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Raman scattering experiments on stoichiometric, Mott-insulating LaTiO$_3$ over a wide range of excitation energies reveal a broad electronic continuum which is featureless in the paramagnetic state, but develops a gap of $\sim 800$…

Strongly Correlated Electrons · Physics 2015-10-28 C. Ulrich , G. Khaliullin , M. Guennou , H. Roth , T. Lorenz , B. Keimer

We determine the nature of coupled phonons and magnetic excitations in AlFeO3 using inelastic light scattering from 5 K to 315 K covering a spectral range from 100-2200 cm-1 and complementary first-principles density functional theory-based…

Strongly Correlated Electrons · Physics 2012-05-01 Pradeep Kumar , A. Bera , D. V. S. Muthu , S. N. Shirodkar , R. Saha , A. Shireen , A. Sundaresan , U. V. Waghmare , A. K. Sood , C. N. R. Rao

We have performed Raman scattering investigations on the high energy magnetic excitations in a BiFeO$_3$ single crystal as a function of both temperature and laser excitation energy. A strong feature observed at 1250 cm$^{-1}$ in the Raman…

Strongly Correlated Electrons · Physics 2018-11-13 M. Cazayous , A. Sacuto , D. Lebeugle , D. Colson

The polarized Raman spectra of layered ruthenates of the Srn+1RunO3n+1 (n=1,2,3) Ruddlesden-Popper series were measured between 10 and 300 K. The phonon spectra of Sr3Ru2O7 and Sr4Ru3O10 confirmed earlier reports for correlated rotations of…

Materials Science · Physics 2009-11-10 M. N. Iliev , V. N. Popov , A. P. Litvinchuk , M. V. Abrashev , J. Backstrom , Y. Y. Sun , R. L. Meng , C. W. Chu

Temperature-dependent Raman spectra of TbMnO$_3$ from 5 K to 300 K in the spectral range of 200 to 1525 cm$^{-1}$ show five first-order Raman allowed modes and two high frequency modes. The intensity ratio of the high frequency Raman band…

Strongly Correlated Electrons · Physics 2010-04-12 Pradeep Kumar , Surajit Saha , D. V. S. Muthu , J. R. Sahu , A. K. Sood , C. N. R. Rao

Polarized Raman scattering and infrared reflection spectra of hexagonal HoMnO$_3$ single crystals in the temperature range 10-300 K are reported. Group-theoretical analysis is performed and scattering selection rules for the second order…

Strongly Correlated Electrons · Physics 2009-11-10 A. P. Litvinchuk , M. N. Iliev , V. N. Popov , M. M. Gospodinov

We have performed polarized Raman scattering measurements on the newly discovered superconductor Ta$_{4}$Pd$_{3}$Te$_{16}$ ($T_c = 4.6$ K). We observe twenty-eight out of thirty-three Raman active modes, with frequencies in good accordance…

Superconductivity · Physics 2015-11-25 D. Chen , P. Richard , Z. -D. Song , W. -L. Zhang , S. -F. Wu , W. H. Jiao , Z. Fang , G. -H. Cao , H. Ding

The Raman-active phonons in perovskite-like LaMn1-xCoxO3 (x = 0, 0.2, 0.3, 0.4, and 1.0) were studied by measuring Raman spectra at temperatures of 295 and 5 K. The changes in the spectra with Co doping are correlated with the decrease of…

Strongly Correlated Electrons · Physics 2007-05-23 V. P. Gnezdilov , Yu. G. Pashkevich , A. V. Yeremenko , P. Lemmens , G. Guentherodt , S. V. Shiryaev , G. L. Bychkov , S. N. Barilo

We have used polarized Raman scattering to probe lattice vibrations and charge ordering in 12 nm thick, epitaxially strained PrNiO$_3$ films, and in superlattices of PrNiO$_3$ with the band-insulator PrAlO$_3$. A carefully adjusted confocal…

Strongly Correlated Electrons · Physics 2015-06-23 M. Hepting , M. Minola , A. Frano , G. Cristiani , G. Logvenov , E. Schierle , M. Wu , M. Bluschke , E. Weschke , H. U. Habermeier , E. Benckiser , M. Le Tacon , B. Keimer

We report an investigation of perovskite-type LaNiO3 thin films by Raman scattering in both various scattering configurations and as a function of temperature. The room-temperature Raman spectra and the associated phonon mode assignment…

Materials Science · Physics 2010-07-30 N. Chaban , M. Weber , S. Pignard , J. Kreisel

We report inelastic neutron scattering measurements over 7-1251 K in CaMnO3 covering various phase transitions, and over 6-150 K in PrMnO3 covering the magnetic transition. The excitations around 20 meV in CaMnO3 and at 17 meV in PrMnO3 are…

Materials Science · Physics 2016-06-29 S. K. Mishra , M. K. Gupta , R. Mittal , A. I. Kolesnikov , S. L. Chaplot

We have used Raman scattering to investigate the magnetic excitations and lattice dynamics in the prototypical spin-orbit Mott insulators Sr2IrO4 and Sr3Ir2O7. Both compounds exhibit pronounced two-magnon Raman scattering features with…

Strongly Correlated Electrons · Physics 2016-04-06 H. Gretarsson , N. H. Sung , M. Hoeppner , B. J. Kim , B. Keimer , M. Le Tacon

The Raman spectra of CaFe2O4 were measured with several exact scattering configurations between 20 and 520K and the symmetry of all observed Raman lines was determined. The Ag and B2g lines were assigned to definite phonon modes by…

Materials Science · Physics 2009-11-10 N. Kolev , M. N. Iliev , V. N. Popov , M. Gospodinov

Raman scattering is used to observe pronounced electronic excitations around 230 meV - well above the two-phonon range - in the Mott insulators LaTiO$_3$ and YTiO$_3$. Based on the temperature, polarization, and photon energy dependence,…

Strongly Correlated Electrons · Physics 2007-05-23 C. Ulrich , A. Gössling , M. Grüninger , M. Guennou , H. Roth , M. Cwik , T. Lorenz , G. Khaliullin , B. Keimer

Polarized Raman scattering measurements have been performed on Na0.5CoO2 single crystal from 8 to 305 K. Both the A1g and E1g phonon modes show a softening below Tc1 ~ 83 K. Additionally, the A1g phonon mode, which is forbidden in the…

Strongly Correlated Electrons · Physics 2008-02-07 Q. M. Zhang , M. an , S. K. Yuan , Y. Wu , D. Wu , J. L. Luo , N. L. Wang , W. Bao , Y. N. Wang

We report inelastic light scattering studies on Ca(Fe0.97Co0.03)2As2 in a wide spectral range of 120-5200 cm-1 from 5K to 300K, covering the tetragonal to orthorhombic structural transition as well as magnetic transition at Tsm ~ 160K. The…

Superconductivity · Physics 2014-07-11 Pradeep Kumar , D. V. S. Muthu , L. Harnagea , S. Wurmehl , B. Büchner , A. K. Sood

We report inelastic light scattering experiments on CaFe_2As_2 in the temperature range of 4 to 290 K. In in-plane polarizations two Raman-active phonon modes are observed at 189 and 211 cm-1, displaying A_1g and B_1g symmetries,…

Superconductivity · Physics 2009-11-13 K. -Y. Choi , D. Wulferding , P. Lemmens , N. Ni , S. L. Bud'ko , P. C. Canfield

In this study, we present a comprehensive analysis of the Raman active phonon modes in orthorhombic LaInO$_3$ based on a combination of polarization-angle resolved Raman spectroscopy and density functional theory calculations. By using…

The novel ferroelectric-like structural transition observed in metallic LiOsO$_3$ [Y. Shi et al., Nat. Mater. 12, 1024 (2013)], has invoked many theoretical and experimental interests. In this work, we have performed polarized and…

Materials Science · Physics 2017-03-09 Feng Jin , Anmin Zhang , Jianting Ji , Kai Liu , Le Wang , Youguo Shi , Yong Tian , Xiaoli Ma , Qingming Zhang

The origin of the low-temperature ferromagnetic instability in YTiO3 driven by the interplay between lattice, orbital, spin, and charge degrees of freedom is on the background of lattice dynamics. We present a comprehensive study of…

Strongly Correlated Electrons · Physics 2022-02-16 N. N. Kovaleva , O. E. Kusmartseva , A. Maljuk
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