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Using molecular simulations and theory, we develop an explicit mapping of the contribution of molecular relaxation modes in glassy thermosets to the shear modulus, where the relaxations were tuned by altering the polarity of side groups.…

Materials Science · Physics 2019-10-15 Robert M. Elder , Alessio Zaccone , Timothy W. Sirk

In view of the important role helix-sheet transitions play in protein aggregation, we introduce a simple model to study secondary structural transitions of helix-coil-sheet systems using a Potts model starting with an effective Hamiltonian.…

Biological Physics · Physics 2011-11-09 John S. Schreck , Jian-Min Yuan

The free surface of glassy polymers exhibits enhanced segmental dynamics compared to the bulk, forming a liquid-like layer that lowers the glass transition temperature (Tg) in nanometersized polymer samples. Recent studies have shown that…

Soft Condensed Matter · Physics 2025-05-12 Xinyu Zhang , Christian Pedersen , Haoqi Zhu , Siming Wang , Yuchen Fu , Liang Dai , Andreas Carlson , Thomas Salez , Yu Chai

The structure of the hot downstream region below a radiative accretion shock, such as that of an accreting compact object, may oscillate due to a global thermal instability. The oscillatory behaviour depends on the functional forms of the…

Astrophysics · Physics 2009-10-31 Curtis J. Saxton , Kinwah Wu

We present results from our simulations of biopolymer translocation in a solvent which explain the main experimental findings. The forced translocation can be described by simple force balance arguments for the relevant range of pore…

Biological Physics · Physics 2009-05-08 V. V. Lehtola , R. P. Linna , K. Kaski

We show that the approach to asymptotic fluctuation-induced critical behavior in polymer solutions is governed by a competition between a correlation length diverging at the critical point and an additional mesoscopic length-scale, the…

Soft Condensed Matter · Physics 2009-11-07 M. A. Anisimov , A. F. Kostko , J. V. Sengers

We simulate the compression of a two-component Lennard-Jones liquid at a variety of constant temperatures using a molecular dynamics algorithm in an isobaric-isothermal ensemble. The viscosity of the liquid increases with pressure,…

chem-ph · Physics 2009-10-22 Shelly L. Shumway , Andrew S. Clarke , Hannes Jónsson

Anion exchange membranes are used in alkaline fuel cells and offer a promising alternative to the more expensive proton exchange membrane fuel cells. However, hydroxide ion conductivity in anion exchange membranes is low, and the quest for…

Soft Condensed Matter · Physics 2024-04-16 Mohammed Al Otmi , Ping Lin , William Schertzer , Coray M. Colina , Rampi Ramprasad , Janani Sampath

We report dynamic Monte Carlo simulation on conformational transition of H-shaped branched polymers by varying main chain (backbone) and side chain (branch) length. H-shaped polymers in comparison with equivalent linear polymers exhibit a…

Soft Condensed Matter · Physics 2015-06-17 Ashok Kumar Dasmahapatra , Venkata Mahanth Sanka

We develop a theoretical and computational approach to deal with systems that involve a disparate range of spatio-temporal scales, such as those comprised of colloidal particles or polymers moving in a fluidic molecular environment. Our…

Soft Condensed Matter · Physics 2017-10-27 Adwait V. Datar , Maria Fyta , Umberto Marini Bettolo Marconi , Simone Melchionna

A coarse-grained multi-blob description of polymer solutions is presented, based on soft, transferable effective interactions between bonded and non-bonded blobs. The number of blobs is chosen such that the blob density does not exceed…

Soft Condensed Matter · Physics 2009-11-13 Carlo Pierleoni , Barbara Capone , Jean-Pierre Hansen

We analytically investigate the dynamic behavior of an an-isotropic active Brownian particle under various stochastic resetting protocols in two dimensions. The motion of shape-asymmetric active Brownian particles in two dimensions leads to…

Statistical Mechanics · Physics 2025-11-26 Anirban Ghosh , Sudipta Mandal , Subhasish Chaki

A coarse-grained molecular dynamics model of linear polyethylene-like polymer chain system was built to investigate the responds of structure and mechanical properties during uniaxial deformation. The influence of chain length, temperature,…

Soft Condensed Matter · Physics 2020-05-19 Cheng Li , Yingrui Shang , Huan Xu , Jinqing Li , Shichun Jiang

We consider a molecular junction immersed in a solvent where the electron transfer is dominated by Marcus-type steps. However, the successive nature of the charge transfer through the junction does not imply that the solvent reach thermal…

Statistical Mechanics · Physics 2022-03-23 Henning Kirchberg , Abraham Nitzan

The properties of butane (C4H10) lubricants confined between two approaching solids are investigated by a model that accounts for the curvature and elastic properties of the solid surfaces. We consider the linear n-butane and the branched…

Materials Science · Physics 2007-05-23 Ugo Tartaglino , Ion M. Sivebaek , Bo N. J. Persson , Erio Tosatti

We present a numerical study of polyelectrolytes electrophoresing in free solution while squeezed by an axisymmetric confinement force transverse to their net displacement. Hybrid multi-particle collision dynamics and molecular dynamics…

Soft Condensed Matter · Physics 2016-06-22 Tyler N. Shendruk , Martin Bertrand , Gary W. Slater

We study the non-equilibrium coarsening dynamics of a binary liquid solvent around a colloidal particle in a presence of a time-dependent temperature gradient that emerges after temperature quench of a suitably coated colloid surface. The…

Soft Condensed Matter · Physics 2018-11-30 Sutapa Roy , Anna Maciolek

We study numerically the crystallization of a hard-sphere mixture with 8\% polydispersity. Although often used as a model glass former, for small system sizes we observe crystallization in molecular dynamics simulations. This opens the…

Soft Condensed Matter · Physics 2016-09-05 Matteo Campo , Thomas Speck

We use large scale molecular dynamics simulations of the isomerizations of azobenzene molecules diluted inside a simple molecular material, to investigate the effect of a modification of the cis isomer shape on the induced diffusion…

Soft Condensed Matter · Physics 2017-12-05 Victor Teboul

The rapid collapse of a polymer, due to external forces or changes in solvent, yields a long-lived `crumpled globule.' The conjectured fractal structure shaped by hierarchical collapse dynamics has proved difficult to establish, even with…

Soft Condensed Matter · Physics 2015-10-07 Guy Bunin , Mehran Kardar