Related papers: Phase Space Manipulation of Cold Free Radical OH M…
We demonstrate feedback control optimization for the Stark deceleration and trapping of neutral polar molecules using evolutionary strategies. In a Stark-decelerator beamline pulsed electric fields are used to decelerate OH radicals and…
Selection of "magic" trapping conditions with ultracold atoms or molecules, where pairs of internal states experience identical trapping potentials, brings substantial benefits to precision measurements and quantum computing schemes.…
We demonstrate how dynamic Stark control (DSC) can be achieved on molecular photodissociation in the dipole limit, using single-cycle (FWHM) laser pulses in the terahertz (THz) regime. As the laser-molecule interaction follows the…
We demonstrate the coherent optical bichromatic force on a molecule, the polar free radical strontium monohydroxide (SrOH). A dual-frequency retro-reflected laser beam addressing the $\tilde{X}^2\Sigma^+\leftrightarrow\tilde{A}^2\Pi_{1/2}$…
A broadband squeezed vacuum photon field is characterized by a complex squeezing function. We show that by controlling the wavelength dependence of its phase it is possible to change the dynamics of the atomic polarization interacting with…
The direct interaction of super-intense laser fields in the optical frequency domain with nuclei is studied. As main observable, we consider the nuclear AC-Stark shift of low-lying nuclear states due to the off-resonant excitation by the…
We use accurate quantum mechanical calculations to analyze the effects of parallel electric and magnetic fields on collision dynamics of OH(2Pi) molecules. It is demonstrated that spin relaxation in 3He-OH collisions at temperatures below…
Polar heavy-atom molecules have been well recognized as promising candidates for precision measurements and tests of fundamental physics. A much slower molecular beam to increase the interaction time should lead to a more sensitive…
The hydroxyl radical, hereafter referred to as the OH molecule (OHM), carries both electric and magnetic dipole moments and, as a diatomic molecule, admits a comparatively simple and accurate model. This makes it a natural quantum probe for…
Stark deceleration allows for precise control over the velocity of a pulsed molecular beam and, by the nature of its limited phase-space acceptance, reduces the energy width of the decelerated packet. We describe an alternate method of…
A strong inhomogeneous static electric field is used to spatially disperse a supersonic beam of polar molecules, according to their quantum state. We show that the molecules residing in the lowest-lying rotational states can be selected and…
We apply the theory of high-order harmonic generation by low-frequency laser fields in the strong field approximation to the study of the spatial and temporal coherence properties of the harmonics. We discuss the role of dynamically induced…
We consider the excitation dynamics of the two-photon \sts transition in a beam of atomic hydrogen by 243 nm laser radiation. Specifically, we study the impact of ionization damping on the transition line shape, caused by the possibility of…
Cold, neutral hydroxyl radicals are Stark decelerated and confined within a magnetic trap consisting of two permanent ring magnets. The OH molecules are trapped in the ro-vibrational ground state at a density of $\sim10^{6}$ cm$^{-3}$ and…
We propose to control light trapping in a large ensemble of cold atoms by an external, static magnetic field. For an appropriate choice of frequency and polarization of the exciting pulse, the field is expected to speed up the fluorescence…
We investigate the effect of far-off-resonant trapping light on ultracold bosonic RbCs molecules. We use kHz-precision microwave spectroscopy to measure the differential AC Stark shifts between the ground and first excited rotational levels…
We demonstrate that a bichromatic standing-wave laser field can exert a significantly larger force on a molecule than ordinary radiation pressure. Our experiment measures the deflection of a pulsed supersonic beam of CaF molecules by a…
We photoionize laser-cooled atoms with a laser beam possessing spatially periodic intensity modulations to create ultracold neutral plasmas with controlled density perturbations. Laser-induced fluorescence imaging reveals that the density…
Strong optical forces with minimal spontaneous emission are desired for molecular deceleration and atom interferometry applications. We report experimental benchmarking of such a stimulated optical force driven by ultrafast laser pulses. We…
We demonstrate a 1D magneto-optical trap of the polar free radical calcium monohydroxide (CaOH). A quasi-closed cycling transition is established to scatter $\sim 10^3$ photons per molecule, predominantly limited by interaction time. This…