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We use a numerically exact real-time path integral Monte Carlo scheme to compute electron transfer dynamics between two redox sites within a spin-boson approach. The case of asymmetric reactions is studied in detail in the least understood…

Condensed Matter · Physics 2009-11-10 L. Muehlbacher , R. Egger

The purpose of this article is to show a different way to calculate the electron transfer between atoms. It can be used as a base for calculating the minimal electricity, showed here by Joules, necessary for the transference of electrons.…

General Physics · Physics 2021-03-22 Matheus Barbiero Pillon

Close to equilibrium, the exchange of particles and heat between macroscopic systems at different temperatures and different chemical potentials is known to be governed by a matrix of transport coefficients which is positive and symmetric.…

Statistical Mechanics · Physics 2017-10-11 Euijin Jeon , Peter Talkner , Juyeon Yi , Yong Woon Kim

Electron transport through Si-C bound alkyl chains, sandwiched between n-Si and Hg, is characterized by two distinct types of barriers, each dominating in a different voltage range. At low voltage, current depends strongly on temperature…

Materials Science · Physics 2009-11-11 Adi Salomon , Olga Girshevitz , David Cahen , Till Bocking , Calvin K. Chan , Fabrice Amy , Antoine Kahn

This paper reports thermopower and conductivity measurements through the metal-insulator transition for 2-dimensional electron gases in high mobility Si-MOSFETs. At low temperatures both thermopower and conductivity show critical behaviour…

Strongly Correlated Electrons · Physics 2009-11-07 R. Fletcher , V. M. Pudalov , A. D. B. Radcliffe , C. Possanzini

The transmission of low-energy (<1.8eV) photoelectrons through the shell of core-shell aerosol particles is studied for liquid squalane, squalene, and DEHS shells. The photoelectrons are exclusively formed in the core of the particles by…

Soft Condensed Matter · Physics 2017-06-15 Stavros Amanatidis , Bruce L. Yoder , Ruth Signorell

We investigate nonradiative emission and absorption rates of two-level quantum emitters embedded in a metal at low temperatures. We obtain the expressions for both nonradiative transition rates and identify a unique, experimentally…

Mesoscale and Nanoscale Physics · Physics 2018-11-21 M. B. Silva Neto , F. M. D'Angelis , P. P. P. Foster , F. A. Pinheiro

Thermo-electric transport at the nano-scale is a rapidly developing topic, in particular in superconductor-based hybrid devices. In this review paper, we first discuss the fundamental principles of electronic cooling in mesoscopic…

Superconductivity · Physics 2015-06-19 Hervé Courtois , Frank W. J. Hekking , Hung Q. Nguyen , Clemens Winkelmann

Thermoelectric devices are heat engines, which operate as generators or refrigerators using the conduction electrons as a working fluid. The thermoelectric heat-to-work conversion efficiency has always been typically quite low, but much…

Statistical Mechanics · Physics 2016-11-11 G. Benenti , H. Ouerdane , C. Goupil

Vapour-deposited organic glasses are currently in use in many optoelectronic devices. Their operation temperature is limited by the glass transition temperature of the organic layers and thermal management strategies become increasingly…

Injection of photoelectrons into gaseous or liquid dielectrics is a widely used technique to produce cold plasmas in weakly ionized systems for investigating the transport properties of electrons. We report measurements of the collection…

Chemical Physics · Physics 2015-06-11 A. F. Borghesani , P. Lamp

Graphene and other 2D materials give a platform for electromechanical sensing of biomolecules in aqueous, room temperature environments. The electronic current changes in response to mechanical deflection, indicating the presence of forces…

Mesoscale and Nanoscale Physics · Physics 2019-04-19 Maicol A. Ochoa , Michael Zwolak

This letter reports thermopower and conductivity measurements through the metal-insulator transition for 2-dimensional electron gases in high mobility Si-MOSFET's. At low temperatures both thermopower and conductivity show critical behavior…

Disordered Systems and Neural Networks · Physics 2007-05-23 R. Fletcher , V. M. Pudalov , A. D. B. Radcliffe , C. Possanzini

Transition absorption of electromagnetic field energy by an electron passing through a boundary between two media with different dielectric permittivities is considered both classically and quantum mechanically. It is shown that transition…

Recent experiments have shown that highly efficient energy transfer can take place in organic nanocrystals at extremely low acceptor densities. This striking phenomenon has been ascribed to the formation of exciton polaritons thanks to the…

Chemical Physics · Physics 2021-01-12 R. Sáez-Blázquez , J. Feist , F. J. García-Vidal , A. I. Fernández-Domínguez

In the present work we theoretically analyze thermoelectric transport in single-molecule junctions (SMJ) characterized by strong interactions between electrons on the molecular linkers and phonons in their nuclear environments where…

Mesoscale and Nanoscale Physics · Physics 2024-01-17 Natalya A. Zimbovskaya

We non-perturbatively analyze the effect of electron-electron interactions on weak localization (WL) in relatively short metallic conductors with a tunnel barrier. We demonstrate that the main effect of interactions is electron dephasing…

Mesoscale and Nanoscale Physics · Physics 2008-07-01 D. S. Golubev , A. D. Zaikin

The electron transport properties of a four-terminal molecular device are computed within the framework of density functional theory and non-equilibrium Keldysh theory. The additional two terminals lead to new properties, including a…

Mesoscale and Nanoscale Physics · Physics 2009-09-01 Kamal K. Saha , Wenchang Lu , J. Bernholc , Vincent Meunier

In the quest for dynamic multimodal probing of a material's structure and functionality, it is critical to be able to quantify the chemical state on the atomic and nanoscale using element specific electronic and structurally sensitive tools…

We report a detailed analytic and numerical study of electronic thermal conductivity in d-wave superconductors. We compare theory of the cross over at low temperatures from T-dependence to T^3-dependence for increasing temperature with…

Superconductivity · Physics 2009-11-11 Tomas Lofwander , Mikael Fogelstrom