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Molecular dynamics simulations for aqueous sodium chloride solutions were carried out at various concentrations. Supplementary to the Debye-H\"uckel theory, reversible transient nucleation of ions was observed even in dilute solutions. The…

Soft Condensed Matter · Physics 2014-11-26 Gan Ren , Yanting Wang

Using molecular dynamics simulations, we reveal emergent properties of hydrated electrode interfaces that while molecular in origin are integral to the behavior of the system across long times scales and large length scales. Specifically,…

Materials Science · Physics 2015-05-20 David T. Limmer , Adam P. Willard

The thermodynamics of strongly anisotropic crystalline surfaces is analogous to that of a binary mixture exhibiting phase separation. On a metastable planar surface, formation of stable orientations requires a nucleation process, in which…

Materials Science · Physics 2019-11-05 Thomas Philippe , Hervé Henry , Mathis Plapp

The electrolyte (comprising of solute ions and solvents) flow-through the porous media is frequently encountered in nature or in many engineering applications, such as the electrochemical systems, manufacturing of composites, oil…

Fluid Dynamics · Physics 2013-09-12 Chengjun Xu , Chin-Tsau Hsu

The traditional approach to nuclear physics encodes phase shift information in a nucleon-nucleon (NN) potential, producing a nucleon-level interaction that captures the sub-GeV consequences of QCD. A further reduction to the nuclear scale…

Nuclear Theory · Physics 2019-09-04 K. S. McElvain , W. C. Haxton

First order phase transitions proceed via nucleation. The rate of nucleation varies exponentially with the free-energy barrier to nucleation, and so is highly sensitive to variations in this barrier. In practice, very few systems are…

Statistical Mechanics · Physics 2009-11-10 Richard P. Sear

Homogeneous nucleation of the new phase of one transition near a second phase transition is considered. The system has two phase transitions, we study the nucleation of the new phase of one of these transitions under conditions such that we…

Statistical Mechanics · Physics 2009-11-07 Z. Tavassoli , R. P. Sear

Classical theory of the electric double layer is based on the fundamental assumption of a dilute solution of point ions. There are a number of situations such as high applied voltages, high concentration of electrolytes, systems with…

Fluid Dynamics · Physics 2015-06-11 Brian D. Storey , Martin Z. Bazant

An analytical model for the evolution of the boundary of the new phase in transformations ruled by nucleation and growth is presented. Both homogeneous and heterogeneous nucleation have been considered: The former includes transformations…

Materials Science · Physics 2020-08-26 Massimo Tomellini

The thermodynamics of the lattice model of intercalation of ions in crystals is considered in the mean field approximation. Pseudospin formalism is used for the description of interaction of electrons with ions and the possibility of…

Strongly Correlated Electrons · Physics 2009-07-08 T. S. Mysakovych , V. O. Krasnov , I. V. Stasyuk

The study of chemical reactions in environments under nonequilibrium conditions has been of interest recently in a variety of contexts, including current-induced reactions in molecular junctions and scanning tunneling microscopy…

Chemical Physics · Physics 2022-07-27 Yaling Ke , Christoph Kaspar , André Erpenbeck , Uri Peskin , Michael Thoss

While nucleation in typical active and driven fluids often appears equilibrium-like, striking departures emerge when large-scale fluctuations are strongly suppressed. Here, we investigate nucleation in nonequilibrium hyperuniform fluids by…

Statistical Mechanics · Physics 2026-04-22 Raphaël Maire

One-dimensional non-equilibrium models of particles subjected to a coagulation-diffusion process are important in understanding non-equilibrium dynamics, and fluctuation-dissipation relation. We consider in this paper transport properties…

Statistical Mechanics · Physics 2015-06-18 Jean-Yves Fortin

The nuclear tunneling crossover temperature ($T_c$) of hydrogen transfer reactions in supported molecular-switch architectures can lie close to room temperature. This calls for the inclusion of nuclear quantum effects (NQE) in the…

Chemical Physics · Physics 2020-11-25 Yair Litman , Mariana Rossi

Transition boiling is an intermediate regime occurring between nucleate boiling, where bubbles at the surface efficiently carry heat away, and film boiling, where a layer of vapor formed over the surface insulates the system reducing heat…

Entanglement may be considered a resource for quantum-information processing, as the origin of robust and universal equilibrium behaviour, but also as a limit to the validity of an effective potential approach, in which the influence of…

Quantum Physics · Physics 2009-11-07 J. Gemmer , G. Mahler

Nucleation is an out-of-equilibrium process, which can be strongly affected by the presence of external fields. In this letter, we report a simple extension of classical nucleation theory to systems submitted to an homogeneous shear flow.…

Statistical Mechanics · Physics 2013-06-17 Anatolii V. Mokshin , Bulat N. Galimzyanov , Jean-Louis Barrat

Classical nucleation theory (CNT), linking rare nucleation events to the free energy landscape of a growing nucleus, is central to understanding phase-change kinetics in passive fluids. Nucleation in non-equilibrium systems is much harder…

Soft Condensed Matter · Physics 2023-03-15 M. E. Cates , C. Nardini

Nucleation is an activated process in which the system has to overcome a free energy barrier in order for a first-order phase transition between the metastable and the stable phases to take place. In the liquid-to-solid transition the…

Soft Condensed Matter · Physics 2016-11-28 John Russo , Hajime Tanaka

Materials with nanoscale phase separation are considered. A system representing a heterophase mixture of ferromagnetic and paramagnetic phases is studied. After averaging over phase configurations, a renormalized Hamiltonian is derived…

Mesoscale and Nanoscale Physics · Physics 2021-12-21 V. I. Yukalov , E. P. Yukalova