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In this paper we motivate, formulate and analyze the Multi-Configuration Time-Dependent Hartree-Fock (MCTDHF) equations for molecular systems under Coulomb interaction. They consist in approximating the N-particle Schrodinger wavefunction…

Mathematical Physics · Physics 2015-05-13 C. Bardos , I. Catto , N. Mauser , S. Trabelsi

Basis set convergence of the Hartree-Fock and the correlation energy is examined for the hydrogen bonded infinite bent chains (HF)_infinity and (HCl)_infinity. We employ series of correlation consistent basis sets up to quintuple zeta…

Other Condensed Matter · Physics 2007-05-23 Christian Buth , Beate Paulus

Ground state energies and decay widths of particle unstable nuclei are calculated within the Hartree-Fock approximation by performing a complex scaling of the many-body Hamiltonian. Through this transformation, the wave functions of the…

Nuclear Theory · Physics 2009-01-23 A. T. Kruppa , P. -H. Heenen , H. Flocard , R. J. Liotta

In this article, mixed finite element methods are discussed for a class of hyperbolic integro-differential equations (HIDEs). Based on a modification of the nonstandard energy formulation of Baker, both semidiscrete and completely discrete…

Numerical Analysis · Mathematics 2014-01-22 Samir Karaa , Amiya K. Pani

In the near future, material and drug design may be aided by quantum computer assisted simulations. These have the potential to target chemical systems intractable by the most powerful classical computers. However, the resources offered by…

The self-consistent field method utilized for solving the Hartree-Fock (HF) problem and the closely related Kohn-Sham problem, is typically thought of as one of the cheapest methods available to quantum chemists. This intuition has been…

Quantum Physics · Physics 2015-06-22 James D. Whitfield , Zoltán Zimborás

We have developed a couple of optimal damping algorithms (ODAs) for unrestricted Hartree-Fock (UHF) calculations of open-shell molecular systems. A series of equations were derived for both concurrent and alternate constructions of alpha-…

Chemical Physics · Physics 2018-01-25 Jun-ichi Yamamoto , Yuji Mochizuki

In this article, we discuss how a kind of hybrid computation, which employs symbolic, numeric, classic, and quantum algorithms, allows us to conduct Hartree-Fock electronic structure computation of molecules. In the proposed algorithm, we…

Quantum Physics · Physics 2024-06-19 Ichio Kikuchi , Akihito Kikuchi

We describe a method of solving the nuclear Skyrme-Hartree-Fock problem by using a deformed Cartesian harmonic oscillator basis. The complete list of expressions required to calculate local densities, total energy, and self-consistent…

Nuclear Theory · Physics 2009-10-30 J. Dobaczewski , J. Dudek

We devise a Hybrid High-Order (HHO) method for highly oscillatory elliptic problems that is capable of handling general meshes. The method hinges on discrete unknowns that are polynomials attached to the faces and cells of a coarse mesh;…

Numerical Analysis · Mathematics 2018-06-18 Matteo Cicuttin , Alexandre Ern , Simon Lemaire

High-precision calculations of the energy levels of the superheavy element Z=120 are presented. The relativistic Hartree-Fock and configuration interaction techniques are employed. The correlations between core and valence electrons are…

Atomic Physics · Physics 2022-01-07 T. H. Dinh , V. A. Dzuba , V. V. Flambaum , J. S. M. Ginges

An efficient nonlinear multigrid method for a mixed finite element method of the Darcy-Forchheimer model is constructed in this paper. A Peaceman-Rachford type iteration is used as a smoother to decouple the nonlinearity from the divergence…

Numerical Analysis · Mathematics 2017-04-27 Jian Huang , Long Chen , Hongxing Rui

This paper introduces and analyses the new grid-based tensor approach to approximate solution of the elliptic eigenvalue problem for the 3D lattice-structured systems. We consider the linearized Hartree-Fock equation over a spatial…

Numerical Analysis · Mathematics 2017-02-02 V. Khoromskaia , B. N. Khoromskij

We are interested in high-order linear multistep schemes for time discretization of adjoint equations arising within optimal control problems. First we consider optimal control problems for ordinary differential equations and show loss of…

Numerical Analysis · Mathematics 2018-07-24 Giacomo Albi , Michael Herty , Lorenzo Pareschi

In this paper, we present an interior penalty discontinuous Galerkin finite element scheme for solving diffusion problems with strong anisotropy arising in magnetized plasmas for fusion applications. We demonstrate the accuracy produced by…

Numerical Analysis · Mathematics 2022-05-18 David Green , Xiaozhe Hu , Jeremy Lore , Lin Mu , Mark L. Stowell

We solve Poisson's equation using new multigrid algorithms that converge rapidly. The novel feature of the 2D and 3D algorithms are the use of extra diagonal grids in the multigrid hierarchy for a much richer and effective communication…

Numerical Analysis · Mathematics 2025-10-20 A. J. Roberts

In this article, we present an interpolative separable density fitting (ISDF) based algorithm to calculate exact exchange in periodic mean field calculations. In the past, decomposing the two-electron integrals into tensor hypercontraction…

Chemical Physics · Physics 2024-04-16 Kori E. Smyser , Alec White , Sandeep Sharma

We propose a multigrid correction scheme to solve a new Steklov eigenvalue problem in inverse scattering. With this scheme, solving an eigenvalue problem in a fine finite element space is reduced to solve a series of boundary value problems…

Numerical Analysis · Mathematics 2018-06-18 Yu Zhang , Hai Bi , Yidu Yang

We perform Hartree-Fock+BCS calculations for even-even nuclei with 2 <= Z <= 82 and N ranging from outside the proton drip line to the experimental frontier on the neutron-rich side. The ground state solutions are obtained for 737 nuclei,…

Nuclear Theory · Physics 2009-10-28 N. Tajima , N. Onishi , S. Takahara

In order to study light unstable nuclei systematically, we propose a new method ''AMD + Hartree-Fock''. This method introduces the concept of the single particle orbits into the usual AMD. Applying AMD + HF to Be isotopes, it is found that…

Nuclear Theory · Physics 2007-05-23 A. Dote , H. Horiuchi , Y. Kanada-En'yo