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The electron dynamics of rare gas clusters in laser fields is investigated quantum mechanically by means of time-dependent density functional theory. The mechanism of early inner and outer ionization is revealed. The formation of an…

Atomic Physics · Physics 2009-11-10 D. Bauer , A. Macchi

A detailed theoretical investigation of rare gas atom clusters under intense short laser pulses reveals that the mechanism of energy absorption is akin to {\it enhanced ionization} first discovered for diatomic molecules. The phenomenon is…

Atomic and Molecular Clusters · Physics 2009-11-07 Christian Siedschlag , Jan-Michael Rost

It is known that rare-gas or metal clusters absorb incident laser energy very efficiently. However, due to the intricate dependencies on all the laser and cluster parameters it is difficult to predict under which circumstances ionization…

Plasma Physics · Physics 2009-11-13 M. Kundu , D. Bauer

The interaction of short laser pulses with small rare gas clusters is investigated by using a microscopic, semi-classical model with an explicit treatment of the inner-atomic dynamics. Field and collisional ionisation as well as…

Atomic and Molecular Clusters · Physics 2007-05-23 D. Bauer

Semi-classical molecular dynamics simulations of small rare gas clusters in short laser pulses of 100 nm wavelength were performed. For comparison, the cluster response to 800 nm laser pulses was investigated as well. The inner ionization…

Atomic and Molecular Clusters · Physics 2009-11-10 D. Bauer

The dynamics of molecular electron excitation and ionisation is studied in real-time for ultra-short IR laser pulses of intensity I>10^{13} W/cm^{2}. The multi-electron molecule is modeled by a system of two active electrons moving in a…

Optics · Physics 2015-06-26 A. I. Pegarkov

We analyze the dynamics of up to $10^5$ electrons resulting from illuminating a Xenon cluster with 9093 atoms with intense laser pulses of different length and peak intensity. Interesting details of electron motion are identified which can…

Atomic and Molecular Clusters · Physics 2007-05-23 Ulf Saalmann , Jan M. Rost

Intense, ultrashort pulses of 800 nm laser light (12 fs, $\sim$4 optical cycles) of peak intensity 5$\times$10$^{14}$ W cm$^{-2}$ have been used to irradiate gas-phase Xe$_n$ clusters ($n$=500-25,000) so as to induce multiple ionization and…

Atomic and Molecular Clusters · Physics 2015-05-19 D. Mathur , F. A. Rajgara

The effect of intense X-ray laser interaction on argon clusters is studied theoretically with a mixed quantum/classical approach. In comparison to a single atom we find that ionization of the cluster is suppressed, which is in striking…

Atomic and Molecular Clusters · Physics 2009-11-07 Ulf Saalmann , Jan M Rost

The interaction of intense laser pulses with nano-scale particles leads to the production of high-energy electrons, ions, neutral atoms, neutrons and photons. Up to now, investigations have focused on near-infrared to X-ray laser pulses…

Calculating the energy absorption of atomic clusters as a function of the laser pulse length $T$ we find a maximum for a critical $T^*$. We show that $T^*$ can be linked to an optimal cluster radius $R^*$. The existence of this radius can…

Atomic and Molecular Clusters · Physics 2009-11-07 Christian Siedschlag , Jan M. Rost

The harmonic emission from cluster nanoplasmas subject to short, intense infrared laser pulses is analyzed by means of particle-in-cell simulations. A pronounced resonant enhancement of the low-order harmonic yields is found when the Mie…

Plasma Physics · Physics 2009-11-13 M. Kundu , S. V. Popruzhenko , D. Bauer

The ionization dynamics of a Xenon cluster with 40 atoms is analyzed under a pum p probe scenario of laser pulses where an infrared laser pulse of 50 fs length follows with a well defined time delay a VUV pulse of the same length and peak…

Atomic and Molecular Clusters · Physics 2009-11-10 Ch. Siedschlag , J. M. Rost

The process of ionization of a hydrogen atom by a short infrared laser pulse is studied in the regime of very large pulse intensity, in the dipole approximation. Let $A$ denote the integral of the electric field of the pulse over time at…

Mathematical Physics · Physics 2015-05-18 Juerg Froehlich , Alessandro Pizzo , Benjamin Schlein

The interaction of intense extreme ultraviolet (XUV) laser pulses ($\lambda=32\rm\,nm$, $I=10^{11-14}$\,W/cm$^2$) with small rare-gas clusters (Ar$_{147}$) is studied by quasi-classical molecular dynamics simulations. Our analysis supports…

Atomic and Molecular Clusters · Physics 2010-09-01 Mathias Arbeiter , Thomas Fennel

Non-equilibrium processes following the irradiation of atomic clusters with short pulses of vacuum ultraviolet radiation are modelled using kinetic Boltzmann equations. The dependence of the ionization dynamics on the cluster size is…

Plasma Physics · Physics 2009-11-13 B. Ziaja , H. Wabnitz , E. Weckert , T. Möller

We study the dynamics of atomic and molecular nano-clusters exposed to short and intense X-fel pulses

Atomic and Molecular Clusters · Physics 2015-10-02 Pierfrancesco Di Cintio

Intense 3-cycle pulses (10 fs) of 800 nm laser light are utilized to measure energy distributions of ions emitted following Coulomb explosion of Ar$_n$ clusters ($n$=400-900) upon their irradiation by peak intensitis of 5$\times$10$^{14}$ W…

Atomic and Molecular Clusters · Physics 2010-05-21 D. Mathur , F. A. Rajgara , A. R. Holkundkar , N. K. Gupta

In this paper we examine the behavior of small cluster of atoms in a short (10-50 fs) very intense hard x-ray (10 keV) pulse. We use numerical modeling based on the non-relativistic classical equation of motion. Quantum processes are taken…

Atomic and Molecular Clusters · Physics 2009-11-10 Zoltan Jurek , Gyula Faigel , Miklos Tegze

The interaction of relativistically strong tailored laser pulses with an atomic system is considered. Due to a special tailoring of the laser pulse, the suppression of the relativistic drift of the ionized electron and a dramatic…

Atomic Physics · Physics 2009-11-13 Michael Klaiber , Karen Z. Hatsagortsyan , Christoph H. Keitel
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