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We present a new method which uses Feynman-like diagrams to calculate the statistical quantities of embedded many-body random matrix problems. The method provides a promising alternative to existing techniques and offers many important…

Statistical Mechanics · Physics 2014-08-06 Rupert Small , Sebastian Müller

The method of many-body Green's functions is developed for arbitrary systems of electrons and nuclei starting from the full (beyond Born-Oppenheimer) Hamiltonian of Coulomb interactions and kinetic energies. The theory presented here…

Other Condensed Matter · Physics 2020-06-23 Ville J. Härkönen , Robert van Leeuwen , E. K. U. Gross

Efficient characterization of highly entangled multi-particle systems is an outstanding challenge in quantum science. Recent developments have shown that a modest number of randomized measurements suffices to learn many properties of a…

Quantum Physics · Physics 2022-12-13 Katherine Van Kirk , Jordan Cotler , Hsin-Yuan Huang , Mikhail D. Lukin

In this article, we describe a recursive method to construct a subset of relevant Slater-determinants for the use in many-body diagonalization schemes that will be employed in our forthcoming papers on the simulation of excited many-body…

Other Condensed Matter · Physics 2007-05-23 K. M. Indlekofer , R. Németh

The quantum equation-of-motion (qEOM) method with singles and doubles has been suggested to study electronically excited states while it fails to predict the excitation energies dominated by double excitations. In this work, we present an…

Quantum Physics · Physics 2024-06-18 Yuhan Zheng , Jie Liu , Zhenyu Li , Jinlong Yang

A model-operator approach to fully relativistic calculations of the nuclear recoil effect on energy levels in many-electron atomic systems is worked out. The one-electron part of the model operator for treating the normal mass shift beyond…

We demonstrate that $V^{N-M}$ approximation is a good starting point for the configuration interaction calculations for many-electron atoms and ions. $N$ is the total number of electrons in the neutral atom, $M$ is the number of valence…

Atomic Physics · Physics 2009-11-11 V. A. Dzuba

Perturbation theory with respect to the kinetic energy of the heavy component of a two-component quantum system is introduced. An effective Hamiltonian that is accurate to second order in the inverse heavy mass is derived. It contains a new…

Quantum Physics · Physics 2024-06-21 Ryan Requist

From celestial mechanics to quantum theory of atoms and molecules, perturbation theory has played a central role in natural sciences. Particularly in quantum mechanics, the amount of information needed for specifying the state of a…

Quantum Physics · Physics 2016-07-06 Yudong Cao , Sabre Kais

In spite of missing dynamical correlations, the projected generator coordinate method (PGCM) was recently shown to be a suitable method to tackle the low-lying spectroscopy of complex nuclei. Still, describing absolute binding energies and…

We present a data-driven approach for the prediction of the electric dipole moment of diatomic molecules, which is one of the most relevant molecular properties. In particular, we apply Gaussian process regression to a novel dataset to show…

Chemical Physics · Physics 2020-12-02 Xiangyue Liu , Gerard Meijer , Jesús Pérez-Ríos

We study the accuracy of analytical wave function based many-body methods derived by energy minimization of a Jastrow-Feenberg ansatz for electrons (`Fermi hypernetted chain / Euler Lagrange' approach). Approximations to avoid the…

Other Condensed Matter · Physics 2019-06-05 Martin Panholzer , Raphael Hobbiger , Helga Böhm

We present an efficient \textit{ab initio} method for calculating the electronic structure and total energy of strongly correlated electron systems. The method extends the traditional Gutzwiller approximation for one-particle operators to…

Strongly Correlated Electrons · Physics 2014-07-01 Y. X. Yao , J. Liu , C. Liu , W. C. Lu , C. Z. Wang , K. M. Ho

Presenting systems of differential equations in the form of diagrams has become common in certain parts of physics, especially electromagnetism and computational physics. In this work, we aim to put such use of diagrams on a firm…

Mathematical Physics · Physics 2022-06-20 Evan Patterson , Andrew Baas , Timothy Hosgood , James Fairbanks

We present a variational Monte Carlo algorithm for estimating the lowest excited states of a quantum system which is a natural generalization of the estimation of ground states. The method has no free parameters and requires no explicit…

Computational Physics · Physics 2024-09-04 David Pfau , Simon Axelrod , Halvard Sutterud , Ingrid von Glehn , James S. Spencer

The distribution $P_1$ of the first many-body excitation energy of a weakly and moderately interacting electron gas in a finite conductor (in the diffusive regime) is calculated. As the interaction is increased, $P_1$ crosses over from…

Disordered Systems and Neural Networks · Physics 2009-11-10 Richard Berkovits , Yuval Gefen , Igor V. Lerner , Boris L. Altshuler

The phase stability and equilibria of carbon dioxide is investigated from 125 -- 325K and 1 -- 10,000 atm using extensive molecular dynamics (MD) simulations and the Two-Phase Thermodynamics (2PT) method. We devise a direct approach for…

Materials Science · Physics 2021-07-28 Amanda A. Chen , Alexandria Do , Tod A. Pascal

We propose a new symbolic algorithm and a C++ program for generating and calculating supersymmetric Feynman diagrams for ${\cal N}=1$ supersymmetric electrodynamics regularized by higher derivatives in four dimensions. According to standard…

High Energy Physics - Theory · Physics 2023-04-27 Ilya Shirokov

Most modern calculations of many-electron atoms use basis sets of atomic orbitals. An accurate account for the electronic correlations in heavy atoms is very difficult computational problem and optimization of the basis sets can reduce…

Atomic Physics · Physics 2024-01-17 M. G. Kozlov , Yu. A. Demidov , M. Y. Kaygorodov , E. V. Triapitsyna

Parity and time-reversal violating electric dipole moment (EDM) of $^{171}$Yb is calculated accounting for the electron correlation effects over the Dirac-Hartree-Fock (DHF) method in the relativistic Rayleigh-Schr\"odinger many-body…

Atomic Physics · Physics 2017-07-05 B. K. Sahoo , Yashpal Singh