang , JunHui Shi , Herschel Rabitz , HaiFeng Wang , JiXin Cheng

We resolve the real-time electric field of a femtosecond third-order nonlinear optical signal in the molecular frame. The electric field emitted by the induced third-order polarization from impulsively pre-aligned gas-phase molecules at…