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Experimental and numerical investigation of single-beam and pump-probe interaction with a resonantly absorbing dense extended medium under strong and weak field-matter coupling is presented. Significant probe beam amplification and conical…

A method based on optical interferences for measuring optical nonlinearities is presented. In a proof-of-principle experiment, the technique is applied to the experimental determination of the intensity dependence of the photoionization…

Optics · Physics 2013-08-06 F. Billard , P. Béjot , E. Hertz , B. Lavorel , O. Faucher

Optical pump-probe spectroscopy is a powerful tool for the study of non-equilibrium electronic dynamics and finds wide applications across a range of fields, from physics and chemistry to material science and biology. However, a shortcoming…

In recent years, electro-optic sampling, which is based on Pockel's effect between an electromagnetic mode and a copropagating, phase-matched ultrashort probe, has been largely used for the investigation of broadband quantum states of…

Quantum Physics · Physics 2023-10-03 Francesca Fabiana Settembrini , Alexa Herter , Jèrôme Faist

This paper attempts a probe into negative refraction without absorption by means of an incoherent pump field and a strong coherent field coupling the dense four-level atomic system.With the application of the incoherent pump field to…

Quantum Physics · Physics 2024-03-05 Shun-Cai Zhao , Zheng-Dong Liu , Qi-Xuan Wu

Nonlinear optics experiments measuring phase shifts induced in a weak probe pulse by a strong pump pulse must account for coherent effects that only occur when the pump and probe pulses are temporally overlapped. It is well known that a…

Conditional Measurement scheme which employs linear optical elements and photon detection is the fertile ground for nonclassical state generation. We consider a simple setup that requires a coherent state and a number state as inputs of the…

Quantum Physics · Physics 2024-12-30 Devibala Esakkimuthu , Basherrudin Mahmud Ahmed A

Twin entangled beams produced by single-pass parametric down-conversion (PDC) offer the opportunity to detect weak amount of absorption with an improved sensitivity with respect to standard techniques which make use of classical light…

Quantum Physics · Physics 2009-11-13 E. Brambilla , L. Caspani , O. Jedrkiewicz , L. A. Lugiato , A. Gatti

Nonlinear frequency conversion provides an elegant method to detect photons in a spectral range which differs from the pump wavelength, making it highly attractive for photons with inherently low energy. Aside from the intensity of the…

Optics · Physics 2022-02-10 Tobias Pfeiffer , Jens Klier , Georg von Freymann , Daniel Molter

A numerical method to calculate optical conductivity based on a pump-probe setup is presented. Its validity and limits are tested and demonstrated via the concrete numerical simulations on the half-filled one-dimensional extended Hubbard…

Strongly Correlated Electrons · Physics 2016-05-26 Can Shao , Takami Tohyama , Hong-Gang Luo , Hantao Lu

We develop a theoretical model for calibrating the absorption imaging of cold atoms under high magnetic fields. Comparing to zero or low magnetic fields, the efficiency of the absorption imaging becomes lower while it requires an additional…

Atomic Physics · Physics 2023-07-20 Yuqi Liu , Zhongchi Zhang , Shiwan Miao , Zihan Zhao , Huaichuan Wang , Wenlan Chen , Jiazhong Hu

Nonlinear spectroscopy is widely used to study the transient dynamics of molecules under strong light-matter coupling, though it remains unclear to what extent uncoupled intracavity molecules obscure signals from the strongly-coupled…

Chemical Physics · Physics 2026-04-08 Alexander M. McKillop , Marissa L. Weichman

We report on the study of the third-order nonlinear optical interactions in In$_{x}$Ga$_{1-x}$As$_{y}$P$_{1-y}$/InP strip-loaded waveguides. The material composition and waveguide structures were optimized for enhanced nonlinear optical…

Standard optical pump-probe methods analyze a system's temporal response to a laser pulse within sub-femtoseconds to several nanoseconds, constrained by the optical delay line's length. While resistance is a sensitive detector in various…

Instrumentation and Detectors · Physics 2024-04-26 M. I. Blumenau , A. Yu. Kuntsevich

We demonstrate optical pump/THz probe (OPTP) spectroscopy with a variable external magnetic field (0-9 T) in which the time-dependent THz signal is measured by echelon-based single-shot detection at a 1 kHz repetition rate. The method…

Accurate absorption models for gases at high pressure and temperature support advanced optical combustion diagnostics and aid in the study of harsh planetary atmospheres. Developing and validating absorption models for these applications…

Multi-photon absorption processes have a nonlinear dependence on the amplitude of the incident optical field i.e. the number of photons. However, multi-photon absorption is generally weak and multi-photon events occur with extremely low…

The photomolecular effect has been hypothesized to enhance evaporation of water at visible wavelengths. This study develops a measurement technique to investigate its presence and magnitude at the liquid-vapor interface of water. The…

Optics · Physics 2026-03-19 Preston Bohm , Mingjun Li , Akanksha K. Menon , Zhuomin M. Zhang

Many applications seek to measure a sample's absorption coefficient spectrum to retrieve the chemical makeup. Many real world samples are optically turbid, causing scattering confounds which many commercial spectrometers cannot address.…

Optics · Physics 2023-01-05 Giles Blaney , Angelo Sassaroli , Sergio Fantini

The determination of the nonlinear optical coefficient \( n_2 \) of pure water is of great interest for applications such as imaging biological systems, performing femtosecond laser surgery, and underwater ablation. Traditionally, probing…

Optics · Physics 2025-02-06 Ilyes Betka