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Related papers: Production of Ultracold, Polar RbCs* Molecules via…

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We develop the theory for the Adiabatic Raman Photoassociation (ARPA) of ultracold atoms to form ultracold molecules in the presence of scattering resonances. Based on a computational method in which we replace the continuum with a discrete…

Atomic Physics · Physics 2012-11-27 Alex C. Han , Evgeny A. Shapiro , Moshe Shapiro

We report continuous direct photoassociative formation of ultracold KRb molecules in the lowest vibrational levels $(v"=0 -10)$ of the electronic ground state $(X ^1\Sigma^+)$, starting from $^{39}$K and $^{85}$Rb atoms in a magneto-optical…

We consider the formation of cold ground-state polar molecules in a low vibrational level by laser fields. Starting from a pair of cold colliding atoms of dissimilar species, we propose a strategy consisting of three steps. In the first…

Atomic Physics · Physics 2026-01-14 Emanuel F. de Lima

Two-color photoassociation of ground state $^6$Li$^{87}$Rb molecules via the $\mathrm{B}^1\Pi$ electronic state using short pulses near a magnetic Feshbach resonance is studied theoretically. A near-resonant magnetic field is applied to mix…

Atomic Physics · Physics 2014-02-04 Marko Gacesa , Subhas Ghosal , Jason Byrd , Robin Côté

We report the production of ultracold RbCs molecules in the rovibronic ground state, i.e., $X^1\Sigma^+ (v=0, J=0)$, by short-range photoassociation to the $2^3\Pi_{0}$ state followed by spontaneous emission. We use narrowband depletion…

Atomic Physics · Physics 2015-06-22 Toshihiko Shimasaki , Michael Bellos , C. D. Bruzewicz , Zack Lasner , David DeMille

We report on the creation of heterospecies bosonic molecules, associated from an ultracold Bose-Bose mixture of 41K and 87Rb, by using a resonantly modulated magnetic field close to two Feshbach resonances. We measure the binding energy of…

Other Condensed Matter · Physics 2009-01-29 C. Weber , G. Barontini , J. Catani , G. Thalhammer , M. Inguscio , F. Minardi

Heteronuclear alkali-metal dimers represent the class of molecules of choice for creating samples of ultracold molecules exhibiting an intrinsic large permanent electric dipole moment. Among them, the KCs molecule, with a permanent dipole…

Atomic Physics · Physics 2015-04-08 D. Borsalino , R. Vexiau , M. Aymar , E. Luc-Koenig , O. Dulieu , N. Bouloufa-Maafa

We report the formation of ultracold $^{7}$Li$^{85}$Rb molecules in the $a^{3}\Sigma^{+}$ electronic state by photoassociation (PA) and their detection via resonantly enhanced multiphoton ionization (REMPI). With our dual-species Li and Rb…

Atomic Physics · Physics 2015-06-22 Adeel Altaf , Sourav Dutta , John Lorenz , Jesús Pérez-Ríos , Yong P. Chen , D. S. Elliott

We produce an ultracold and dense sample of rovibronic ground state Cs_2 molecules close to the regime of quantum degeneracy, in a single hyperfine level, in the presence of an optical lattice. The molecules are individually trapped, in the…

Ultracold ground-state molecules can be formed from ultracold atoms via photoassociation followed by a spontaneous emission process. Typically, the molecular products are distributed over a range of final states. Here, we propose to use an…

Quantum Physics · Physics 2018-12-20 Tobias Kampschulte , Johannes Hecker Denschlag

We report on the production of ultracold heteronuclear YbLi* molecules in a dual-species magneto-optical trap by photoassociation (PA). The formation of the electronically excited molecules close to dissociation was observed by trap loss…

The creation of ultracold molecules is currently limited to diatomic species. In this letter we present a theoretical description of the photoassociation of ultracold atoms and molecules to create ultracold excited triatomic molecules, thus…

Atomic Physics · Physics 2015-09-02 Jesús Pérez-Ríos , Maxence Lepers , Olivier Dulieu

We report the creation and characterization of a near quantum-degenerate gas of polar $^{40}$K-$^{87}$Rb molecules in their absolute rovibrational ground state. Starting from weakly bound heteronuclear KRb Feshbach molecules, we implement…

Utilizing single-photon photoassociation, we have achieved ultracold rubidium molecules with a high number density that provides a new efficient approach toward molecular quantum degeneracy. A new detection mechanism for ultracold molecule…

Atomic Physics · Physics 2015-06-12 Jun-Ren Chen , Cheng-Yang Kao , Hung-Bin Chen , Yi-Wei Liu

State-of-the-art {\em ab initio} techniques have been applied to compute the potential energy curves for the SrYb molecule in the Born-Oppenheimer approximation for the ground state and first fifteen excited singlet and triplet states…

Photoassociation (PA) is a powerful technique to synthesize molecules directly and continuously from cold and ultracold atoms into deeply bound molecular states. In freespace, however, PA efficiency is constrained by the number of…

Atomic Physics · Physics 2018-01-17 J. Pérez-Ríos , May E. Kim , Chen-Lung Hung

The paper investigates cold molecules formation in the photoassociation of two cold atoms by a strong laser pulse applied at short interatomic distances, which lead to a molecular dynamics taking place in the light-induced (adiabatic)…

Quantum Physics · Physics 2009-07-23 M. Vatasescu

This theoretical paper investigates the formation of ground state molecules from ultracold cesium atoms in a two-color scheme. Following previous work on photoassociation with chirped picosecond pulses [Luc-Koenig et al., Phys. Rev. A {\bf…

Atomic Physics · Physics 2007-05-23 Christiane P. Koch , Eliane Luc-Koenig , Françoise Masnou-Seeuws

Recently, the quest for an ultracold and dense ensemble of polar molecules has attracted strong interest. Polar molecules have bright prospects for novel quantum gases with long-range and anisotropic interactions, for quantum information…

The generation of cold molecules is a core topic in the field of cold atoms and molecules, which has advanced relevant research like ultracold chemistry, quantum computation, and quantum metrology. With high atomic phase space density,…

Atomic Physics · Physics 2024-02-27 Li Li , Yi-Jia Liu , Xiao-Long Zhou , Ze-Min Shen , Si-Jian He , Zhao-Di Liu , Jian Wang