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Understanding how to produce forces using biomolecular building blocks is essential for the development of adaptive synthetic cells and living materials. Here we ask whether a dynamic polymer system can generate deformation forces in soft…

Soft Condensed Matter · Physics 2024-11-13 Dino Osmanovic , Elisa Franco

Constitutive equations are derived for the time-dependent behavior of particle-reinforced elastomers at isothermal loading with finite strains. A rubbery polymer is modelled as a network of macromolecules bridged by junctions which can slip…

Materials Science · Physics 2007-05-23 Aleksey D. Drozdov , Al Dorfmann

Using molecular dynamics simulations, we provide chain-level insights into the dissimilarities in rearrangements of polymers under uniaxial tensile and compressive deformation in glassy and semicrystalline samples of varying chain lengths.…

Soft Condensed Matter · Physics 2019-01-23 Sara Jabbari-Farouji , Damien Vandembroucq

I develop a kinetic mechanism to explain chain folding in polymer crystallization which is based on the competition between the formation of stems, which is due to frequent occupations of trans states along the chains in the supercooled…

Soft Condensed Matter · Physics 2014-09-23 S. Stepanow

This paper adopts a previously developed activation model of shear thickening, published by the authors, to sterically stabilized colloidal suspensions. When particles arranged along the compression axis of a sheared suspension, they may…

Soft Condensed Matter · Physics 2012-07-12 Joachim Kaldasch , Bernhard Senge

The equilibrium properties of polymer droplets on a soft deformable surface are investigated by molecular dynamics simulations of a bead-spring model. The surface consists of a polymer brush with irreversibly end-tethered linear homopolymer…

Soft Condensed Matter · Physics 2015-05-28 Fabien Léonforte , Marcus Müller

We investigate the dissipative mechanisms exhibited by creased material sheets when subjected to mechanical loading, which comes in the form of plasticity and relaxation phenomena within the creases. After demonstrating that plasticity…

Soft Condensed Matter · Physics 2020-09-30 Théo Jules , Frédéric Lechenault , Mokhtar Adda-Bedia

We consider a stiff polymer chain in poor solvent and apply a force at one end of the chain. We find that by varying the stiffness parameter, polymer undergoes a transition from the globule state to the folded like state. The conformation…

Soft Condensed Matter · Physics 2015-05-13 Sanjay Kumar , Debaprasad Giri

In a recent letter, a simple method was proposed to generate solvable models that predict the critical properties of statistical systems in hyperspherical geometries. To that end, it was shown how to reduce a random walk in $D$ dimensions…

High Energy Physics - Lattice · Physics 2018-07-06 S. Boettcher

Living tissues show an extraordinary adaptiveness to strain, which is crucial for their proper biological functioning. The physical origin of this mechanical behaviour has been widely investigated using reconstituted networks of collagen…

Soft Condensed Matter · Physics 2019-02-25 Federica Burla , Justin Tauber , Simone Dussi , Jasper van der Gucht , Gijsje H. Koenderink

We report molecular dynamics simulations of a system of repulsive, polymer-tethered colloidal particles. We use an explicit polymer model to explore how the length and the behavior of the polymer (ideal or self-avoiding) affect the ability…

Soft Condensed Matter · Physics 2015-05-14 Behnaz Bozorgui , Maya Sen , William L. Miller , Josep C. Pamies , Angelo Cacciuto

Self-consistent field approach is used to model a single end-tethered polymer chain on a substrate subject to various forces in three dimensions. Starting from a continuous Gaussian chain model, the following perturbations are considered:…

We investigate the crumpling of a sheet as it is repeatedly crushed onto itself by rolling it into a cylinder and twisting it axially while allowing the end-to-end length to evolve freely. As deduced from its plastic deformations, the sheet…

Soft Condensed Matter · Physics 2025-01-22 Amit Dawadi , Arshad Kudrolli

Hydrophobically modified polymers are good candidates for the stabilization of liquid interfaces thanks to the high anchoring energy of the hydrophobic parts. In this article we probe the interfacial anchoring of a series of home-made…

Applied Physics · Physics 2019-03-04 C. Trégouët , Thomas Salez , N. Pantoustier , P. Perrin , M. Reyssat , C. Monteux

This study focused on the expansion in polydisperse granular materials owing to mechanical annealing, which involved compression and decompression. Following minor annealing, the polydisperse systems exhibited compaction as well as the…

Soft Condensed Matter · Physics 2024-09-04 Daisuke S. Shimamoto , Miho Yanagisawa

Glassy polymers show strain hardening: at constant extensional load, their flow first accelerates, then arrests. Recent experiments have found this to be accompanied by a striking and unexplained dip in the segmental relaxation time. Here…

Soft Condensed Matter · Physics 2015-05-30 S. M. Fielding , R. G. Larson , M. E. Cates

The progressive onset of slip at the wall, which corresponds to a slip length increasing with the solicitation time before reaching a plateau, has been investigated for model viscoelastic polymer solutions, allowing one to vary the longest…

Understanding surface mechanics of soft solids, such as soft polymeric gels, is crucial in many engineering processes, such as dynamic wetting and adhesive failure. In these situations, a combination of capillary and elastic forces drives…

Soft Condensed Matter · Physics 2020-12-02 Qin Xu , Lawrence A. Wilen , Katharine E. Jensen , Robert W. Style , Eric R. Dufresne

We analyze equilibrium properties and adsorption desorption phase transition behaviour of a linear semiflexible copolymer chain under constrained geometrical situation on square lattice in a good solvent. One dimensional stair shaped line…

Statistical Mechanics · Physics 2010-06-04 Pramod Kumar Mishra

Predicting the large-amplitude deformations of thin elastic sheets is difficult due to the complications of self-contact, geometric nonlinearities, and a multitude of low-lying energy states. We study a simple two-dimensional setting where…