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The recent development of electron sensitive and pixelated detectors has attracted the use of four-dimensional scanning transmission electron microscopy (4D-STEM). Here, we present a precession electron diffraction assisted 4D-STEM…
We report on the first observation of stimulated Raman scattering from a Lambda-type three-level atom, where the stimulation is realized by the vacuum field of a high-finesse optical cavity. The scheme produces one intracavity photon by…
The recently developed precession electron diffraction (PED) technique in scanning transmission electron microscopy (STEM) has been used to elucidate the local strain distribution and crystalline misorientation in CMOS fabricated strained…
Surface enhanced Raman scattering (SERS) exploits surface plasmons induced by the incident field in metallic nanostructures to significantly increase the Raman intensity. Graphene provides the ideal prototype two dimensional (2d) test…
We have performed polarized Raman scattering measurements on the newly discovered superconductor Ta$_{4}$Pd$_{3}$Te$_{16}$ ($T_c = 4.6$ K). We observe twenty-eight out of thirty-three Raman active modes, with frequencies in good accordance…
Ce-doped SiO x N y films are deposited by magnetron reactive sputtering from a CeO 2 target under nitrogen reactive gas atmosphere. Visible photoluminescence measurements regarding the nitrogen gas flow reveal a large emission band centered…
Raman amplification of a short laser pulse off a long laser beam has been demonstrated successfully for moderate probe intensities ($\sim 10^{16}$ W/cm$^2$) and widths ($\sim 50$ micron). However, truly competitive intensities can only be…
We report new experiments on polarization squeezing using ultrashort photonic pulses in a single pass of a birefringent fiber. We measure what is to our knowledge a record squeezing of -6.8 +/- 0.3 dB in optical fibers which when corrected…
Radon and its progenies are significant sources of background in rare event detection experiments, including dark matter searches like the PandaX-4T experiment and other rare decay studies such as neutrinoless double beta decay (NLDBD). In…
Surface enhanced Raman spectra from molecules (bipyridyl ethylene) adsorbed on gold dumbells are observed to become increasingly asymmetric (Fano-like) at higher incident light intensity. The electronic temperature (inferred from the…
Due to their high circulating intensities, ultra-high quality factor dielectric whispering-gallery mode resonators have enabled the development of low threshold Raman microlasers. Subsequently, other Raman-related phenomena, such as…
Raman and photoluminescence (PL) measurements were performed on suspended and supported MoS2 up to 6 trilayers (TLs). The difference in the dielectric environment of suspended and supported MoS2 does not lead to large differences in the PL…
We report on the generation of a Raman cascade spanning the wavelength range of 523 to 1750 nm wavelength range, in a standard telecommunication graded-index multimode optical fiber. Despite the highly multimode nature of the pump, the…
Laser-plasma accelerators offer a compact means of producing high-energy electron beams, but their performance is fundamentally limited by dephasing between the accelerated electrons and the plasma wave. To overcome this limitation, we…
Room temperature Terahertz stimulated emission and population inversion in optically pumped graphene is reported. We experimentally observe fast relaxation and relatively slow recombination dynamics of photogenerated electrons/holes in an…
High-power lasers with narrow linewidth and high beam quality in the visible spectrum are essential for emerging quantum and space technologies. Here we report significant advances in diamond Raman lasers, generating diffraction-limited…
Stimulated Raman scattering (SRS) microscopy allows for high-speed label-free chemical imaging of biomedical systems. The imaging sensitivity of SRS microscopy is limited to ~10 mM for endogenous biomolecules. Electronic pre-resonant SRS…
Metastable qubits in atomic systems can enable large-scale quantum computing by simplifying hardware requirements and adding efficient erasure conversion to the pre-existing toolbox of high-fidelity laser-based control. For trapped atomic…
Nanoscale strain control of exciton funneling is an increasingly critical tool for the scalable production of single photon emitters (SPEs) in two-dimensional materials. However, conventional far-field optical microscopies remain…
Single crystals of the optimally doped, moderately and strongly overdoped high temperature superconductor Tl2Ba2CuO6+x (Tl-2201) with Tc=80, 56 and 30K, respectively, have been investigated by polarized Raman scattering. By taking the peak…